Exploring, tailoring, and traversing the solution landscape of a phase-shaped CARS process

Pulse shaping techniques are used to improve the selectivity of broadband CARS experiments, and to reject the overwhelming background. Knowledge about the fitness landscape and the capability of tailoring it is crucial for both fundamental insight and performing an efficient optimization of phase shapes. We use an evolutionary algorithm to find the optimal spectral phase of the broadband pump and probe beams in a background-suppressed shaped CARS process. We then investigate the shapes, symmetries, and topologies of the landscape contour lines around the optimal solution and also around the point corresponding to zero phase. We demonstrate the significance of the employed phase bases in achieving convex contour lines, suppressed local optima, and high optimization fitness with a few (and even a single) optimization parameter

Implementation of vibrational phase contrast coherent anti-Stokes Raman scattering microscopy

Detection of molecules using vibrational resonances in the fingerprint region for narrowband coherent anti-Stokes Raman scattering (CARS) is challenging. The spectrum is highly congested resulting in a large background and a reduced specificity. Recently we introduced vibrational phase contrast CARS (VPC-CARS) microscopy as a technique capable of detecting both the amplitude and phase of the CARS signal, providing background-free images and high specificity. In this paper we present a new implementation of VPC-CARS based on a third-order cascaded phase-preserving chain, where the CARS signal is generated at a single (constant) wavelength independent of the vibrational frequency that is addressed. This implementation will simplify the detection side considerably

Sub-wavelength scale characterization of on-chip coupling mirrors

Miniature free-space optical beams, originating from on-chip microstructures, are usually measured and quoted without reference to a particular polarization state. We develop an automated platform to characterize tightly focused free-space optical beams in three dimensions. We present a detailed description of each subsystem including the calibration and test procedure. We demonstrate how amplitude and phase are measured at sub-wavelength resolution using a cleaved fiber with a heterodyne reference. Further analysis provides information about the phase and intensity profile of the beam with regards to its polarization content and spatial confinement. We perform a proof-of-concept experiment for a custom waveguide-coupled micro-mirror. The work opens new possibilities for rapid analysis of micro-mirrors in prototyping and optimization of integrated optical systems.</p

A route to sub-diffraction-limited CARS Microscopy

We theoretically investigate a scheme to obtain sub-diffraction-limited resolution in coherent anti-Stokes Raman scattering (CARS) microscopy. We find using density matrix calculations that the rise of vibrational (Raman) coherence can be strongly suppressed, and thereby the emission of CARS signals can be significantly reduced, when pre-populating the corresponding vibrational state through an incoherent process. The effectiveness of pre-populating the vibrational state of interest is investigated by considering the excitation of a neighbouring vibrational (control) state through an intense, mid-infrared control laser. We observe that, similar to the processes employed in stimulated emission depletion microscopy, the CARS signal exhibits saturation behaviour if the transition rate between the vibrational and the control state is large. Our approach opens up the possibility of achieving chemically selectivity sub-diffraction-limited spatially resolved imaging

Hyperspectral imaging in biomedical applications

No abstract available

Polarization-resolved near-field characterization of coupling between a bus waveguide and a ring resonator

Light propagation in Photonic integrated circuits (PICs), which can nowadays involve complex systems of light-guiding structures, is measured with different approaches(Nuzhdin et al., 2020, Lončar et al., 2002, Hopman et al., 2007, Morichetti et al., 2014, Sapienza et al., 2012, Vesseur et al., 2007). An interferometric polarization-sensitive measurement of the evanescent fields of these structures provides insight in the performance of the circuit detects possible malfunction with sub-wavelength precision(Engelen et al., 2007, Gersen et al., 2005, Barwick et al., 2009). We demonstrate a Near-field scanning optical microscopy (NSOM) measurement on coupled ring resonators that shows how the guided modes evolve as they propagate across the optical chip. Analysis of the measurements provides information about intensity distribution of the two polarization components (TE and TM) and their spatial confinement. The data validates our methodology and opens new possibilities for analysis of signal propagation in prototyping and optimization of integrated optical systems. Direct observation of polarization state of the guided modes allows for clear understanding of mode conversion in coupling systems.</p

Large bandwidth, highly efficient optical gratings through high index materials

We analyze the diffraction characteristics of dielectric gratings that feature a high index grating layer, and devise, through rigorous numerical calculations, large bandwidth, highly efficient, high dispersion dielectric gratings in reflection, transmission, and immersed transmission geometry. A dielectric TIR grating is suggested, whose -1dB spectral bandwidth is doubled as compared to its all-glass equivalent. The short wavelength diffraction efficiency is additionally improved by allowing for slanted lamella. The grating surpasses a blazed gold grating over the full octave. An immersed transmission grating is devised, whose -1dB bandwidth is tripled as compared to its all-glass equivalent, and that surpasses an equivalent classical transmission grating over nearly the full octave. A transmission grating in the classical scattering geometry is suggested, that features a buried high index layer. This grating provides effectively 100% diffraction efficiency at its design wavelegth, and surpasses an equivalent fused silica grating over the full octave.Comment: 15 pages, 7 figure