Magnetocrystalline anisotropy in single-crystal Co-Ni-Al ferromagnetic shape-memory alloy

科研費報告書収録論文(課題番号:13555181・基盤研究(B)(2) ・H13～H14/研究代表者:貝沼, 亮介/新しいB2型強磁性形状記憶合金の開発と多機能素子への展開

Lattice dynamics and phonon softening in Ni-Mn-Al Heusler alloys

Inelastic and elastic neutron scattering have been used to study a single crystal of the Ni$_{54}$Mn$_{23}$Al$_{23}$ Heusler alloy over a broad temperature range. The paper reports the first experimental determination of the low-lying phonon dispersion curves for this alloy system. We find that the frequencies of the TA$_2$ modes are relatively low. This branch exhibits an anomaly (dip) at a wave number $\xi_{0} ={1/3}\approx 0.33$, which softens with decreasing temperature. Associated with this anomalous dip at $\xi_{0}$, an elastic central peak scattering is also present. We have also observed satellites due to the magnetic ordering.Comment: 6 pages, 6 figures. Accepted for publication in the Physical Review

Geometrical Magnetic Frustration in Rare Earth Chalcogenide Spinels

We have characterized the magnetic and structural properties of the CdLn2Se4 (Ln = Dy, Ho), and CdLn2S4 (Ln = Ho, Er, Tm, Yb) spinels. We observe all compounds to be normal spinels, possessing a geometrically frustrated sublattice of lanthanide atoms with no observable structural disorder. Fits to the high temperature magnetic susceptibilities indicate these materials to have effective antiferromagnetic interactions, with Curie-Weiss temperatures theta ~ -10 K, except CdYb2S4 for which theta ~ -40 K. The absence of magnetic long range order or glassiness above T = 1.8 K strongly suggests that these materials are a new venue in which to study the effects of strong geometrical frustration, potentially as rich in new physical phenomena as that of the pyrochlore oxides.Comment: 17 pages, 5 figures, submitted to Phys Rev B; added acknowledgement