17 research outputs found
Observation of anomalous decoherence effect in a quantum bath at room temperature
Decoherence of quantum objects is critical to modern quantum sciences and
technologies. It is generally believed that stronger noises cause faster
decoherence. Strikingly, recent theoretical research discovers the opposite
case for spins in quantum baths. Here we report experimental observation of the
anomalous decoherence effect for the electron spin-1 of a nitrogen-vacancy
centre in high-purity diamond at room temperature. We demonstrate that under
dynamical decoupling, the double-transition can have longer coherence time than
the single-transition, even though the former couples to the nuclear spin bath
as twice strongly as the latter does. The excellent agreement between the
experimental and the theoretical results confirms the controllability of the
weakly coupled nuclear spins in the bath, which is useful in quantum
information processing and quantum metrology.Comment: 22 pages, related paper at http://arxiv.org/abs/1102.557
Ultrafast control of donor-bound electron spins with single detuned optical pulses
The ability to control spins in semiconductors is important in a variety of
fields including spintronics and quantum information processing. Due to the
potentially fast dephasing times of spins in the solid state [1-3], spin
control operating on the picosecond or faster timescale may be necessary. Such
speeds, which are not possible to attain with standard electron spin resonance
(ESR) techniques based on microwave sources, can be attained with broadband
optical pulses. One promising ultrafast technique utilizes single broadband
pulses detuned from resonance in a three-level Lambda system [4]. This
attractive technique is robust against optical pulse imperfections and does not
require a fixed optical reference phase. Here we demonstrate the principle of
coherent manipulation of spins theoretically and experimentally. Using this
technique, donor-bound electron spin rotations with single-pulse areas
exceeding pi/4 and two-pulses areas exceeding pi/2 are demonstrated. We believe
the maximum pulse areas attained do not reflect a fundamental limit of the
technique and larger pulse areas could be achieved in other material systems.
This technique has applications from basic solid-state ESR spectroscopy to
arbitrary single-qubit rotations [4, 5] and bang-bang control[6] for quantum
computation.Comment: 15 pages, 4 figures, submitted 12/2008. Since the submission of this
work we have become aware of related work: J. Berezovsky, M. H. Mikkelsen, N.
G. Stoltz, L. A. Coldren, and D. D. Awschalom, Science 320: 349-352 (2008
Nuclear spin pair coherence in diamond for atomic scale magnetometry
The nitrogen-vacancy (NV) centre, as a promising candidate solid state system
of quantum information processing, its electron spin coherence is influenced by
the magnetic field fluctuations due to the local environment. In pure diamonds,
the environment consists of hundreds of C-13 nuclear spins randomly spreading
in several nanometers range forming a spin bath. Controlling and prolonging the
electron spin coherence under the influence of spin bath are challenging tasks
for the quantum information processing. On the other hand, for a given bath
distribution, many of its characters are encoded in the electron spin
coherence. So it is natural to ask the question: is it possible to 'decode' the
electron spin coherence, and extract the information about the bath structures?
Here we show that, among hundreds of C-13 bath spins, there exist strong
coupling clusters, which give rise to the millisecond oscillations of the
electron spin coherence. By analyzing these oscillation features, the key
properties of the coherent nuclear spin clusters, such as positions,
orientations, and coupling strengths, could be uniquely identified. This
addressability of the few-nuclear-spin cluster extends the feasibility of using
the nuclear spins in diamond as qubits in quantum computing. Furthermore, it
provides a novel prototype of single-electron spin based, high-resolution and
ultra-sensitive detector for the chemical and biological applications.Comment: 15 pages, 4 figures, Nature Nanotechnology (2011
A Diamond Nanowire Single Photon Antenna
The development of a robust light source that emits one photon at a time is
an outstanding challenge in quantum science and technology. Here, at the
transition from many to single photon optical communication systems, fully
quantum mechanical effects may be utilized to achieve new capabilities, most
notably perfectly secure communication via quantum cryptography. Practical
implementations place stringent requirements on the device properties,
including stable photon generation, room temperature operation, and efficient
extraction of many photons. Single photon light emitting devices based on
fluorescent dye molecules, quantum dots, and carbon nanotube material systems
have all been explored, but none have simultaneously demonstrated all criteria.
Here, we describe the design, fabrication, and characterization of a bright
source of single photons consisting of an individual Nitrogen-vacancy color
center (NV center) in a diamond nanowire operating in ambient conditions. The
nanowire plays a positive role in increasing the number of single photons
collected from the NV center by an order of magnitude over devices based on
bulk diamond crystals, and allows operation at an order of magnitude lower
power levels. This result enables a new class of nanostructured diamond devices
for room temperature photonic and quantum information processing applications,
and will also impact fields as diverse as biological and chemical sensing,
opto-mechanics, and scanning-probe microscopy.Comment: 16 pages, 4 figures, v2: Includes improved reference list; modified
figure 1 to show a large array of NW and FDTD simulation of field profile;
direct experimental comparsion of several bulk/NW devices in figure
Enhanced Single Photon Emission from a Diamond-Silver Aperture
We have developed a scalable method for coupling single color centers in
diamond to plasmonic resonators and demonstrated Purcell enhancement of the
single photon emission rate of nitrogen-vacancy (NV) centers. Our structures
consist of single nitrogen-vacancy (NV) center-containing diamond nanoposts
embedded in a thin silver film. We have utilized the strong plasmon resonances
in the diamond-silver apertures to enhance the spontaneous emission of the
enclosed dipole. The devices were realized by a combination of ion implantation
and top-down nanofabrication techniques, which have enabled deterministic
coupling between single NV centers and the plasmonic modes for multiple devices
in parallel. The plasmon-enhanced NV centers exhibited over six-fold
improvements in spontaneous emission rate in comparison to bare nanoposts and
up to a factor of 3.6 in radiative lifetime reduction over bulk samples, with
comparable increases in photon counts. The hybrid diamond-plasmon system
presented here could provide a stable platform for the implementation of
diamond-based quantum information processing and magnetometry schemes.Comment: 16 pages, 4 figure