9,240 research outputs found
Formation of rectifier with gold nanoclusters
Gold nanoclusters encapsulated with organic molecules are of great interest
for its possible applications in the fields of molecular electronics, catalysis
and medical science. Here we demonstrate that monolayer and bilayer films of
thiol-capped gold nanoclusters can exhibit diode-like properties provided
controlled spatial asymmetry exist between two tunnel junctions used to connect
a thiol capped gold nanoclusters. Current-voltage characteristics of this
rectifier were obtained from conducting probe atomic force microscopy
measurements and also from conventional two probe resistance measurements.
Systematic x-ray reflectivity and atomic force microscopy measurements were
carried out to characterize the spatial asymmetry introduced by a monolayer of
fatty acid salt gadolinium stearate used to deposit thiol-capped gold
nanocluster molecules on hydrophilic SiO2-Si(001) substrate by Langmuir
Blodgett technique. This information was used to explain prominent
rectification observed in these nano-structured films.Comment: 13 pages, 3 figure
Formation rates of Dark Matter Haloes
We derive an estimate of the rate of formation of dark matter halos per unit
volume as a function of the halo mass and redshift of formation. Analytical
estimates of the number density of dark matter halos are useful in modeling
several cosmological phenomena. We use the excursion set formalism for
computing the formation rate of dark matter halos. We use an approach that
allows us to differentiate between major and minor mergers, as this is a
pertinent issue for semi-analytic models of galaxy formation. We compute the
formation rate for the Press-Schechter and the Sheth-Tormen mass function. We
show that the formation rate computed in this manner is positive at all scales.
We comment on the Sasaki formalism where negative halo formation rates are
obtained. Our estimates compare very well with N-Body simulations for a variety
of models. We also discuss the halo survival probability and the formation
redshift distributions using our method.Comment: 30 pages, 9 figure
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