15 research outputs found
Radiative cascades in charged quantum dots
We measured, for the first time, two photon radiative cascades due to
sequential recombination of quantum dot confined electron hole pairs in the
presence of an additional spectator charge carrier. We identified direct, all
optical cascades involving spin blockaded intermediate states, and indirect
cascades, in which non radiative relaxation precedes the second recombination.
Our measurements provide also spin dephasing rates of confined carriers.Comment: 4 pages, 3 figure
Complete control of a matter qubit using a single picosecond laser pulse
We demonstrate for the first time that a matter physical two level system, a
qubit, can be fully controlled using one ultrafast step. We show that the spin
state of an optically excited electron, an exciton, confined in a quantum dot,
can be rotated by any desired angle, about any desired axis, during such a
step. For this we use a single, resonantly tuned, picosecond long, polarized
optical pulse. The polarization of the pulse defines the rotation axis, while
the pulse detuning from a non-degenerate absorption resonance, defines the
magnitude of the rotation angle. We thereby achieve a high fidelity, universal
gate operation, applicable to other spin systems, using only one short optical
pulse. The operation duration equals the pulse temporal width, orders of
magnitude shorter than the qubit evolution life and coherence times.Comment: main text: 4 pages, 3 figures Supplemental material: 3 pages, 1
figur
Two-photon- photoluminescence excitation spectroscopy of single quantum-dots
We present experimental and theoretical study of single semiconductor quantum
dots excited by two non-degenerate, resonantly tuned variably polarized lasers.
The first laser is tuned to excitonic resonances. Depending on its polarization
it photogenerates a coherent single exciton state. The second laser is tuned to
biexciton resonances. By scanning the energy of the second laser for various
polarizations of the two lasers, while monitoring the emission from the
biexciton and exciton spectral lines, we map the biexciton photoluminescence
excitation spectra. The resonances rich spectra of the second photon absorption
are analyzed and fully understood in terms of a many carrier theoretical model
which takes into account the direct and exchange Coulomb interactions between
the quantum confined carriers.Comment: Accepted for publication in PR
Excitation spectroscopy of single quantum dots at tunable positive, neutral and negative charge states
We present a comprehensive study of the optical transitions and selection
rules of variably charged single self-assembled InAs/GaAs quantum dots. We
apply high resolution polarization sensitive photoluminescence excitation
spectroscopy to the same quantum dot for three different charge states: neutral
and negatively or positively charged by one additional electron or hole. From
the detailed analysis of the excitation spectra, a full understanding of the
single-carrier energy levels and the interactions between carriers in these
levels is extracted for the first time.Comment: 8 pages, 5 figure
Spontaneously Localized Photonic Modes Due to Disorder in the Dielectric Constant
We present the first experimental evidence for the existence of strongly
localized photonic modes due to random two dimensional fluctuations in the
dielectric constant. In one direction, the modes are trapped by ordered Bragg
reflecting mirrors of a planar, one wavelength long, microcavity. In the cavity
plane, they are localized by disorder, which is due to randomness in the
position, composition and sizes of quantum dots located in the anti-node of the
cavity. We extend the theory of disorder induced strong localization of
electron states to optical modes and obtain quantitative agreement with the
main experimental observations.Comment: 6 page
Optically induced rotation of a quantum dot exciton spin
We demonstrate control over the spin state of a semiconductor quantum dot
exciton using a polarized picosecond laser pulse slightly detuned from a
biexciton resonance. The control pulse follows an earlier pulse, which
generates an exciton and initializes its spin state as a coherent superposition
of its two non-degenerate eigenstates. The control pulse preferentially couples
one component of the exciton state to the biexciton state, thereby rotating the
exciton's spin direction. We detect the rotation by measuring the polarization
of the exciton spectral line as a function of the time-difference between the
two pulses. We show experimentally and theoretically how the angle of rotation
depends on the detuning of the second pulse from the biexciton resonance.Comment: 4 pages, 4 figures, accepted for publication in Physical Review
Letter
Radiative cascade from quantum dot metastable spin-blockaded biexciton
We detect a novel radiative cascade from a neutral semiconductor quantum dot.
The cascade initiates from a metastable biexciton state in which the holes form
a spin-triplet configuration, Pauli-blockaded from relaxation to the
spin-singlet ground state. The triplet biexciton has two photon-phonon-photon
decay paths. Unlike in the singlet-ground state biexciton radiative cascade, in
which the two photons are co-linearly polarized, in the triplet biexciton
cascade they are crosslinearly polarized. We measured the two-photon
polarization density matrix and show that the phonon emitted when the
intermediate exciton relaxes from excited to ground state, preserves the
exciton's spin. The phonon, thus, does not carry with it any which-path
information other than its energy. Nevertheless, entanglement distillation by
spectral filtering was found to be rather ineffective for this cascade. This
deficiency results from the opposite sign of the anisotropic electron-hole
exchange interaction in the excited exciton relative to that in the ground
exciton.Comment: 6 pages, 4 figure
The dark exciton in a quantum dot- A novel bright qubit with very long coherence time
We demonstrate for the first time that the quantum dot confined dark exciton is a natural, coherent and long-lived qubit. We optically “write” its spin state and successfully “read” its subsequent coherent evolution