271 research outputs found
Charge modulations vs. strain waves in resonant x-ray scattering
A method is described for using resonant x-ray scattering to separately
quantify the charge (valence) modulation and the strain wave associated with a
charge density wave. The essence of the method is a separation of the atomic
form factor into a "raw" amplitude, fR(w), and a valence-dependent amplitude,
fD(w), which in many cases may be determined independently from absorption
measurements. The advantage of this separation is that the strain wave follows
the quantity |fR(w) + fD(w)|^2 whereas the charge modulation follows only
|fD(w)|^2. This allows the two distinct modulations to be quantified
separately. A scheme for characterizing a given CDW as Peierls-like or
Wigner-like naturally follows. The method is illustrated for an idealized model
of a one-dimensional chain.Comment: 6 pages, 4 figure
Evidence of 1D behaviour of He confined within carbon-nanotube bundles
We present the first low-temperature thermodynamic investigation of the
controlled physisorption of He gas in carbon single-wall nanotube (SWNT)
samples. The vibrational specific heat measured between 100 mK and 6 K
demonstrates an extreme sensitivity to outgassing conditions. For bundles with
a few number of NTs the extra contribution to the specific heat, C,
originating from adsorbed He at very low density displays 1D behavior,
typical for He atoms localized within linear channels as grooves and
interstitials, for the first time evidenced. For larger bundles, C
recovers the 2D behaviour akin to the case of He films on planar
substrates (grafoil).Comment: 4 pages, 3 figures, submitted to Phys. Rev. Let
Relaxation time spectrum of low-energy excitations in one- and two-dimensional materials with charge or spin density waves
The long-time thermal relaxation of (TMTTF)Br, SrCuO
and SrCaCuO single crystals at temperatures below 1 K
and magnetic field up to 10 T is investigated. The data allow us to determine
the relaxation time spectrum of the low energy excitations caused by the
charge-density wave (CDW) or spin-density wave (SDW). The relaxation time is
mainly determined by a thermal activated process for all investigated
materials. The maximum relaxation time increases with increasing magnetic
field. The distribution of barrier heights corresponds to one or two Gaussian
functions. The doping of SrCaCuO with Ca leads to
a drastic shift of the relaxation time spectrum to longer time. The maximum
relaxation time changes from 50 s (x = 0) to 3000 s (x = 12) at 0.1 K and 10 T.
The observed thermal relaxation at x=12 clearly indicates the formation of the
SDW ground state at low temperatures
Current-driven orbital order-disorder transition in LaMnO3
We report significant influence of electric current on the orbital
order-disorder transition in LaMnO3. The transition temperature T_OO, thermal
hysteresis in the resistivity (rho) versus temperature (T) plot around T_OO,
and latent heat L associated with the transition decrease with the increase in
current density. Eventually, at a critical current density, L reaches zero. The
transition zone, on the other hand, broadens with the increase in current
density. The states at ordered, disordered, and transition zone are all found
to be stable within the time window from ~10^-3 to ~10^4 seconds.Comment: 7 pages including 5 figures; resolution of Fig.1 is better here than
the published versio
Phase transition and phase diagram at a general filling in the spinless one-dimensional Holstein Model
Among the mechanisms for lattice structural deformation, the electron-phonon
interaction mediated Peierls charge-density-wave (CDW) instability in single
band low-dimensional systems is perhaps the most ubiquitous. The standard
mean-field picture predicts that the CDW transition occurs at all fillings and
all values of the electron-phonon coupling and the adiabaticity parameter
. Here, we correct the mean-field expression for the Peierls
instability condition by showing that the non-interacting static
susceptibility, at twice the Fermi momentum, should be replaced by the dynamic
one. We derive the Luttinger liquid (LL) to CDW transition condition, {\it
exact to second order in a novel blocked perturbative approach}, for the
spinless one-dimensional Holstein model in the adiabatic regime. The small
parameter is the ratio . We present the phase diagram at
non-half-filling by obtaining the surprising result that the CDW occurs in a
more restrictive region of a two parameter ( and )
space than at half-filling.Comment: Made changes in the appendices and also in notatio
Sliding charge-density-wave in two-dimensional rare-earth tellurides
Nonlinear transport properties are reported in the layered DyTe compound
at temperature below the charge-density-wave (CDW) transition, K.
Conductivity is increasing sharply above the threshold electric field. Under
application of a rf field Shapiro steps are clearly observed. These features
demonstrate for the first time CDW sliding in two-dimensional compounds.Comment: 4 pages, 4 figure
Fractional power-law susceptibility and specific heat in low temperature insulating state of o-TaS_{3}
Measurements of the magnetic susceptibility and its anisotropy in the
quasi-one-dimensional system o-TaS_{3} in its low-T charge density wave (CDW)
ground state are reported. Both sets of data reveal below 40 K an extra
paramagnetic contribution obeying a power-law temperature dependence
\chi(T)=AT^{-0.7}. The fact that the extra term measured previously in specific
heat in zero field, ascribed to low-energy CDW excitations, also follows a
power law C_{LEE}(0,T)=CT^{0.3}, strongly revives the case of random exchange
spin chains. Introduced impurities (0.5% Nb) only increase the amplitude C, but
do not change essentially the exponent. Within the two-level system (TLS)
model, we estimate from the amplitudes A and C that there is one TLS with a
spin s=1/2 localized on the chain at the lattice site per cca 900 Ta atoms. We
discuss the possibility that it is the charge frozen within a soliton-network
below the glass transition T_{g}~40 K determined recently in this system.Comment: 7 pages, 3 figures, submitted to Europhysics Letter
Electronic Instability in a Zero-Gap Semiconductor: The Charge-DensityWave in (TaSe4)(2)I
We report a comprehensive study of the paradigmatic quasi-1D compound (TaSe4)(2)I performed by means of angle-resolved photoemission spectroscopy (ARPES) and first-principles electronic structure calculations. We find it to be a zero-gap semiconductor in the nondistorted structure, with non-negligible interchain coupling. Theory and experiment support a Peierls-like scenario for the charge-density wave formation below T-CDW = 263 K, where the incommensurability is a direct consequence of the finite interchain coupling. The formation of small polarons, strongly suggested by the ARPES data, explains the puzzling semiconductor-to-semiconductor transition observed in transport at T-CDW.open114sciescopu
Equilibrium Low Temperature Heat Capacity of the Spin Density Wave compound (TMTTF)2 Br: effect of a Magnetic Field
We have investigated the effect of the magnetic field (B) on the very
low-temperature equilibrium heat capacity ceq of the quasi-1 D organic compound
(TMTTF)2Br, characterized by a commensurate Spin Density Wave (SDW) ground
state. Below 1K, ceq is dominated by a Schottky-like contribution, very
sensitive to the experimental time scale, a property that we have previously
measured in numerous DW compounds. Under applied field (in the range 0.2- 7 T),
the equilibrium dynamics, and hence ceq extracted from the time constant,
increases enormously. For B = 2-3 T, ceq varies like B2, in agreement with a
magnetic Zeeman coupling. Another specific property, common to other
Charge/Spin density wave (DW) compounds, is the occurrence of metastable
branches in ceq, induced at very low temperature by the field exceeding a
critical value. These effects are discussed within a generalization to SDWs in
a magnetic field of the available Larkin-Ovchinnikov local model of strong
pinning. A limitation of the model when compared to experiments is pointed out.Comment: 10 pages, 11 figure
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