3 research outputs found
Unusual magnetic relaxation behavior in La0.5Ca0.5MnO3 and Nd0.5Sr0.5MnO3
We have carried out a systematic magnetic relaxation study, measured after
applying and switching off a 5 T magnetic field to polycrystalline samples of
La0.5Ca0.5MnO3 and Nd0.5Sr0.5MnO3. The long time logarithmic relaxation rate
(LTLRR), decreased from 10 K to 150 K and increased from 150 K to 195 K in
La0.5Ca0.5MnO3. This change in behavior was found to be related to the complete
suppression of the antiferromagnetic phase above 150 K and in the presence of a
5 T magnetic field. At 195 K, the magnetization first decreased, and after a
few minutes increased slowly as a function of time. Moreover, between 200 K and
245 K, the magnetization increased throughout the measured time span. The
change in the slope of the curves, from negative to positive at about 200 K was
found to be related to the suppression of antiferromagnetic fluctuations in
small magnetic fields. A similar temperature dependence of the LTLRR was found
for the Nd0.5Sr0.5MnO3 sample. However, the temperature where the LTLRR reached
the minimum in Nd0.5Sr0.5MnO3 was lower than that of La0.5Ca0.5MnO3. This
result agrees with the stronger ferromagnetic interactions that exist in
Nd0.5Sr0.5MnO3 in comparison to La0.5Ca0.5MnO3. The above measurements
suggested that the general temperature dependence of the LTLRR and the
underlying physics were mainly independent of the particular charge ordering
system considered. All relaxation curves could be fitted using a logarithmic
law at long times. This slow relaxation was attributed to the coexistence of
ferromagnetic and antiferromagnetic interactions between Mn ions, which
produced a distribution of energy barriers.Comment: Accepted to PRB as a regular article, 10 figures, Scheduled Issue: 01
June 200