Few-femtosecond phase-sensitive detection of infrared electric fields with a third-order nonlinearity

Abstract Measuring an electric field waveform beyond radio frequencies is often accomplished via a second-order nonlinear interaction with a laser pulse shorter than half of the field’s oscillation period. However, synthesizing such a gate pulse is extremely challenging when sampling mid- (MIR) and near- (NIR) infrared transients. Here, we demonstrate an alternative approach: a third-order nonlinear interaction with a relatively long multi-cycle pulse directly retrieves an electric-field transient whose central frequency is 156 THz. A theoretical model, exploring the different nonlinear frequency mixing processes, accurately reproduces our results. Furthermore, we demonstrate a measurement of the real part of a sample’s dielectric function, information that is challenging to retrieve in time-resolved spectroscopy and is therefore often overlooked. Our method paves the way towards experimentally simple MIR-to-NIR time-resolved spectroscopy that simultaneously extracts the spectral amplitude and phase information, an important extension of optical pump-probe spectroscopy of, e.g., molecular vibrations and fundamental excitations in condensed-matter physics

Ultrabroadband out-of-loop characterization of the carrier-envelope phase noise of an offset-free Er:fiber frequency comb

Recent demonstrations of passively phase-locked fiber-based combs motivate broadband characterization of the noise associated with the stabilized carrier-envelope offset frequency. In our study, we analyze the phase noise of a 100 MHz Er:fiber system in a wide range spanning from microhertz to the Nyquist frequency. An interferometric detection method enables analysis of the high-frequency output of an f-to-2f interferometer. The dominant contribution of a broadband white noise floor at high frequencies attests quantum-limited performance. An out-of-loop measurement of the carrier-envelope phase reveals its jitter to be as low as 250 mrad when integrated over 12 orders of magnitude of the radio-frequency spectrum.publishe

Deterministic Nonlinear Transformations of Phase Noise in Quantum-Limited Frequency Combs

Optical phase noise of femtosecond lasers is analyzed over various steps of broadband nonlinear frequency conversion. The intrinsic phase jitter of our system originates from quantum statistics in the mode-locked oscillator. Supercontinuum generation by four-wave-mixing processes preserves a noise minimum at the optical carrier frequency. From there, a quadratic increase of the comb linewidth results with mutually anticorrelated phase fluctuations of both spectral wings. Passive phase locking by difference frequency generation strongly enhances the optical phase noise to a level equaling the carrier-envelope phase jitter of the fundamental comb. The same value results from quadratic extrapolation of the optical phase noise to radio frequencies. Our findings are consistent with a fully deterministic transformation of phase noise according to the elastic tape model.publishe

Free-running performance and full control of a passively phase-stable Er:fiber frequency comb

Optical frequency combs based on erbium-doped fiber lasers are attractive tools in precision metrology due to their inherent compactness and stability. Here we study a femtosecond Er:fiber comb that passively eliminates the carrier–envelope phase slip by difference frequency generation. Quantum statistics inside the all-fiber soliton oscillator governs its free-running performance. Active stabilization of the repetition rate supports a subhertz optical linewidth and does not necessitate additional intracavity elements. Direct locking to an optical atomic frequency standard enables generation of a 100 MHz microwave signal with a stability of 3.4 mHz maintained over 15 min

Ultrabroadband suppression of mid-infrared reflection losses of a layered semiconductor by nanopatterning with a focused ion beam

Moth-eye structures are patterned onto gallium selenide surfaces with sub-micrometer precision. In this way, Fresnel reflection losses are suppressed to below one percent within an ultrabroad optical bandwidth from 15 to 65 THz. We tune the geometry by rigorous coupled-wave analysis. Subsequently, ablation with a Ga+ ion beam serves to write optimized structures in areas covering 30 by 30 μm. The benefits are demonstrated via optical rectification of femtosecond laser pulses under tight focusing, resulting in emission of phase-stable transients in the mid-infrared. We analyze the performance of antireflection coating directly in the time domain by ultrabroadband electro-optic sampling.publishe

Broadband analysis and self-control of spectral fluctuations in a passively phase-stable Er-doped fiber frequency comb

Carrier-envelope and optical phase noise of a femtosecond frequency comb based on Er-doped fiber technology is investigated and minimized without exploiting active external references. Ultrabroadband, coherent, and tailorable supercontinua are generated in a highly nonlinear germanosilicate fiber assembly. Difference frequency mixing between comb modes in their spectral extrema passively eliminates the carrier-envelope phase slip. This step generates an inherently offset-free comb with a relative frequency stability better than 10−21. In contrast, the phase fluctuations at the carrier frequency of 193 THz are increased as compared to the fundamental comb. Their level matches the value found by parabolic extrapolation of the phase noise of the fundamental comb to zero frequency. The latter is unambiguously accessible by means of any beat note centered at the carrier-envelope offset frequency. All these findings rely on strong correlations between the comb modes that are quantitatively described by an elastic tape model, underlining the deterministic character of the processes involved. The superior optical phase noise of the fundamental comb is transferred to the difference-frequency comb while not compromising the inherent cancellation of the carrier-envelope offset frequency. In this way, the optical linewidth of the passively phase-locked comb is reduced from 100 kHz to a measured value of 5 kHz, which is limited by the cw laser reference used for out-of-loop characterization.publishe