386 research outputs found
Hysteresis loops and adiabatic Landau-Zener-St\"uckelberg transitions in the magnetic molecule V
We have observed hysteresis loops and abrupt magnetization steps in the
magnetic molecule V, where each molecule comprises a pair of identical spin
triangles, in the temperature range 1-5 K for external magnetic fields with
sweep rates of several Tesla/ms executing a variety of closed cycles. The
hysteresis loops are accurately reproduced using a generalization of the Bloch
equation based on direct one-phonon transitions between the instantaneous
Zeeman-split levels of the ground state (an doublet) of each spin
triangle. The magnetization steps occur for and they are explained
in terms of adiabatic Landau-Zener-St\"{u}ckelberg transitions between the
lowest magnetic energy levels as modified by inter-triangle anisotropic
exchange of order 0.4 K.Comment: 4 pages, 3 figure
Quantum Monte Carlo Study on Magnetization Processes
A quantum Monte Carlo method combining update of the loop algorithm with the
global flip of the world line is proposed as an efficient method to study the
magnetization process in an external field, which has been difficult because of
inefficiency of the update of the total magnetization. The method is
demonstrated in the one dimensional antiferromagnetic Heisenberg model and the
trimer model. We attempted various other Monte Carlo algorithms to study
systems in the external field and compared their efficiency.Comment: 5 pages, 9 figures; added references for section 1, corrected typo
Nonlocal Landau theory of the magnetic phase diagram of highly frustrated magnetoelectric CuFeO
A nonlocal Landau-type free energy functional of the spin density is
developed to model the large variety of magnetic states which occur in the
magnetic field-temperature phase diagram of magnetoelectric CuFeO.
Competition among long-range quadratic exchange, biquadratic anti-symmetric
exchange, and trigonal anisotropy terms, consistent with the high-temperature
rhombohedral Rm crystal symmetry, are shown to all play important
roles in stabilizing the unusual combination of commensurate and incommensurate
spin structures in this highly frustrated triangular antiferromagnet. It is
argued that strong magnetoelastic coupling is largely responsible for the
nonlocal nature of the free energy. A key feature of the analysis is that an
electric polarization is induced by a canting of the non-collinear
incommensurate spin structure. Application of the model to ordered spin states
in the triangular antiferromagnets MnBr and NaFeO is also discussed.Comment: 20 pages, 2 figure
High Magnetic Field Behaviour of the Triangular Lattice Antiferromagnet, CuFeO_2
The high magnetic field behaviour of the triangular lattice antiferromagnet
CuFeO_2 is studied using single crystal neutron diffraction measurements in a
field of up to 14.5 T and also by magnetisation measurements in a field of up
to 12 T. At low temperature, two well-defined first order magnetic phase
transitions are found in this range of applied magnetic field (H // c): at
H_c1=7.6(3)/7.1(3) T and H_c2=13.2(1)/12.7(1) T when ramping the field up/down.
In a field above H_c2 the magnetic Bragg peaks show unusual history dependence.
In zero field T_N1=14.2(1) K separates a high temperature paramagnetic and an
intermediate incommensurate structure, while T_N2=11.1(3) K divides an
incommensurate phase from the low-temperature 4-sublattice ground state. The
ordering temperature T_N1 is found to be almost field independent, while T_N2
decreases noticeably in applied field. The magnetic phase diagram is discussed
in terms of the interactions between an applied magnetic field and the highly
frustrated magnetic structure of CuFeO_2Comment: 7 pages, 8 figures in ReVTeX. To appear in PR
Neutron Scattering Study of Temperature-Concentration Phase Diagram of (Cu1-xMgx)GeO3
In doped CuGeO3 systems, such as (Cu1-xZnx)GeO3 and Cu(Ge1-xSix)O3, the
spin-Peierls (SP) ordering (T<Tsp) coexists with the antiferromagnetic (AF)
phase (T<TN<Tsp). Tsp decreases while TN increases with increasing x in low
doping region. For higher x, however, the SP state disappears and only the AF
state remains. These features are common for all the doped CuGeO3 systems so
far studied, indicating the existence of universal T-x phase diagram. Recently,
Masuda et al. carried out comprehensive magnetic susceptibility (chi)
measurements of (Cu1-xMgx)GeO3, in which doping concentration can be controlled
significantly better than the Zn doped systems. They found that TN suddenly
jumps from 3.43 to 3.98K at the critical concentration xc sim 0.023 and that a
drop in chi corresponding to the SP ordering also disappears at x>xc. They thus
concluded that there is a compositional phase boundary between two distinct
magnetic phases. To clarify the nature of two phases, we performed
neutron-scattering measurements on (Cu1-xMgx)GeO3 single crystals with various
x. Analysis of the data at fixed temperature points as a function of doping
concentration has revealed sudden changes of order parameters at the critical
concentration xc=0.027 +- 0.001. At finite temperatures below TN, the drastic
increase of the AF moment takes place at xc. The spin-Peierls order parameter
delta associated with lattice dimerization shows a precipitous decrease at all
temperature below Tsp. However, it goes to zero above xc only at the low
temperature limit.Comment: 9 pages, 9 figure
Large-Scale Numerical Evidence for Bose Condensation in the S=1 Antiferromagnetic Chain in a Strong Field
Using the recently proposed density matrix renormalization group technique we
show that the magnons in the S=1 antiferromagnetic Heisenberg chain effectively
behaves as bosons that condense at a critical field h_c.Comment: 12 pages, REVTEX 3.0, 3 postscript figures appended, UBCTP-93-00
Exact Analysis of ESR Shift in the Spin-1/2 Heisenberg Antiferromagnetic Chain
A systematic perturbation theory is developed for the ESR shift and is
applied to the spin-1/2 Heisenberg chain. Using the Bethe ansatz technique, we
exactly analyze the resonance shift in the first order of perturbative
expansion with respect to an anisotropic exchange interaction. Exact result for
the whole range of temperature and magnetic field, as well as asymptotic
behavior in the low-temperature limit are presented. The obtained g-shift
strongly depends on magnetic fields at low temperature, showing a significant
deviation from the previous classical result.Comment: 4 pages, 3 figures,to be published in Phys. Rev. Let
Theory of Low Temperature Electron Spin Resonance in Half-integer Spin Antiferromagnetic Chains
A theory of low temperature (T) electron spin resonance (ESR) in half-integer
spin antiferromagnetic chains is developed using field theory methods and
avoiding previous approximations. It is compared to experiments on Cu benzoate.
Power laws are predicted for the line-width broadening due to various types of
anisotropy. At T -> 0, zero width absorption peaks occur in some cases. The
second ESR peak in Cu benzoate, observed at T<.76K, is argued not to indicate
Neel order as previously claimed, but to correspond to a sine-Gordon "breather"
excitation.Comment: 4 pages, REVTEX, 3 PostScript figures embedded in tex
Vortex-induced topological transition of the bilinear-biquadratic Heisenberg antiferromagnet on the triangular lattice
The ordering of the classical Heisenberg antiferromagnet on the triangular
lattice with the the bilinear-biquadratic interaction is studied by Monte Carlo
simulations. It is shown that the model exhibits a topological phase transition
at a finite-temperature driven by topologically stable vortices, while the spin
correlation length remains finite even at and below the transition point. The
relevant vortices could be of three different types, depending on the value of
the biquadratic coupling. Implications to recent experiments on the triangular
antiferromagnet NiGaS is discussed
- …