Realistic many-body models for Manganese Monoxide under pressure

In materials like transition metals oxides where electronic Coulomb correlations impede a description in terms of standard band-theories, the application of genuine many-body techniques is inevitable. Interfacing the realism of density-functional based methods with the virtues of Hubbard-like Hamiltonians, requires the joint ab initio construction of transfer integrals and interaction matrix elements (like the Hubbard U) in a localized basis set. In this work, we employ the scheme of maximally localized Wannier functions and the constrained random phase approximation to create effective low-energy models for Manganese monoxide, and track their evolution under external pressure. We find that in the low pressure antiferromagnetic phase, the compression results in an increase of the bare Coulomb interaction for specific orbitals. As we rationalized in recent model considerations [Phys. Rev. B 79, 235133 (2009)], this seemingly counter-intuitive behavior is a consequence of the delocalization of the respective Wannier functions. The change of screening processes does not alter this tendency, and thus, the screened on-site component of the interaction - the Hubbard U of the effective low-energy system - increases with pressure as well. The orbital anisotropy of the effects originates from the orientation of the orbitals vis-a-vis the deformation of the unit-cell. Within the high pressure paramagnetic phase, on the other hand, we find the significant increase of the Hubbard U is insensitive to the orbital orientation and almost exclusively owing to a substantial weakening of screening channels upon compression.Comment: 13 pages, 6 figure

Space charge and charge trapping characteristics of cross-linked polyethylene subjected to ac electric stresses

This paper reports on the result of space charge evolution in cross-linked polyethylene (XLPE) planar samples of approximately 220 ?m thick. The space charge measurement technique used in this study is the PEA method. There are two phases to this experiment. In the first phase, the samples were subjected to dc 30 kVdc/mm and ac (sinusoidal) electric stress level of 30 kVpk/mm at frequencies of 1 Hz, 10 Hz and 50 Hz ac. In addition, ac space charge under 30 kVrms/mm and 60 kVpk/mm electric stress at 50 Hz was also investigated. The volts off results showed that the amount of charge trapped in XLPE sample under dc electric stress is significantly bigger than samples under ac stress even when the applied ac stresses are substantially higher. The second phase of the experiment involves studying the dc space charge evolution in samples that were tested under ac stress during the first phase of the experiment. Ac ageing causes positive charge to become more dominant over negative charge. It was also discovered that ac ageing creates deeper traps, particularly for negative charge. This paper also gave a brief overview of the data processing methods used to analyse space charge under ac electric stress

Realization of odd-frequency p-wave spin-singlet superconductivity coexisting with antiferromagnetic order near quantum critical point

A possibility of the realization of the p-wave spin-singlet superconductivity ($p$SS), whose gap function is odd both in momentum and in frequency, is investigated by solving the gap equation with the phenomenological interaction mediated by the antiferromagnetic spin fluctuation. The $p$SS is realized prevailing over the d-wave singlet superconductivity ($d$SS) in the vicinity of antiferromagnetic quantum critical pint (QCP) both on the paramagnetic and on the antiferromagnetic sides. Off the QCP in the paramagnetic phase, however, the $d$SS with line-nodes is realized as \textit{conventional} anisotropic superconductivity. For the present $p$SS state, there is no gap in the quasiparticle spectrum everywhere on the Fermi surface due to its odd frequency. These features can give a qualitative understanding of the anomalous behaviors of NQR relaxation rate on CeCu$_2$Si$_2$ or CeRhIn$_5$ where the antiferromagnetism and superconductivity coexist on a microscopic level.Comment: 20 pages with 12 figures. To appear in J. Phys. Soc. Jpn. Vol. 72, No. 1

Low-energy excitations in electron-doped metal phthalocyanine from NMR in Li0.5_{0.5}MnPc

$^7$Li and $^1$H NMR and magnetization measurements in \lpc (Pc$\equiv$C$_{32}$H$_{16}$N$_8$), recently proposed as a strongly correlated metal, are presented. Two different low-frequency dynamics are evidenced. The first one, probed by $^1$H nuclei gives rise to a slowly relaxing magnetization at low temperature and is associated with the freezing of MnPc $S=3/2$ spins. This dynamic is similar to the one observed in pristine $\beta$-MnPc and originates from Li depleted chain segments. The second one, evidenced by $^7$Li spin-lattice relaxation rate, is associated with the hopping of the electrons along Li-rich chains. The characteristic correlation times for the two dynamics are derived and the role of disorder is briefly discussed.Comment: 7 two-columns pages, 11 figure

A theory of new type of heavy-electron superconductivity in PrOs_4Sb_12: quadrupolar-fluctuation mediated odd-parity pairings

It is shown that unconventional nature of superconducting state of PrOs_4Sb_12, a Pr-based heavy electron compound with the filled-Skutterudite structure, can be explained in a unified way by taking into account the structure of the crystalline-electric-field (CEF) level, the shape of the Fermi surface determined by the band structure calculation, and a picture of the quasiparticles in f$^{2}$-configuration with magnetically singlet CEF ground state. Possible types of pairing are narrowed down by consulting recent experimental results. In particular, the chiral "p"-wave states such as p_x+ip_y is favoured under the magnetic field due to the orbital Zeeman effect, while the "p"-wave states with two-fold symmetery such as p_x can be stabilized by a feedback effect without the magnetic field. It is also discussed that the double superconducting transition without the magnetic field is possible due to the spin-orbit coupling of the "triplet" Cooper pairs in the chiral state.Comment: 12 pages, 2 figures, submitted to J. Phys.: Condens. Matter Lette

Real-space observation of current-driven domain wall motion in submicron magnetic wires

Spintronic devices, whose operation is based on the motion of a magnetic domain wall (DW), have been proposed recently. If a DW could be driven directly by flowing an electric current instead of a magnetic field, the performance and functions of such device would be drastically improved. Here we report real-space observation of the current-driven DW motion by using a well-defined single DW in a micro-fabricated magnetic wire with submicron width. Magnetic force microscopy (MFM) visualizes that a single DW introduced in the wire is displaced back and forth by positive and negative pulsed-current, respectively. We can control the DW position in the wire by tuning the intensity, the duration and the polarity of the pulsed-current. It is, thus, demonstrated that spintronic device operation by the current-driven DW motion is possible.Comment: Accepted and published in PR