High-order harmonic generation from polyatomic molecules including nuclear motion and a nuclear modes analysis

We present a generic approach for treating the effect of nuclear motion in the high-order harmonic generation from polyatomic molecules. Our procedure relies on a separation of nuclear and electron dynamics where we account for the electronic part using the Lewenstein model and nuclear motion enters as a nuclear correlation function. We express the nuclear correlation function in terms of Franck-Condon factors which allows us to decompose nuclear motion into modes and identify the modes that are dominant in the high-order harmonic generation process. We show results for the isotopes CH$_4$ and CD$_4$ and thereby provide direct theoretical support for a recent experiment [Baker {\it et al.}, Science {\bf 312}, 424 (2006)] that uses high-order harmonic generation to probe the ultra-fast structural nuclear rearrangement of ionized methane.Comment: 6 pages, 6 figure

Zero-Point cooling and low heating of trapped 111Cd+ ions

We report on ground state laser cooling of single 111Cd+ ions confined in radio-frequency (Paul) traps. Heating rates of trapped ion motion are measured for two different trapping geometries and electrode materials, where no effort was made to shield the electrodes from the atomic Cd source. The low measured heating rates suggest that trapped 111Cd+ ions may be well-suited for experiments involving quantum control of atomic motion, including applications in quantum information science.Comment: 4 pages, 6 figures, Submitted to PR

Manipulating the torsion of molecules by strong laser pulses

A proof-of-principle experiment is reported, where torsional motion of a molecule, consisting of a pair of phenyl rings, is induced by strong laser pulses. A nanosecond laser pulse spatially aligns the carbon-carbon bond axis, connecting the two phenyl rings, allowing a perpendicularly polarized, intense femtosecond pulse to initiate torsional motion accompanied by an overall rotation about the fixed axis. The induced motion is monitored by femtosecond time-resolved Coulomb explosion imaging. Our theoretical analysis accounts for and generalizes the experimental findings.Comment: 4 pages, 4 figures, submitted to PRL; Major revision of the presentation of the material; Correction of ion labels in Fig. 2(a

Strong Orientation Effects in Ionization of H2+_2^+ by Short, Intense, High-Frequency Light Sources

We present three dimensional time-dependent calculations of ionization of arbitrarily spatially oriented H$_2^+$ by attosecond, intense, high-frequency laser fields. The ionization probability shows a strong dependence on both the internuclear distance and the relative orientation between the laser field and the internuclear axis.Comment: 4 pages, 4 figure

Unemployment in the OECD : Models and Mysteries

This paper compares models used to explain OECD unemployment. The models suggest that the ?natural rate of unemployment? has been driven up mainly by wage push factors. Panel data on twenty-two OECD countries are used to investigate the explanatory power of these models over the past two decades. Our estimates reveal that coefficients on key variables often turn out with signs which are at odds with the theories or are insignificant and that a second order autoregressive model performs nearly as well as all the other models. The conclusion offers some directions for future research

Electronic structure of the ferromagnetic superconductor UCoGe from first principles

The superconductor UCoGe is analyzed with electronic structure calculations using Linearized Augmented Plane Wave method based on Density Functional Theory. Ferromagnetic and antiferromagnetic calculations with and without correlations (via LDA+U) were done. In this compound the Fermi level is situated in a region where the main contribution to DOS comes from the U-5f orbital. The magnetic moment is mainly due to the Co-3d orbital with a small contribution from the U-5f orbital. The possibility of fully non-collinear magnetism in this compound seems to be ruled out. These results are compared with the isostructural compound URhGe, in this case the magnetism comes mostly from the U-5f orbital

Production of Strange Clusters and Strange Matter in Nucleus-Nucleus Collisions at the AGS

Production probabilities for strange clusters and strange matter in Au+Au collisions at AGS energy are obtained in the thermal fireball model. The only parameters of the model, the baryon chemical potential and temperature, were determined from a description of the rather complete set of hadron yields from Si+nucleus collisions at the AGS. For the production of light nuclear fragments and strange clusters the results are similar to recent coalescence model calculations. Strange matter production with baryon number larger than 10 is predicted to be much smaller than any current experimental sensitivities.Comment: 9 Pages (no figures