194 research outputs found
Experimental evidence for exciton scaling effects in self-assembled molecular wires
Journal ArticleResonant Rayleigh scattering from self-assembled one-dimensional molecular J-aggregate wires reveals a distinct dependence of the exciton energy on the width of lateral extension. For the J aggregates used in this study, strong in-line dipole coupling leads to a delocalization of the exciton wave function over several molecular units. Polarization dependent measurements of resonantly scattered light from the wires show that the exciton dipole moment is oriented perpendicular to the long axis. The experimental observations can be described by applying a quantization condition to the center of mass motion of the J-band exciton in the wires
Penrose-Onsager Criterion Validation in a One-Dimensional Polariton Condensate
We perform quantum tomography on one-dimensional polariton condensates,
spontaneously occurring in linear disorder valleys in a CdTe planar microcavity
sample. By the use of optical interferometric techniques, we determine the
first-order coherence function and the amplitude and phase of the order
parameter of the condensate, providing a full reconstruction of the single
particle density matrix for the polariton system. The experimental data are
used as input to theoretically test the consistency of Penrose-Onsager
criterion for Bose-Einstein condensation in the framework of nonequilibrium
polariton condensates. The results confirm the pertinence and validity of the
criterion for a non equilibrium condensed gas.Comment: 5 pages, 4 figure
Single-mode tuneable laser operation of hybrid microcavities based on CdSe/CdS core/shell colloidal nanorods on silica microspheres
Colloidal core/shell semiconductor nanonorystals have generated a great deal of interest as gain media in recent years due to a number of salient properties originating from their small size and the associated quantum confinement [1]. These include low-threshold and temperature-insensitive lasing, reduced trapping of excited carriers, and the possibility to alleviate non-radiative Auger recombination by engineering the wavefunction distributions of the electrons, and holes within their volume. Here, single-mode, tuneable operation of fiber-coupled hybrid lasers based on colloidal CdSe/CdS core/shell nanorods on silica microspheres is reported
Ultimate photo-induced Kerr rotation achieved in semiconductor microcavities
Photoinduced Kerr rotation by more than radians is demonstrated in
planar quantum well microcavity in the strong coupling regime. This result is
close to the predicted theoretical maximum of . It is achieved by
engineering microcavity parameters such that the optical impedance matching
condition is reached at the smallest negative detuning between exciton
resonance and the cavity mode. This ensures the optimum combination of the
exciton induced optical non-linearity and the enhancement of the Kerr angle by
the cavity. Comprehensive analysis of the polarization state of the light in
this regime shows that both renormalization of the exciton energy and the
saturation of the excitonic resonance contribute to the observed optical
nonlinearities.Comment: Shortened version prepared to submit in Phys. Rev. Letter
Spin noise spectroscopy of a single-quantum-well microcavity
We report on the first experimental observation of spin noise in a single
semiconductor quantum well embedded into a microcavity. The great
cavity-enhanced sensitivity to fluctuations of optical anisotropy has allowed
us to measure the Kerr rotation and ellipticity noise spectra in the strong
coupling regime. The spin noise spectra clearly show two resonant features: a
conventional magneto-resonant component shifting towards higher frequencies
with magnetic field and an unusual "nonmagnetic" component centered at zero
frequency and getting suppressed with increasing magnetic field. We attribute
the first of them to the Larmor precession of free electron spins, while the
second one being presumably due to hyperfine electron-nuclei spin interactions.Comment: 5 pages, 6 figures + supplement (4 pages, 1 figure
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