333 research outputs found
Lattice-form dependent orbital shape and charge disproportionation in charge- and orbital-ordered manganites
The orbital shapes and charge disproportionations at nominal Mn and
Mn sites for the charge- and orbital-ordered phases have been studied on
half-doped manganites Pr(SrCa)MnO and
EuCaMnO with double-layer and single-layer Mn-O networks,
respectively, by means of x-ray structural analyses, in comparison with
PrCaMnO with the pseudo cubic network. In a single-layer
EuCaMnO system, the ()/()-type orbital
shape is observed, while the ()/()-type orbital shape in a
pseudo cubic PrCaMnO system. In a double-layer
Pr(SrCa)MnO system, the orbital shape is found to
undergo a large change upon thermally induced rotation of orbital stripe.
Furthermore, clear charge disproportionation is observed for the pseudo cubic
and double-layer systems, while not in the single-layer system. These results
indicate that the orbital shape and charge disproportionation are sensitive to
the dimension of Mn-O network.Comment: 12 page, 5 figures, 11 table
Fe-doping-induced evolution of charge-orbital ordering in a bicritical-state manganite
Impurity effects on the stability of a ferromagnetic metallic state in a
bicritical-state manganite, (La0.7Pr0.3)0.65Ca0.35MnO3, on the verge of
metal-insulator transition have been investigated by substituting a variety of
transition-metal atoms for Mn ones. Among them, Fe doping exhibits the
exceptional ability to dramatically decrease the ferromagnetic transition
temperature. Systematic studies on the magnetotransport properties and x-ray
diffraction for the Fe-doped crystals have revealed that charge-orbital
ordering evolves down to low temperatures, which strongly suppresses the
ferromagnetic metallic state. The observed glassy magnetic and transport
properties as well as diffuse phase transition can be attributed to the
phase-separated state where short-range charge-orbital-ordered clusters are
embedded in the ferromagnetic metallic matrix. Such a behavior in the Fe-doped
manganites form a marked contrast to the Cr-doping effects on
charge-orbital-ordered manganites known as impurity-induced collapse of
charge-orbital ordering.Comment: 8 pages, 7 figure
Epitaxial-strain effect on charge/orbital order in Pr0.5Ca0.5MnO3 films
Effect of growth orientation on charge- and orbital-ordering (CO-OO)
phenomena has been studied for Pr0.5Ca0.5MnO3 epitaxial thin films fabricated
on (LaAlO3)0.3-(SrAl0.5Ta0.5O3)0.7 (LSAT) substrates by means of resistivity,
synchrotron x-ray diffraction, and polarized optical microscopy measurements.
CO-OO transition is observed around 220 K for a film grown on an LSAT (011)
substrate ((011)-film), similarly to a bulk sample, while a film grown on a
(001) plane of LSAT ((001)-film) shows much higher transition temperature
around 300 K. The domain size of OO is approximately 3 times as large in the
(011)-film as in the (001)-film. These results demonstrate that various
properties of CO-OO phenomena can be controlled with the growth orientation via
the epitaxial strain from the substrate.Comment: 4 pages, 4 figure
Bandwidth-disorder phase diagram of half doped layered manganites
Phase diagrams in the plane of (the average ionic radius, related to
one-electron bandwidth ) and (the ionic radius variance,
measuring the quenched disorder), or ``bandwidth-disorder phase diagrams'',
have been established for perovskite manganites, with three-dimensional (3)
Mn-O network. Here we establish the intrinsic bandwidth-disorder phase diagram
of half-doped layered manganites with the two-dimensional (2) Mn-O network,
examining in detail the ``mother state'' of the colossal magnetoresistance
(CMR) phenomenon in crystals without ferromagnetic instability. The
consequences of the reduced dimensionality, from 3 to 2, on the
order-disorder phenomena in the charge-orbital sectors are also highlighted.Comment: REVTeX 4 style; 5 pages, 4 figure
Pseudogap of metallic layered nickelate R2-xSrxNiO4 (R=Nd, Eu) crystals measured using angle-resolved photoemission spectroscopy
We have investigated charge dynamics and electronic structures for single
crystals of metallic layered nickelates, R2-xSrxNiO4 (R=Nd, Eu), isostructural
to La2-xSrxCuO4. Angle-resolved photoemission spectroscopy on the
barely-metallic Eu0.9Sr1.1NiO4 (R=Eu, x=1.1) has revealed a large hole surface
of x2-y2 character with a high-energy pseudogap of the same symmetry and
comparable magnitude with those of underdoped (x<0.1) cuprates, although the
antiferromagnetic interactions are one order of magnitude smaller. This finding
strongly indicates that the momentum-dependent pseudogap feature in the layered
nickelate arises from the real-space charge correlation.Comment: 4 pages, 4 figures. Accepted in Physical Review Letter
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