Precise measurement of the 222Rn half-life: a probe to monitor the stability of radioactivity

We give the results of a study on the 222Rn decay we performed in the Gran Sasso Laboratory (LNGS) by detecting the gamma rays from the radon progeny. The motivation was to monitor the stability of radioactivity measuring several times per year the half-life of a short lifetime (days) source instead of measuring over a long period the activity of a long lifetime (tens or hundreds of years) source. In particular, we give a possible reason of the large periodical fluctuations in the count rate of the gamma rays due to radon inside a closed canister which has been described in literature and which has been attributed to a possible influence of a component in the solar irradiation affecting the nuclear decay rates. We then provide the result of four half-life measurements we performed underground at LNGS in the period from May 2014 to January 2015 with radon diffused into olive oil. Briefly, we did not measure any change of the 222Rn half-life with a 8*10^-5 precision. Finally, we provide the most precise value for the 222Rn half-life: 3.82146(16){stat}(4){syst} days.Comment: Accepted for publication in Physics Letters B, 6 pages, 6 figure

Search for correlations between solar flares and decay rate of radioactive nuclei

The deacay rate of three different radioactive sources 40K, 137Cs and natTh has been measured with NaI and Ge detectors. Data have been analyzed to search for possible variations in coincidence with the two strongest solar flares of the years 2011 and 2012. No significant deviations from standard expectation have been observed, with a few 10-4 sensitivity. As a consequence, we could not find any effect like that recently reported by Jenkins and Fischbach: a few per mil decrease in the decay rate of 54Mn during solar flares in December 2006.Comment: 5 pages, 3 figure

Search for time modulations in the decay rate of 40K and 232Th

Time modulations at per mil level have been reported to take place in the decay constant of about 15 nuclei with period of one year (most cases) but also of about one month or one day. In this paper we give the results of the activity measurement of a 40K source and a 232Th one. The two experiments have been done at the Gran Sasso Laboratory during a period of about 500 days, above ground (40K) and underground (232Th) with a target sensitivity of a few parts over 10^5. We also give the results of the activity measurement at the time of the X-class solar flares which took place in May 2013. Briefly, our measurements do not show any evidence of unexpected time dependence in the decay rate of 40K and 232Th.Comment: version accepted for publication (Astroparticle Physics

Low level γ-ray germanium-spectrometer to measure very low primordial radionuclide concentrations

Abstract A new germanium spectrometer especially suited for large sample measurements is described in detail. It is operated in the Gran Sasso underground laboratory under shielding rock of 3300 m water equivalent, which reduces the muon flux by six orders of magnitude. The integral background counting rate in the energy range from 50 to 2750 keV is about 0.15 min−1. The low peak count rates of mostly less than 1 count per day together with a relative efficiency of 102% and the high sample capacity makes this spectrometer one of the most sensitive worldwide. Some sample measurements for the solar neutrino experiment BOREXINO and the detector efficiency calibration by the Monte Carlo method are discussed as well

First limits on double beta decays in 232^{\bf 232}Th

As one of the primordial radioactive isotopes, $^{232}$Th mainly undergoes $\alpha$-decay with a half-life of $1.402 \times 10^{10}$ yr. However, it is also one of 35 double beta decay candidates in which the single $\beta$-decay is forbidden or strongly suppressed. 181 mg of thorium contained in a gas mantle was measured in an HPGe well-detector at the Gran Sasso Underground Laboratory (LNGS) with a total exposure of 3.25 g $\times$ d. We obtain half-life limits on all double beta decay modes of $^{232}$Th to excited states of $^{232}$U on the order of $10^{11-15}$ yr. For the most likely transition into the $0_1^+$ state we find a lower half-life limit of $6.3 \times 10^{14}$ yr (90% credibility). These are the first constraints on double beta decay excited state transition in $^{232}$Th

An innovative technique for the investigation of the 4-fold forbidden beta-decay of 50^{50}V

For the first time a Vanadium-based crystal was operated as cryogenic particle detector. The scintillating low temperature calorimetric technique was used for the characterization of a 22 g YVO$_4$ crystal aiming at the investigation of the 4-fold forbidden non-unique $\beta^-$ decay of $^{50}$V. The excellent bolometric performance of the compound together with high light output of the crystal makes it an outstanding technique for the study of such elusive rate process. The internal radioactive contaminations of the crystal are also investigated showing that an improvement on the current status of material selection and purification are needed, $^{235/238}$U and $^{232}$Th are measured at the level of 28 mBq/kg, 1.3 Bq/kg and 28 mBq/kg, respectively. In this work, we also discuss a future upgrade of the experimental set-up which may pave the road for the detection of the rare $^{50}$V $\beta^-$ decay

Highly Sensitive Gamma-Spectrometers of GERDA for Material Screening: Part 2

The previous article about material screening for GERDA points out the importance of strict material screening and selection for radioimpurities as a key to meet the aspired background levels of the GERDA experiment. This is directly done using low-level gamma-spectroscopy. In order to provide sufficient selective power in the mBq/kg range and below, the employed gamma-spectrometers themselves have to meet strict material requirements, and make use of an elaborate shielding system. This article gives an account of the setup of two such spectrometers. Corrado is located in a depth of 15 m w.e. at the MPI-K in Heidelberg (Germany), GeMPI III is situated at the Gran-Sasso underground laboratory at 3500 m w.e. (Italy). The latter one aims at detecting sample activities of the order ~0.01 mBq/kg, which is the current state-of-the-art level. The applied techniques to meet the respective needs are discussed and demonstrated by experimental results.Comment: Featured in: Proceedings of the XIV International Baksan School "Particles and Cosmology" Baksan Valley, Kabardino-Balkaria, Russia, April 16-21,2007. INR RAS, Moscow 2008. ISBN 978-5-94274-055-9, pp. 233-238; (6 pages, 4 figures

A new investigation of half-lives for the decay modes of 50^{50}V

A new search for the decay modes of the 4-fold forbidden non-unique decay of $^{50}$V has been performed at the Gran Sasso Underground Laboratory (LNGS). In total an exposure of 197 kg $\times$ d has been accumulated. The half-life for the electron capture into the first excited state of $^{50}$Ti has been measured with the highest precision to date as $2.67_{-0.18}^{+0.16} \times 10^{17}$ yr (68% C.I.) in which systematics uncertainties dominate. The search for the $\beta$-decay into the first excited state of $^{50}$Cr resulted in a lower limit of ${1.9} \times 10^{19}$ yr (90% C.I.), which is an improvement of almost one order of magnitude compared to existing results. The sensitivity of the new measurement is now in the region of theoretical predictions