Local lattice disorder in the geometrically-frustrated spin glass pyrochlore Y2Mo2O7

The geometrically-frustrated spin glass Y2Mo2O7 has been considered widely to be crystallographically ordered with a unique nearest neighbor magnetic exchange interaction, J. To test this assertion, we present x-ray-absorption fine-structure results for the Mo and Y K edges as a function of temperature and compare them to results from a well-ordered pyrochlore, Tl2Mn2O7. We find that the Mo-Mo pair distances are significantly disordered at approximately right angles to the Y-Mo pairs. These results strongly suggest that lattice disorder nucleates the spin-glass phase in this material.Comment: 9 pages, 2 Postscript figures, Phys. Rev. B: Rapid, in pres

Pd/Cu Site Interchange and Non-Fermi-Liquid Behavior in UCu_4Pd

X-ray-absorption fine-structure measurements of the local structure in UCu_4Pd are described which indicate a probable lattice-disorder origin for non-Fermi-liquid behavior in this material. Short Pd-Cu distances are observed, consistent with 24 +/- 3% of the Pd atoms occupying nominally Cu sites. A "Kondo disorder" model, based on the effect on the local Kondo temperature T_K of this interchange and some additional bond-length disorder, agrees quantitatively with previous experimental susceptibility data, and therefore also with specific heat and magnetic resonance experiments.Comment: 4 pages, 3 PostScript figures, to be published in PR

Prospects for Direct CP Violaton in Exclusive and Inclusive Charmless B decays

Within the Standard Model, CP rate asymmetries for $B\to K^-\pi^{+,0}$ could reach 10%. With strong final state phases, they could go up to 20--30%, even for $\bar K^0\pi^-$ mode which would have opposite sign. We can account for $K^-\pi^{+}$, $\bar K^0\pi^-$ and $\phi K$ rate data with new physics enhanced color dipole coupling and destructive interference. Asymmetries could reach 40--60% for $K\pi$ and $\phi K$ modes and are all of the same sign. We are unable to account for $K^-\pi^0$ rate. Our inclusive study supports our exclusive results.Comment: Minor changes, correct a small bug in Fig. 1(b). Version to appear in Phys. Rev. Let

Analysis of B-> \phi K Decays in QCD Factorization

We analyze the decay $B\to \phi K$ within the framework of QCD-improved factorization. We found that although the twist-3 kaon distribution amplitude dominates the spectator interactions, it will suppress the decay rates slightly. The weak annihilation diagrams induced by $(S-P)(S+P)$ penguin operators, which are formally power-suppressed by order $(\Lambda/m_b)^2$, are chirally and logarithmically enhanced. Therefore, these annihilation contributions are not subject to helicity suppression and can be sizable. The predicted branching ratio of $B^-\to\phi K^-$ is $(3.8\pm0.6)\times 10^{-6}$ in the absence of annihilation contributions and it becomes $(4.3^{+3.0}_{-1.4})\times 10^{-6}$ when annihilation effects are taken into account. The prediction is consistent with CLEO and BaBar data but smaller than the BELLE result.Comment: 13 pages, 3 figures. A major change for the presentation of branching-ratio predictions. Experimental data are update

Local structural origins of the distinct electronic properties of Nb-substituted SrTiO3_3 and BaTiO3O_3

Near or less than 10% Nb substitution on the Ti site in perovskite SrTiO$_3$ results in metallic behavior, in contrast to what is seen in BaTiO$_3$. Given the nearly identical structure and electron counts of the two materials, the distinct ground states for low substitution have been a long-standing puzzle. Here we find from neutron studies of average and local structure, the subtle yet critical difference that we believe underpins the distinct electronic properties in these fascinating materials. While SrTi$_{0.875}$Nb_${0.125}$O$_3$ possesses a distorted non-cubic structure at 15 K, the BO$_6$ octahedra in the structure are regular. BaTi$_{0.875}$Nb$_{0.125}$O$_3$ on the other hand shows evidence for local cation off-centering whilst retaining a cubic structure.Comment: 4 pages, 5 figure

Possible charge inhomogeneities in the CuO2 planes of YBa2Cu3O6+x (x=0.25, 0.45, 0.65, 0.94) from pulsed neutron diffraction

The atomic pair distribution functions (PDF) of four powder samples of YBa2Cu3O6+x (x=0.25, 0.45, 0.65, 0.94) at 15 K have been measured by means of pulsed neutron diffraction. The PDF is modelled using a full-profile fitting approach to yield structural parameters. In contrast to earlier XAFS work we find no evidence of a split apical oxygen site. However, a slightly improved fit over the average crystallographic model results when the planar Cu(2) site is split along the z-direction. This is interpreted in terms of charge inhomogeneities in the CuO2 planes.Comment: 8 pages, 3 figure

Spin Dynamics of the Magnetoresistive Pyrochlore Tl_2Mn_2O_7

Neutron scattering has been used to study the magnetic order and spin dynamics of the colossal magnetoresistive pyrochlore Tl_2Mn_2O_7. On cooling from the paramagnetic state, magnetic correlations develop and appear to diverge at T_C (123 K). In the ferromagnetic phase well defined spin waves are observed, with a gapless ($\Delta <0.04$ meV) dispersion relation E=Dq^{2} as expected for an ideal isotropic ferromagnet. As T approaches T_C from low T, the spin waves renormalize, but no significant central diffusive component to the fluctuation spectrum is observed in stark contrast to the La$_{1-x}$(Ca,Ba,Sr)$_x$MnO$_3$ system. These results argue strongly that the mechanism responsible for the magnetoresistive effect has a different origin in these two classes of materials.Comment: 4 pages (RevTex), 4 figures (encapsulated postscript), to be published in Phys. Rev. Let