Origin of the inner ring in photoluminescence patterns of quantum well excitons

In order to explain and model the inner ring in photoluminescence (PL) patterns of indirect excitons in GaAs/AlGaAs quantum wells (QWs), we develop a microscopic approach formulated in terms of coupled nonlinear equations for the diffusion, thermalization and optical decay of the particles. The origin of the inner ring is unambiguously identified: it is due to cooling of indirect excitons in their propagation from the excitation spot. We infer that in our high-quality structures the in-plane diffusion coefficient is about 10-30cm^2/s and the amplitude of the disorder potential is about 0.45meV.Comment: 4 pages, 3 figure

Pattern Formation as a Signature of Quantum Degeneracy in a Cold Exciton System

The development of a Turing instability to a spatially modulated state in a photoexcited electron-hole system is proposed as a novel signature of exciton Bose statistics. We show that such an instability, which is driven by kinetics of exciton formation, can result from stimulated processes that build up near quantum degeneracy. In the spatially uniform 2d electron-hole system, the instability leads to a triangular lattice pattern while, at an electron-hole interface, a periodic 1d pattern develops. We analyze the mechanism of wavelength selection, and show that the transition is abrupt (type I) for the uniform 2d system, and continuous (type II) for the electron-hole interface.Comment: 5 pages, 3 figure

Theory of condensation of indirect excitons in a trap

We present theoretical studies of condensation of indirect excitons in a trap. Our model quantifies the effect of screening of the trap potential by indirect excitons on exciton condensation. The theoretical studies are applied to a system of indirect excitons in a GaAs/AlGaAs coupled quantum well structure in a diamond-shaped electrostatic trap where exciton condensation was studied in earlier experiments. The estimated condensation temperature of the indirect excitons in the trap reaches hundreds of milliKelvin

Kinetics of Exciton Emission Patterns and Carrier Transport

We report on the measurements of the kinetics of expanding and collapsing rings in the exciton emission pattern. The rings are found to preserve their integrity during expansion and collapse, indicating that the observed kinetics is controlled by charge carrier transport rather than by a much faster process of exciton production and decay. The relation between ring kinetics and carrier transport, revealed by our experiment and confirmed by comparison with a theoretical model, is used to determine electron and hole transport characteristics in a contactless fashion.Comment: 6 pages, 4 figure

The Interaction in the Macroscopically Ordered Exciton State

The macroscopically ordered exciton state (MOES) - a periodic array of beads with spatial order on a macroscopic length - appears in the external exciton rings at low temperatures below a few Kelvin. Here, we report on the experimental study of the interaction in the MOES. The exciton PL energy varies in concert with the intensity along the circumference of the ring, with the largest energy found in the brightest regions. This shows that the MOES is characterized by the repulsive interaction and is not driven by the attractive interaction.Comment: 3 pages, 3 figure

Kinetics of the inner ring in the exciton emission pattern in GaAs coupled quantum wells

We report on the kinetics of the inner ring in the exciton emission pattern. The formation time of the inner ring following the onset of the laser excitation is found to be about 30 ns. The inner ring was also found to disappear within 4 ns after the laser termination. The latter process is accompanied by a jump in the photoluminescence (PL) intensity. The spatial dependence of the PL-jump indicates that the excitons outside of the region of laser excitation, including the inner ring region, are efficiently cooled to the lattice temperature even during the laser excitation. The ring formation and disappearance are explained in terms of exciton transport and cooling.Comment: 19 pages, 6 figure

Photoluminescence and spectral switching of single CdSe/ZnS colloidal nanocrystals in poly(methyl methacrylate)

Emission from single CdSe nanocrystals in PMMA was investigated. A fraction of the nanocrystals exhibiting switching between two energy states, which have similar total intensities, but distinctly different spectra were observed. We found that the spectral shift characteristic frequency increases with the pump power. By using the dynamic shift in the spectral position of emission peaks, we were able to correlate peaks from the same nanocrystal. The measured correlation is consistent with assignment of low energy lines to phonon replicas.Comment: 5 pages, 4 figure