Probing quantum-mechanical level repulsion in disordered systems by means of time-resolved selectively-excited resonance fluorescence

We argue that the time-resolved spectrum of selectively-excited resonance fluorescence at low temperature provides a tool for probing the quantum-mechanical level repulsion in the Lifshits tail of the electronic density of states in a wide variety of disordered materials. The technique, based on detecting the fast growth of a fluorescence peak that is red-shifted relative to the excitation frequency, is demonstrated explicitly by simulations on linear Frenkel exciton chains.Comment: 4 pages, 4 figures, to appear in Phys. Rev. Let

Low-temperature dynamics of weakly localized Frenkel excitons in disordered linar chains

We calculate the temperature dependence of the fluorescence Stokes shift and the fluorescence decay time in linear Frenkel exciton systems resulting from the thermal redistribution of exciton population over the band states. The following factors, relevant to common experimental conditions, are accounted for in our kinetic model: (weak) localization of the exciton states by static disorder, coupling of the localized excitons to vibrations in the host medium, a possible non-equilibrium of the subsystem of localized Frenkel excitons on the time scale of the emission process, and different excitation conditions (resonant or non resonant). A Pauli master equation, with microscopically calculated transition rates, is used to describe the redistribution of the exciton population over the manifold of localized exciton states. We find a counterintuitive non-monotonic temperature dependence of the Stokes shift. In addition, we show that depending on experimental conditions, the observed fluorescence decay time may be determined by vibration-induced intra-band relaxation, rather than radiative relaxation to the ground state. The model considered has relevance to a wide variety of materials, such as linear molecular aggregates, conjugated polymers, and polysilanes.Comment: 15 pages, 8 figure

Particle Event Generator: A Simple-in-Use System PEGASUS version 1.0

PEGASUS is a parton-level Monte-Carlo event generator designed to calculate cross sections for a wide range of hard QCD processes at high energy $pp$ and $p\bar p$ collisions, which incorporates the dynamics of transverse momentum dependent (TMD) parton distributions in a proton. Being supplemented with off-shell production amplitudes for a number of partonic subprocesses and provided with necessary TMD gluon density functions, it produces weighted or unweighted event records which can be saved as a plain data file or a file in a commonly used Les Houches Event format. A distinctive feature of PEGASUS is an intuitive and extremely user friendly interface, allowing one to easily implement various kinematical cuts into the calculations. Results can be also presented "on the fly" with built-in tool \textsc{pegasus plotter}. A short theoretical basis is presented and detailed program description is given.Comment: 24 pages, 8 figure

Localization properties of one-dimensional Frenkel excitons: Gaussian versus Lorentzian diagonal disorder

We compare localization properties of one-dimensional Frenkel excitons with Gaussian and Lorentzian uncorrelated diagonal disorder. We focus on the states of the Lifshits tail, which dominate the optical response and low-temperature energy transport in molecular J-aggregates. The absence of exchange narrowing in chains with Lorentzian disorder is shown to manifest itself in the disorder scaling of the localization length distribution. Also, we show that the local exciton level structure of the Lifshits tail differs substantially for these two types of disorder: In addition to the singlets and doublets of localized states near the bare band edge, strongly resembling those found for Gaussian disorder, for Lorentzian disorder two other types of states are found in this energy region as well, namely multiplets of three or four states localized on the same chain segment and isolated states localized on short segments. Finally, below the Lifshits tail, Lorentzian disorder induces strongly localized exciton states, centered around low energy sites, with localization properties that strongly depend on energy. For Gaussian disorder with a magnitude that does not exceed the exciton bandwidth, the likelihood to find such very deep states is exponentially small.Comment: 9 two-column pages, 4 figures, to appear in Phys. Rev.

Leptonic origin of the 100 MeV gamma-ray emission from the Galactic Centre

The Galactic centre is a bright gamma-ray source with the GeV-TeV band spectrum composed of two distinct components in the 1-10 GeV and 1-10 TeV energy ranges. The nature of these two components is not clearly understood. We investigate the gamma-ray properties of the Galactic centre to clarify the origin of the observed emission. We report imaging, spectral, and timing analysis of data from 74 months of observations of the Galactic centre by FERMI/LAT gamma-ray telescope complemented by sub-MeV data from approximately ten years of INTEGRAL/PICsIT observations. We find that the Galactic centre is spatially consistent with the point source in the GeV band. The tightest 3 sigma upper limit on its radius is 0.13 degree in the 10-300 GeV energy band. The spectrum of the source in the 100 MeV energy range does not have a characteristic turnover that would point to the pion decay origin of the signal. Instead, the source spectrum is consistent with a model of inverse Compton scattering by high-energy electrons. In this a model, the GeV bump in the spectrum originates from an episode of injection of high-energy particles, which happened ~300 years ago. This injection episode coincides with the known activity episode of the Galactic centre region, previously identified using X-ray observations. The hadronic model of source activity could be still compatible with the data if bremsstrahlung emission from high-energy electrons was present in addition to pion decay emission.Comment: To match the accepted versio