1,144 research outputs found
Meiotic recombination proteins localize to linear elements in Schizosaccharomyces pombe
Peer reviewedPostprin
Magnetic susceptibility of the frustrated spinels ZnCr2O4, MgCr2O4 and CdCr2O4
We analyzed the magnetic susceptibilities of several Cr spinels using two
recent models for the geometrically frustrated pyrochlore lattice, the Quantum
Tetrahedral Mean Field model and a Generalized Constant Coupling model. Both
models can describe the experimental data for ACr2 O4 (with A = Zn, Mg, and Cd)
satisfactorily, with the former yielding a somewhat better agreement with
experiment for A = Zn, Mg. The obtained exchange constants for nearest and
next-nearest neighbors are discussed.Comment: 4 pages, 1 figure, 1 table, conferenc
Large and Small Polaron Excitations in La2/3(Sr/Ca)1/3MnO3 Films
We present detailed optical measurements of the mid-infrared (MIR)
excitations in thin films of La2/3Sr1/3MnO3 (LSMO) and La2/3Ca1/3MnO3 (LCMO)
across the magnetic transition. The shape of the excitation at about 0.2 eV in
both samples is analyzed in terms of polaron models. We propose to identify the
MIR resonance in LSMO as the excitation of large polarons and that in LCMO as a
small polaron excitation. A scaling behavior for the low-energy side of the
polaronic MIR resonance in LSMO is established
Tuning orbital-selective correlation effects in superconducting RbFeSeS
We report on terahertz time-domain spectroscopy on superconducting and
metallic iron chalcogenides RbFeSeS. The
superconducting transition is reduced from 32 K () to 22 K
(), and finally suppressed () by isoelectronic substitution of Se
with S. Dielectric constant and optical conductivity exhibit a
metal-to-insulator transition associated with an orbital-selective Mott phase.
This orbital-selective Mott transition appears at higher temperature
with increasing sulfur content, identifying sulfur substitution as an efficient
parameter to tune orbital-dependent correlation effects in iron-chalcogenide
superconductors. The reduced correlations of the charge carriers can
account for the suppression of the superconductivity and the pseudogap-like
feature between and that was observed for .Comment: 6 pages, 4 figure
Multiferroicity and colossal magneto-capacitance in Cr-thiospinels
The sulfur based Cr-spinels RCr2S4 with R = Cd and Hg exhibit the coexistence
of ferromagnetic and ferroelectric properties together with a pronounced
magnetocapacitive coupling. While in CdCr2S4 purely ferromagnetic order is
established, in HgCr2S4 a bond-frustrated magnetic ground state is realized,
which, however, easily can be driven towards a ferromagnetic configuration in
weak magnetic fields. This paper shall review our recent investigation for both
compounds. Besides the characterization of the magnetic properties, the complex
dielectric permittivity was studied by means of broadband dielectric
spectroscopy as well as measurements of polarization hysteresis and
pyro-currents. The observed colossal magneto-capacitive effect at the magnetic
transition seems to be driven by an enormous variation of the relaxation
dynamics.Comment: 10 pages, 11 figure
Study of one-dimensional nature of (Sr,Ba)_2Cu(PO_4)_2 and BaCuP_2O_7 via 31P NMR
The magnetic behavior of the low-dimensional phosphates (Sr,Ba)_2 Cu(PO_4)_2
and BaCuP_2O_7 was investigated by means of magnetic susceptibility and ^{31}P
nuclear magnetic resonance (NMR) measurements. We present here the NMR shift
K(T), the spin-lattice 1/T_1 and spin-spin 1/T_2 relaxation-rate data over a
wide temperature range 0.02 K < T < 300 K. The T-dependence of the NMR K(T) is
well described by the S=1/2 Heisenberg antiferromagnetic chain model with an
intrachain exchange of J/k_B = 165 K, 151 K, and 108 K in Sr_2Cu(PO_4)_2,
Ba_2Cu(PO_4)_2, and BaCuP_2O_7, respectively. Our measurements suggest the
presence of magnetic ordering at 0.8 K in BaCuP_2O_7 (J/k_B = 108 K). For all
the samples, we find that 1/T_1 is nearly T-independent at low-temperatures (1
K < T < 10 K), which is theoretically expected for 1D chains when relaxation is
dominated by fluctuations of the staggered susceptibility. At high
temperatures, 1/T_1 varies nearly linearly with temperature
Multiferroic behavior in CdCr2X4 (X = S, Se)
The recently discovered multiferroic material CdCr2S4 shows a coexistence of
ferromagnetism and relaxor ferroelectricity together with a colossal
magnetocapacitive effect. The complex dielectric permittivity of this compound
and of the structurally related CdCr2Se4 was studied by means of broadband
dielectric spectroscopy using different electrode materials. The observed
magnetocapacitive coupling at the magnetic transition is driven by enormous
changes of the relaxation dynamics induced by the development of magnetic
order
Colossal magnetocapacitance and colossal magnetoresistance in HgCr2S4
We present a detailed study of the dielectric and charge transport properties
of the antiferromagnetic cubic spinel HgCr2S4. Similar to the findings in
ferromagnetic CdCr2S4, the dielectric constant of HgCr2S4 becomes strongly
enhanced in the region below 60 - 80 K, which can be ascribed to polar
relaxational dynamics triggered by the onset of ferromagnetic correlations. In
addition, the observation of polarization hysteresis curves indicates the
development of ferroelectric order below about 70 K. Moreover, our
investigations in external magnetic fields up to 5 T reveal the simultaneous
occurrence of magnetocapacitance and magnetoresistance of truly colossal
magnitudes in this material.Comment: 4 pages, 4 figure
Spin-phonon coupling in antiferromagnetic chromium spinels
The temperature dependence of eigenfrequencies and intensities of the IR
active modes has been investigated for the antiferromagnetic chromium spinel
compounds CdCr2O4, ZnCr2O4, ZnCr2S4, ZnCr2Se4, and HgCr2S4 by IR spectroscopy
for temperatures from 5 K to 300 K. At the transition into the magnetically
ordered phases, and driven by spin-phonon coupling, most compounds reveal
significant splittings of the phonon modes. This is true for geometrically
frustrated CdCr2O4, and ZnCr2O4, for bond frustrated ZnCr2S4 and for ZnCr2Se4,
which also is bond frustrated, but dominated by ferromagnetic exchange. The
pattern of splitting is different for the different compounds and crucially
depends on the nature of frustration and of the resulting spin order. HgCr2S4,
which is almost ferromagnetic, exhibits no splitting of the eigenfrequencies,
but shows significant shifts due to ferromagnetic spin fluctuations.Comment: 15 pages, 6 figure
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