High-harmonic generation from arbitrarily oriented diatomic molecules including nuclear motion and field-free alignment

We present a theoretical model of high-harmonic generation from diatomic molecules. The theory includes effects of alignment as well as nuclear motion and is used to predict results for N$_2$, O$_2$, H$_2$ and D$_2$. The results show that the alignment dependence of high-harmonics is governed by the symmetry of the highest occupied molecular orbital and that the inclusion of the nuclear motion in the theoretical description generally reduces the intensity of the harmonic radiation. We compare our model with experimental results on N$_2$ and O$_2$, and obtain very good agreement.Comment: 12 pages, 8 figures, 2 tables; legends revised on Figs. 1,3,4,6 and

Observation of force-detected nuclear magnetic resonance in a homogeneous field

We report the experimental realization of BOOMERANG (better observation of magnetization, enhanced resolution, and no gradient), a sensitive and general method of magnetic resonance. The prototype millimeter-scale NMR spectrometer shows signal and noise levels in agreement with the design principles. We present H-1 and F-19 NMR in both solid and liquid samples, including time-domain Fourier transform NMR spectroscopy, multiple-pulse echoes, and heteronuclear J spectroscopy. By measuring a H-1-F-19 J coupling, this last experiment accomplishes chemically specific spectroscopy with force-detected NMR. In BOOMERANG, an assembly of permanent magnets provides a homogeneous field throughout the sample, while a harmonically suspended part of the assembly, a detector, is mechanically driven by spin-dependent forces. By placing the sample in a homogeneous field, signal dephasing by diffusion in a field gradient is made negligible, enabling application to liquids, in contrast to other force-detection methods. The design appears readily scalable to µm-scale samples where it should have sensitivity advantages over inductive detection with microcoils and where it holds great promise for application of magnetic resonance in biology, chemistry, physics, and surface science. We briefly discuss extensions of the BOOMERANG method to the µm and nm scales

High-order harmonic generation from polyatomic molecules including nuclear motion and a nuclear modes analysis

We present a generic approach for treating the effect of nuclear motion in the high-order harmonic generation from polyatomic molecules. Our procedure relies on a separation of nuclear and electron dynamics where we account for the electronic part using the Lewenstein model and nuclear motion enters as a nuclear correlation function. We express the nuclear correlation function in terms of Franck-Condon factors which allows us to decompose nuclear motion into modes and identify the modes that are dominant in the high-order harmonic generation process. We show results for the isotopes CH$_4$ and CD$_4$ and thereby provide direct theoretical support for a recent experiment [Baker {\it et al.}, Science {\bf 312}, 424 (2006)] that uses high-order harmonic generation to probe the ultra-fast structural nuclear rearrangement of ionized methane.Comment: 6 pages, 6 figure

Classification of String-like Solutions in Dilaton Gravity

The static string-like solutions of the Abelian Higgs model coupled to dilaton gravity are analyzed and compared to the non-dilatonic case. Except for a special coupling between the Higgs Lagrangian and the dilaton, the solutions are flux tubes that generate a non-asymptotically flat geometry. Any point in parameter space corresponds to two branches of solutions with two different asymptotic behaviors. Unlike the non-dilatonic case, where one branch is always asymptotically conic, in the present case the asymptotic behavior changes continuously along each branch.Comment: 15 pages, 6 figures. To be published in Phys. Rev.

Angular Normal Modes of a Circular Coulomb Cluster

We investigate the angular normal modes for small oscillations about an equilibrium of a single-component coulomb cluster confined by a radially symmetric external potential to a circle. The dynamical matrix for this system is a Laplacian symmetrically circulant matrix and this result leads to an analytic solution for the eigenfrequencies of the angular normal modes. We also show the limiting dependence of the largest eigenfrequency for large numbers of particles

Experimental Bell Inequality Violation with an Atom and a Photon

We report the measurement of a Bell inequality violation with a single atom and a single photon prepared in a probabilistic entangled state. This is the first demonstration of such a violation with particles of different species. The entanglement characterization of this hybrid system may also be useful in quantum information applications.Comment: 4 pages, 2 figure