Neel order in the two-dimensional S=1/2 Heisenberg Model

The existence of Neel order in the S=1/2 Heisenberg model on the square lattice at T=0 is shown using inequalities set up by Kennedy, Lieb and Shastry in combination with high precision Quantum Monte Carlo data.Comment: 4 pages, 1 figur

Finite size effects and magnetic order in the spin-1/2 honeycomb lattice compound InCu{2/3}V{1/3}O{3}

High field electron spin resonance, nuclear magnetic resonance and magnetization studies addressing the ground state of the quasi two-dimensional spin-1/2 honeycomb lattice compound InCu{2/3}V{1/3}O{3} are reported. Uncorrelated finite size structural domains occurring in the honeycomb planes are expected to inhibit long range magnetic order. Surprisingly, ESR data reveal the development of two collinear antiferromagnetic (AFM) sublattices below ~ 20 K whereas NMR results show the presence of the staggered internal field. Magnetization data evidence a spin reorientation transition at ~ 5.7 T. Quantum Monte-Carlo calculations show that switching on the coupling between the honeycomb spin planes in a finite size cluster yields a Neel-like AFM spin structure with a substantial staggered magnetization at finite temperatures. This may explain the occurrence of a robust AFM state in InCu{2/3}V{1/3}O{3} despite an unfavorable effect of structural disorder.Comment: revised version, accepted as a Rapid Communication in Phys. Rev. B (2010

Room temperature Rydberg Single Photon Source

We present an optimal protocol to implement a room temperature Rydberg single photon source within an experimental setup based on micro cells filled with thermal vapor. The optimization of a pulsed four wave mixing scheme allows to double the effective Rydberg blockade radius as compared to a simple Gaussian pulse scheme, releasing some of the constrains on the geometry of the micro cells. The performance of the optimized protocol is improved by about 70% with respect to the standard protocol.Comment: 5 pages, 6 figure

Gapped Heisenberg spin chains in a field

We consider the fully anisotropic Heisenberg spin-1/2 antiferromagnet in a uniform magnetic field, whose ground-state is characterized by broken spin rotation symmetry and gapped spinon excitations. We expand on a recent mean-field approach to the problem by incorporating fluctuations in a loop expansion. Quantitative results for the magnetization, excitation gap and specific heat are obtained. We compare our predictions with new DMRG and exact diagonalization data and, for zero field, with the exact solution of the ${XYZ}$ spin chain from the Bethe Ansatz.Comment: 11 pages, 14 figure

The interfacial structure of InP(100) in contact with HCl and H2SO4 studied by reflection anisotropy spectroscopy

Indium phosphide and derived compound semiconductors are materials often involved in high-efficiency solar water splitting due to their versatile opto-electronic properties. Surface corrosion, however, typically deteriorates the performance of photoelectrochemical solar cells based on this material class. It has been reported that (photo)electrochemical surface functionalisation protects the surface by combining etching and controlled corrosion. Nevertheless, the overall involved process is not fully understood. Therefore, access to the electrochemical interface structure under operando conditions is crucial for a more detailed understanding. One approach for gaining structural insight is the use of operando reflection anisotropy spectroscopy. This technique allows the time-resolved investigation of the interfacial structure while applying potentials in the electrolyte. In this study, p-doped InP(100) surfaces are cycled between anodic and cathodic potentials in two different electrolytes, hydrochloric acid and sulphuric acid. For low, 10 mM electrolyte concentrations, we observe a reversible processes related to the reduction of a surface oxide phase in the cathodic potential range which is reformed near open-circuit potentials. Higher concentrations of 0.5 N, however, already lead to initial surface corrosion.Comment: 10 pages, 6 figure