21 research outputs found

    Suppression of both superconductivity and structural transition in hole-doped MoTe2_2 induced by Ta substitution

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    Type-II Weyl semimetal MoTe2_2 exhibits a first-order structural transition at TsT_s ∼\sim250~K and superconducts at TcT_c ∼\sim0.1~K at ambient pressure. Both TsT_s and TcT_c can be manipulated by several tuning parameters, such as hydrostatic pressure and chemical substitution. It is often reported that suppressing TsT_s enhances TcT_c, but our study shows a different behaviour when MoTe2_2 is hole-doped by Ta. When TsT_s is suppressed by Ta doping, TcT_c is also suppressed. Our findings suggest that the suppression of TsT_s does not necessarily enhance superconductivity in MoTe2_2. By connecting with the findings of electron-doped MoTe2_2, we argue that varying electron carrier concentration can effectively tune TcT_c. In addition, the Hall coefficient is enhanced around the doping region, where TsT_s is completely suppressed, suggesting that the critical scattering around the structural transition may also play a role in suppressing TcT_c

    Peak in the critical current density in (Cax_{x}Sr1βˆ’x_{1-x})3_3Rh4_4Sn13_{13} tuned towards the structural quantum critical point

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    (Cax_{x}Sr1βˆ’x_{1-x})3_3Rh4_4Sn13_{13} is a rare system that has been shown to display an interesting interplay between structural quantum criticality and superconductivity. A putative structural quantum critical point, which is hidden beneath a broad superconducting dome, is believed to give rise to optimized superconducting properties in (Cax_{x}Sr1βˆ’x_{1-x})3_3Rh4_4Sn13_{13}. However, the presence of the superconducting dome itself hinders the examination of the quantum critical point through electrical transport, as the transport coefficients vanish in the superconducting state. Here, we use critical current density to explore within the superconducting dome. Our measurements reveal a large enhancement of the critical current density at the zero-temperature limit when the system is tuned towards the structural quantum critical point.Comment: 7 pages, 4 figure

    Tunable non-Lifshitz-Kosevich temperature dependence of Shubnikov-de Haas oscillation amplitudes in SmSb

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    The Lifshitz-Kosevich (LK) theory is the pillar of magnetic quantum oscillations, which have been extensively applied to characterize a wide range of metallic states. In this study, we focus on the Shubnikov-de Haas (SdH) effect observed in SmSb, a rare-earth monopnictide. We observed a significant departure from the expected LK theory near TN=2.4T_N=2.4~K: both a peak-like anomaly and an enhancement in the temperature dependence of quantum oscillation amplitude are seen in SmSb. Moreover, we discovered a remarkable sensitivity of the SdH amplitudes to sample purity. By adjusting the sample purity, we were able to tune the temperature dependence of the Ξ±\alpha band's SdH amplitudes from a peak-like anomalous behavior to an enhancement. Therefore, SdH oscillations from the Ξ±\alpha band connect the two well-known non-LK behaviours, controllable through varying the sample purity, paving the way for developing further understanding of the mechanism leading to the anomalous quantum oscillations.Comment: 4 figure

    Similarities and Differences in the Fermiology of Kagome Metals AV3_{3}Sb5_{5} (A=K, Rb, Cs) Revealed by Shubnikov-de Haas Oscillations

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    Materials with AV3_3Sb5_5 (A=K, Rb, Cs) stoichiometry are recently discovered kagome superconductors with the electronic structure featuring a Dirac band, van Hove singularities and flat bands. These systems undergo anomalous charge-density-wave (CDW) transitions at TCDWT_{\rm CDW}~80-100 K, resulting in the reconstruction of the Fermi surface from the pristine phase. Although comprehensive investigations of the electronic structure via quantum oscillations (QOs) have been performed on the sister compounds CsV3_3Sb5_5 and RbV3_3Sb5_5, a detailed QO study of KV3_3Sb5_5 is so far absent. Here, we report the Shubnikov-de Haas QO study in KV3_3Sb5_5. We resolve a large number of new frequencies with the highest frequency of 2202 T (occupying ~54% of the Brillouin zone area in the kxk_x-kyk_y plane). The Lifshitz-Kosevich analysis further gives relatively small cyclotron effective masses, and the angular dependence study reveals the two-dimensional nature of the frequencies with a sufficient signal-to-noise ratio. Finally, we compare the QO spectra for all three AV3_3Sb5_5 compounds collected under the same conditions, enabling us to point out the similarities and differences across these systems. Our results fill in the gap of the QO study in KV3_3Sb5_5 and provide valuable data to understand the band structure of all three members of AV3_3Sb5_5.Comment: 8 pages, 4 figure

    Nodeless superconductivity in kagome metal CsV3_{3}Sb5_{5} with and without time reversal symmetry breaking

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    The kagome metal CsV3_{3}Sb5_{5} features an unusual competition between the charge-density-wave (CDW) order and superconductivity. Evidence for time-reversal symmetry breaking (TRSB) inside the CDW phase has been accumulating. Hence, the superconductivity in CsV3_{3}Sb5_{5} emerges from a TRSB normal state, potentially resulting in an exotic superconducting state. To reveal the pairing symmetry, we first investigate the effect of nonmagnetic impurity. Our results show that the superconducting critical temperature is insensitive to disorder, pointing to conventional ss-wave superconductivity. Moreover, our measurements of the self-field critical current (Ic,sfI_{c,sf}), which is related to the London penetration depth, also confirm conventional ss-wave superconductivity with strong coupling. Finally, we measure Ic,sfI_{c,sf} where the CDW order is removed by pressure and superconductivity emerges from the pristine normal state. Our results show that ss-wave gap symmetry is retained, providing strong evidence for the presence of conventional ss-wave superconductivity in CsV3_{3}Sb5_{5} irrespective of the presence of the TRSBComment: 8 pages, 4 figures. Nano Letters (in press
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