Excitonic and lattice contributions to the charge density wave in 1T-TiSe2 revealed by a phonon bottleneck

Understanding collective electronic states such as superconductivity and charge density waves is pivotal for fundamental science and applications. The layered transition metal dichalcogenide 1T-TiSe2 hosts a unique charge density wave (CDW) phase transition whose origins are still not fully understood. Here, we present ultrafast time- and angle-resolved photoemission spectroscopy (TR-ARPES) measurements complemented by time-resolved reflectivity (TRR) which allows us to establish the contribution of excitonic and electron-phonon interactions to the CDW. We monitor the energy shift of the valence band (VB) and coupling to coherent phonons as a function of laser fluence. The VB shift, directly related to the CDW gap closure, exhibits a markedly slower recovery dynamics at fluences above Fth = 60 microJ cm-2. This observation coincides with a shift in the relative weight of coherently coupled phonons to higher frequency modes in time-resolved reflectivity (TRR), suggesting a phonon bottleneck. Using a rate equation model, the emergence of a high-fluence bottleneck is attributed to an abrupt reduction in coupled phonon damping and an increase in exciton dissociation rate linked to the loss of CDW superlattice phonons. Thus, our work establishes the important role of both excitonic and phononic interactions in the CDW phase transition and the advantage of combining complementary femtosecond techniques to understand the complex interactions in quantum materials.Comment: 11 pages, 4 figure

Anisotropic Zeeman Splitting in YbNi4P2

The electronic structure of heavy-fermion materials is highly renormalised at low temperatures with localised moments contributing to the electronic excitation spectrum via the Kondo effect. Thus, heavy-fermion materials are very susceptible to Lifshitz transitions due to the small effective Fermi energy arising on parts of the renormalised Fermi surface. Here, we study Lifshitz transitions that have been discovered in YbNi4P2 in high magnetic fields. We measure the angular dependence of the critical fields necessary to induce a number of Lifshitz transitions and find it to follow a simple Zeeman-shift model with anisotropic g-factor. This highlights the coherent nature of the heavy quasiparticles forming a renormalised Fermi surface. We extract information on the orientation of the Fermi surface parts giving rise to the Lifshitz transitions and we determine the anisotropy of the effective g-factor to be $\eta \approx 3.8$ in good agreement with the crystal field scheme of YbNi4P2

Numerical studies on vibration propagation and damping test V1

Earthquakes and aircraft impacts induce vibrations that propagate throughout the entire building and they need to be considered in designing SSCs (Structures, Systems and Components). Mainly linear calculation methods have been in use in design practice and the codes and standards consider damping ratios only for linear structural analyses. Induced vibrations, especially in damaged concrete structures, have not been studied extensively enough for optimization of structural frameworks and/or qualified systems and components. Experimental data on damping properties of damaged reinforced concrete are needed also for benchmarking analysis programs and methods. Recently, within IMPACT project, a new type of test series considering vibration propagation has been carried out at VTT. The test target is a reinforced concrete structure with two parallel walls connected to a floor slab. The front wall is additionally supported by triangular shaped side walls which are connected to the floor slab too. The test structure is supported on elastomeric bearing pads, with back pipes effective mainly in compression and with bars effective in tension. In order to obtain information on vibration propagation in damaged concrete structure at different levels of damage grades the same structure was tested six times. At each time the mass of the deformable stainless steel missile was 50 kg. The hit point located in the middle of the front wall. The impact velocity was about 110 m/s in the first four tests (V1A-D) and about 60 m/s in the remaining two tests (V1E and F). In this paper, numerical results on tests V1A and V1F are compared with the corresponding experimental ones. The calculated results, such as accelerations, displacements, their response spectra and strains, are compared with experimental measurements. Five finite element (FE) programs are used in computations: Abaqus, Europlexus, LS-DYNA, SOFiSTiK and an in-house code (IHC). Most of the FE-codes in the present study use shell elements. In Abaqus and SOFiSTiK non-linear behaviour of shell section is modelled by dividing the cross section into layers. Reinforcements are also modelled as layers. In Europlexus and IHC, an alternative approach is adopted in which the non-linear behaviour of concrete and reinforcement is homogenized beforehand in the shell thickness direction obtaining relations between stress resultants and generalized strains valid for the shell section. In LS-DYNA, 3D solid elements for modelling concrete and beam elements for modelling reinforcements are used. Equations of motion are integrated with explicit central difference time integration method, except in SOFiSTiK implicit integration method is used. Modelling and computations with the mentioned FE-programs are made independently of each other. Computations with LS-DYNA are carried out as blind exercises. Consideration of the results from benchmarking point of view is still on-going. However it is evident that analysed results follow reasonable well test results in main design parameter level such as maximum displacements, accelerations and strains. Also frequency spectra are estimated reasonably well