Observation of strong electromagnetic fields around laser-entrance holes of ignition-scale hohlraums in inertial-confinement fusion experiments at the National Ignition Facility

Energy spectra and spectrally resolved one-dimensional fluence images of self-emitted charged-fusion products (14.7 MeV D[superscript 3]He protons) are routinely measured from indirectly driven inertial-confinement fusion (ICF) experiments utilizing ignition-scaled hohlraums at the National Ignition Facility (NIF). A striking and consistent feature of these images is that the fluence of protons leaving the ICF target in the direction of the hohlraum's laser entrance holes (LEHs) is very nonuniform spatially, in contrast to the very uniform fluence of protons leaving through the hohlraum equator. In addition, the measured nonuniformities are unpredictable, and vary greatly from shot to shot. These observations were made separately at the times of shock flash and of compression burn, indicating that the asymmetry persists even at ~0.5–2.5 ns after the laser has turned off. These phenomena have also been observed in experiments on the OMEGA laser facility with energy-scaled hohlraums, suggesting that the underlying physics is similar. Comprehensive data sets provide compelling evidence that the nonuniformities result from proton deflections due to strong spontaneous electromagnetic fields around the hohlraum LEHs. Although it has not yet been possible to uniquely determine whether the fields are magnetic (B) or electric (E), preliminary analysis indicates that the strength is ~1 MG if B fields or ~10[superscript 9] V cm[superscript −1] if E fields. These measurements provide important physics insight into the ongoing ignition experiments at the NIF. Understanding the generation, evolution, interaction and dissipation of the self-generated fields may help to answer many physics questions, such as why the electron temperatures measured in the LEH region are anomalously large, and may help to validate hydrodynamic models of plasma dynamics prior to plasma stagnation in the center of the hohlraum.United States. Dept. of Energy (DE-FG52-07 NA280 59)United States. Dept. of Energy (DE-FG03-03SF22691)Lawrence Livermore National Laboratory (B543881)Lawrence Livermore National Laboratory (LD RD-08-ER-062)University of Rochester. Fusion Science Center (412761-G)General Atomics (DE-AC52-06NA 27279)Stewardship Science Graduate Fellowship (DE-FC52-08NA28752

Demonstration of High Performance in Layered Deuterium-Tritium Capsule Implosions in Uranium Hohlraums at the National Ignition Facility

We report on the first layered deuterium-tritium (DT) capsule implosions indirectly driven by a “high-foot” laser pulse that were fielded in depleted uranium hohlraums at the National Ignition Facility. Recently, high-foot implosions have demonstrated improved resistance to ablation-front Rayleigh-Taylor instability induced mixing of ablator material into the DT hot spot [Hurricane et al., Nature (London) 506, 343 (2014)]. Uranium hohlraums provide a higher albedo and thus an increased drive equivalent to an additional 25 TW laser power at the peak of the drive compared to standard gold hohlraums leading to higher implosion velocity. Additionally, we observe an improved hot-spot shape closer to round which indicates enhanced drive from the waist. In contrast to findings in the National Ignition Campaign, now all of our highest performing experiments have been done in uranium hohlraums and achieved total yields approaching 10[superscript 16] neutrons where more than 50% of the yield was due to additional heating of alpha particles stopping in the DT fuel.United States. Dept. of Energy (Lawrence Livermore National Laboratory Contract DE-AC52-07NA27344

Review on catalytic cleavage of C-C inter-unit linkages in lignin model compounds: Towards lignin depolymerisation

Lignin depolymerisation has received considerable attention recently due to the pressing need to find sustainable alternatives to fossil fuel feedstock to produce chemicals and fuels. Two types of interunit linkages (C–C and C–O linkages) link several aromatic units in the structure of lignin. Between these two inter-unit linkages, the bond energies of C–C linkages are higher than that of C–O linkages, making them harder to break. However, for an efficient lignin depolymerisation, both types of inter-unit linkages have to be broken. This is more relevant because of the fact that many delignification processes tend to result in the formation of additional C–C inter-unit bonds. Here we review the strategies reported for the cleavage of C–C inter-unit linkages in lignin model compounds and lignin. Although a number of articles are available on the cleavage of C–O inter-unit linkages, reports on the selective cleavage of C–C inter-unit linkages are relatively less. Oxidative cleavage, hydrogenolysis, two-step redox-neutral process, microwave assisted cleavage, biocatalytic and photocatalytic methods have been reported for the breaking of C–C inter-unit linkages in lignin. Here we review all these methods in detail, focused only on the breaking of C–C linkages. The objective of this review is to motivate researchers to design new strategies to break this strong C–C inter-unit bonds to valorise lignins, technical lignins in particular

Lawson criterion for ignition exceeded in an inertial fusion experiment

For more than half a century, researchers around the world have been engaged in attempts to achieve fusion ignition as a proof of principle of various fusion concepts. Following the Lawson criterion, an ignited plasma is one where the fusion heating power is high enough to overcome all the physical processes that cool the fusion plasma, creating a positive thermodynamic feedback loop with rapidly increasing temperature. In inertially confined fusion, ignition is a state where the fusion plasma can begin "burn propagation" into surrounding cold fuel, enabling the possibility of high energy gain. While "scientific breakeven" (i.e., unity target gain) has not yet been achieved (here target gain is 0.72, 1.37 MJ of fusion for 1.92 MJ of laser energy), this Letter reports the first controlled fusion experiment, using laser indirect drive, on the National Ignition Facility to produce capsule gain (here 5.8) and reach ignition by nine different formulations of the Lawson criterion