227 research outputs found
Processing conditions for (Nd, Eu, Gd)-Ba-Cu-O ternary bulk superconductors
Abstract(Nd, Eu, Gd)-Ba-Cu-O ternary bulk superconductors have high potential for practical applications since they exhibit very high critical current densities and thus high field trapping capabilities. (Nd, Eu, Gd)-Ba-Cu-O superconductors are synthesized in a reduced oxygen atmosphere, which requires a control of oxygen partial pressure and needs a special device for hot seeding. In the present study, for simplicity, we employed Ar gas flow into the furnace to control oxygen partial pressure instead of flowing oxygen-controlled gas. Hence, it was necessary to modify the melt processing conditions to produce a single domain. Through the optimization of seeding temperature and cooling rate, we obtained the processing conditions, in which a single domain bulk (Nd, Eu, Gd)-Ba-Cu-O of 20mm diameter could be synthesized
Re-appearance of antiferromagnetic ordering with Zn and Ni substitution in La_{2-x}Sr_xCuO_4
The effects of nonmagnetic Zn and magnetic Ni substitution for Cu site on
magnetism are studied by measurements of uniform magnetic susceptibility for
lightly doped La_{2-x}Sr_xCu_{1-z}M_zO_4 (M=Zn or Ni) polycrystalline samples.
For the parent x=0, Zn doping suppresses the N\'{e}el temperature T_N whereas
Ni doping hardly changes T_N up to z=0.3. For the lightly doped samples with
T_N~0, the Ni doping recovers T_N. For the superconducting samples, the Ni
doping induces the superconductivity-to-antiferromagnetic transition (or
crossover). All the heavily Ni doped samples indicate a spin glass behavior at
\~15 K.Comment: 2 pages including 3 figures, to be published in Physica C (LT23,
Hiroshima 2002
Cu Nuclear Quadrupole Resonance Study of Site-Disorder and Chemical Pressure Effects on Y(Ba1-xSrx)2Cu4O8
We report a zero-field Cu nuclear quadrupole resonance (NQR) study on the
effects of nonmagnetic Sr substitution for high-Tc superconductors,
Y(Ba1-xSrx)2Cu4O8 (Tc=82-80 K for x=0-0.4), using a spin-echo technique. The
site-disordering and chemical pressure effects associated with doping Sr were
observed in the broadened, shifted Cu NQR spectra. Nevertheless, the site
disorder did not significantly affect the homogeneity of Cu electron spin
dynamics, in contrast to the in-plane impurity. The peak shift of Cu NQR
spectrum due to Sr was different between the chain- and the plane-Cu sites,
more remarkably than those under a hydrostatic physical pressure, suggesting
anisotropic or nonuniform local structural strains. The small decrease of Tc
due to Sr can be traced back to either a cancellation effect on Tc between the
disorder and the pressure, or an anisotropic or nonuniform chemical pressure
effect on Tc.Comment: 4 pages, 5 figure
Doping Effect of Nano-Diamond on Superconductivity and Flux Pinning in MgB2
Doping effect of diamond nanoparticles on the superconducting properties of
MgB2 bulk material has been studied. It is found that the superconducting
transition temperature Tc of MgB2 is suppressed by the diamond-doping, however,
the irreversibility field Hirr and the critical current density Jc are
systematically enhanced. Microstructural analysis shows that the diamond-doped
MgB2 superconductor consists of tightly-packed MgB2 nano-grains (~50-100 nm)
with highly-dispersed and uniformly-distributed diamond nanoparticles (~10-20
nm) inside the grains. High density of dislocations and diamond nanoparticles
may take the responsibility for the enhanced flux pinning in the diamond-doped
MgB2.Comment: 16 pages, 6 figure
Ni-substituted sites and the effect on Cu electron spin dynamics of YBa2Cu{3-x}NixO{7-\delta}
We report Cu nuclear quadrupole resonance experiment on magnetic impurity
Ni-substituted YBaCuNiO. The distribution of
Ni-substituted sites and its effect on the Cu electron spin dynamics are
investigated. Two samples with the same Ni concentration =0.10 and nearly
the same oxygen content but different 's were prepared: One is an
as-synthesized sample (7-=6.93) in air (), and the
other is a quenched one (7-=6.92) in a reduced oxygen atmosphere
(). The plane-site Cu(2) nuclear spin-lattice
relaxation for the quenched sample was faster than that for the as-synthesized
sample, in contrast to the Cu(1) relaxation that was faster for the
as-synthesized sample. This indicates that the density of plane-site Ni(2) is
higher in the quenched sample, contrary to the chain-site Ni(1) density which
is lower in the quenched sample. From the analysis in terms of the Ni-induced
nuclear spin-lattice relaxation, we suggest that the primary origin of
suppression of is associated with nonmagnetic depairing effect of the
plane-site Ni(2).Comment: 7 pages, 5 figure
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Nonlinear microwave switching response of BSCCO single crystals
Measurements of the surface impedance in Bi{sub 2}Sr{sub 2}CaCu{sub 2}O{sub 8+{delta}} single crystal with microwave currents flowing along the {cflx c} axis show clear evidence of a step-like nonlinearity. The surface resistance switches between apparently quantized levels for microwave field strength changes < 1 mG. This nonlinear response can arise from the presence of intrinsic Josephson junctions along the {cflx c} axis of these samples driven by the microwave current
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