Smith-Purcell Radiation from Low-Energy Electrons

Recent advances in the fabrication of nanostructures and nanoscale features in metasurfaces offer a new prospect for generating visible, light emission from low energy electrons. In this paper, we present the experimental observation of visible light emission from low-energy free electrons interacting with nanoscale periodic surfaces through the Smith-Purcell (SP) effect. SP radiation is emitted when electrons pass in close proximity over a periodic structure, inducing collective charge motion or dipole excitations near the surface, thereby giving rise to electromagnetic radiation. We demonstrate a controlled emission of SP light from nanoscale gold gratings with periodicity as small as 50 nm, enabling the observation of visible SP radiation by low energy electrons (1.5 to 6 keV), an order of magnitude lower than previously reported. We study the emission wavelength and intensity dependence on the grating pitch and electron energy, showing agreement between experiment and theory. Further reduction of structure periodicity should enable the production of SP-based devices that operate with even slower electrons that allow an even smaller footprint and facilitate the investigation of quantum effects for light generation in nanoscale devices. A tunable light source integrated in an electron microscope would enable the development of novel electron-optical correlated spectroscopic techniques, with additional applications ranging from biological imaging to solid-state lighting.Comment: 16 pages, 4 figure

Rapid fabrication of 3D terahertz split ring resonator arrays by novel single-shot direct write focused proximity field nanopatterning

For the next generation of phoXonic, plasmonic, optomechanical and microfluidic devices, the capability to create 3D microstructures is highly desirable. Fabrication of such structures by conventional top-down techniques generally requires multiple timeconsuming steps and is limited in the ability to define features spanning multiple layers at prescribed angles. 3D direct write lithography (3DDW) has the capability to draw nearly arbitrary structures, but is an inherently slow serial writing process. Here we present a method, denoted focused proximity field nanopatterning (FPnP), that combines 3DDW with single or multiphoton interference lithography (IL). By exposing a thick photoresist layer having a phase mask pattern imprinted on its surface with a tightly focused laser beam, we produce locally unique complex structures. The morphology can be varied based on beam and mask parameters. Patterns may be written rapidly in a single shot mode with arbitrary positions defined by the direct write, thus exploiting the control of 3DDW with the enhanced speed of phase mask IL. Here we show the ability for this technique to rapidly produce arrays of “stand-up” far IR resonators

Interferometric analysis of laser-driven cylindrically focusing shock waves in a thin liquid layer

Shock waves in condensed matter are of great importance for many areas of science and technology ranging from inertially confined fusion to planetary science and medicine. In laboratory studies of shock waves, there is a need in developing diagnostic techniques capable of measuring parameters of materials under shock with high spatial resolution. Here, time-resolved interferometric imaging is used to study laser-driven focusing shock waves in a thin liquid layer in an all-optical experiment. Shock waves are generated in a 10 µm-thick layer of water by focusing intense picosecond laser pulses into a ring of 95 µm radius. Using a Mach-Zehnder interferometer and time-delayed femtosecond laser pulses, we obtain a series of images tracing the shock wave as it converges at the center of the ring before reemerging as a diverging shock, resulting in the formation of a cavitation bubble. Through quantitative analysis of the interferograms, density profiles of shocked samples are extracted. The experimental geometry used in our study opens prospects for spatially resolved spectroscopic studies of materials under shock compression.Massachusetts Institute of Technology. Institute for Soldier Nanotechnologies (Contract W911NF-13-D-0001

Fullwave Maxwell inverse design of axisymmetric, tunable, and multi-scale multi-wavelength metalenses

We demonstrate new axisymmetric inverse-design techniques that can solve problems radically different from traditional lenses, including \emph{reconfigurable} lenses (that shift a multi-frequency focal spot in response to refractive-index changes) and {\emph{widely separated}} multi-wavelength lenses ($\lambda = 1\,\mu$m and $10\,\mu$m). We also present experimental validation for an axisymmetric inverse-designed monochrome lens in the near-infrared fabricated via two-photon polymerization. Axisymmetry allows fullwave Maxwell solvers to be scaled up to structures hundreds or even thousands of wavelengths in diameter before requiring domain-decomposition approximations, while multilayer topology optimization with $\sim 10^5$ degrees of freedom can tackle challenging design problems even when restricted to axisymmetric structures.Comment: 13 pages, 6 figure

Multi-frame Interferometric Imaging with a Femtosecond Stroboscopic Pulse Train for Observing Irreversible Phenomena

We describe a high-speed single-shot multi-frame interferometric imaging technique enabling multiple interferometric images with femtosecond exposure time over a 50 ns event window to be recorded following a single laser-induced excitation event. The stroboscopic illumination of a framing camera is made possible through the use of a doubling cavity which produces a femtosecond pulse train that is synchronized to the gated exposure windows of the individual frames of the camera. The imaging system utilizes a Michelson interferometer to extract phase and ultimately displacement information. We demonstrate the method by monitoring laser-induced deformation and the propagation of high-amplitude acoustic waves in a silicon nitride membrane. The method is applicable to a wide range of fast irreversible phenomena such as crack branching, shock-induced material damage, cavitation and dielectric breakdown

Additive Laser Excitation of Giant Nonlinear Surface Acoustic Wave Pulses

The laser ultrasonics technique perfectly fits the needs for non-contact, non-invasive, non-destructive mechanical probing of samples of mm to nm sizes. This technique is however limited to the excitation of low-amplitude strains, below the threshold for optical damage of the sample. In the context of strain engineering of materials, alternative optical techniques enabling the excitation of high amplitude strains in a non-destructive optical regime are seeking. We introduce here a non-destructive method for laser-shock wave generation based on additive superposition of multiple laser-excited strain waves. This technique enables strain generation up to mechanical failure of a sample at pump laser fluences below optical ablation or melting thresholds. We demonstrate the ability to generate nonlinear surface acoustic waves (SAWs) in Nb:SrTiO$_3$ substrates, at typically 1 kHz repetition rate, with associated strains in the percent range and pressures close to 100 kbars. This study paves the way for the investigation of a host of high-strength SAW-induced phenomena, including phase transitions in conventional and quantum materials, plasticity and a myriad of material failure modes, chemistry and other effects in bulk samples, thin layers, or two-dimensional materials

Biasing the quantum vacuum to control macroscopic probability distributions

One of the most important insights of quantum field theory is that electromagnetic fields must fluctuate. Even in the vacuum state, the electric and magnetic fields have a nonzero variance, leading to ubiquitous effects such as spontaneous emission, the Lamb shift, the Casimir effect, and more. These "vacuum fluctuations" have also been harnessed as a source of perfect randomness, for example to generate perfectly random photonic bits. Despite these achievements, many potential applications of quantum randomness in fields such as probabilistic computing rely on controllable probability distributions, which have not yet been realized on photonic platforms. In this work, we show that the injection of vacuum-level "bias" fields into a multi-stable optical system enables a controllable source of "biased" quantum randomness. We demonstrate this concept in an optical parametric oscillator (OPO). Ordinarily, an OPO initiated from the ground state develops a signal field in one of two degenerate phase states (0 and $\pi$) with equal probability. By injecting bias pulses which contain less than one photon on average, we control the probabilities associated with the two output states, leading to the first controllable photonic probabilistic bit (p-bit). We shed light on the physics behind this process, showing quantitative agreement between theory and experiment. Finally, we demonstrate the potential of our approach for sensing sub-photon level fields by showing that our system is sensitive to the temporal shape of bias field pulses far below the single photon level. Our results suggest a new platform for the study of stochastic quantum dynamics in nonlinear driven-dissipative systems, and point toward possible applications in ultrafast photonic probabilistic computing, as well as the sensing of extremely weak fields

Maximal Spontaneous Photon Emission and Energy Loss from Free Electrons

Free electron radiation such as Cerenkov, Smith--Purcell, and transition radiation can be greatly affected by structured optical environments, as has been demonstrated in a variety of polaritonic, photonic-crystal, and metamaterial systems. However, the amount of radiation that can ultimately be extracted from free electrons near an arbitrary material structure has remained elusive. Here we derive a fundamental upper limit to the spontaneous photon emission and energy loss of free electrons, regardless of geometry, which illuminates the effects of material properties and electron velocities. We obtain experimental evidence for our theory with quantitative measurements of Smith--Purcell radiation. Our framework allows us to make two predictions. One is a new regime of radiation operation---at subwavelength separations, slower (nonrelativistic) electrons can achieve stronger radiation than fast (relativistic) electrons. The second is a divergence of the emission probability in the limit of lossless materials. We further reveal that such divergences can be approached by coupling free electrons to photonic bound states in the continuum (BICs). Our findings suggest that compact and efficient free-electron radiation sources from microwaves to the soft X-ray regime may be achievable without requiring ultrahigh accelerating voltages.Comment: 7 pages, 4 figure