169 research outputs found
The Yellow Excitonic Series of Cu2O Revisited by Lyman Spectroscopy
We report on the observation of the yellow exciton Lyman series up to the
fourth term in Cu2O by time-resolved mid-infrared spectroscopy. The dependence
of the oscillator strength on the principal quantum number n can be well
reproduced using the hydrogenic model including an AC dielectric constant, and
precise information on the electronic structure of the 1s exciton state can be
obtained. A Bohr radius a_{1s}=7.9 A and a 1s-2p transition dipole moment
\mu_{1s-2p}= 4.2 eA were found
Study of ortho-to-paraexciton conversion in CuO by excitonic Lyman spectroscopy
Using time-resolved - excitonic Lyman spectroscopy, we study the
orthoexciton-to-paraexcitons transfer, following the creation of a high density
population of ultracold orthoexcitons by resonant two-photon excitation
with femtosecond pulses.
An observed fast exciton-density dependent conversion rate is attributed to
spin exchange between pairs of orthoexcitons.
Implication of these results on the feasibility of BEC of paraexcitons in
CuO is discussed
Formation and decay of electron-hole droplets in diamond
We study the formation and decay of electron-hole droplets in diamonds at
both low and high temperatures under different excitations by master equations.
The calculation reveals that at low temperature the kinetics of the system
behaves as in direct-gap semiconductors, whereas at high temperature it shows
metastability as in traditional indirect-gap semiconductors. Our results at low
temperature are consistent with the experimental findings by Nagai {\em et al.}
[Phys. Rev. B {\bf 68}, 081202 (R) (2003)]. The kinetics of the e-h system in
diamonds at high temperature under both low and high excitations is also
predicted.Comment: 7 pages, 8 figures, revised with some modifications in physics
discussion, to be published in PR
Signatures of the excitonic memory effects in four-wave mixing processes in cavity polaritons
We report the signatures of the exciton correlation effects with finite
memory time in frequency domain degenerate four-wave mixing (DFWM) in
semiconductor microcavity. By utilizing the polarization selection rules, we
discriminate instantaneous, mean field interactions between excitons with the
same spins, long-living correlation due to the formation of biexciton state by
excitons with opposite spins, and short-memory correlation effects in the
continuum of unbound two-exciton states. The DFWM spectra give us the relative
contributions of these effects and the upper limit for the time of the
exciton-exciton correlation in the unbound two-exciton continuum. The obtained
results reveal the basis of the cavity polariton scattering model for the DFWM
processes in high-Q GaAs microcavity.Comment: 11 pages, 1 figur
Quasi-degenerate self-trapping in one-dimensional charge transfer exciton
The self-trapping by the nondiagonal particle-phonon interaction between two
quasi-degenerate energy levels of excitonic system, is studied. We propose this
is realized in charge transfer exciton, where the directions of the
polarization give the quasi-degeneracy. It is shown that this mechanism, unlike
the conventional diagonal one, allows a coexistence and resonance of the free
and self-trapped states even in one-dimensional systems and a quantitative
theory for the optical properties (light absorption and time-resolved
luminescence) of the resonating states is presented. This theory gives a
consistent resolution for the long-standing puzzles in quasi-one-dimensional
compound A-PMDA.Comment: accepted to Phys. Rev. Letter
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