770 research outputs found
High-energy spin and charge excitations in electron-doped copper oxide superconductors
The evolution of electronic (spin and charge) excitations upon carrier doping
is an extremely important issue in superconducting layered cuprates and the
knowledge of its asymmetry between electron- and hole-dopings is still
fragmentary. Here we combine x-ray and neutron inelastic scattering
measurements to track the doping dependence of both spin and charge excitations
in electron-doped materials. Copper L3 resonant inelastic x-ray scattering
spectra show that magnetic excitations shift to higher energy upon doping.
Their dispersion becomes steeper near the magnetic zone center and deeply mix
with charge excitations, indicating that electrons acquire a highly itinerant
character in the doped metallic state. Moreover, above the magnetic
excitations, an additional dispersing feature is observed near the
{\Gamma}-point, and we ascribe it to particle-hole charge excitations. These
properties are in stark contrast with the more localized spin-excitations
(paramagnons) recently observed in hole-doped compounds even at high
doping-levels.Comment: 20 page
The Effect of - Magnetic Coupling in Multiferroic MnO Crystals
We have established detailed magnetoelectric phase diagrams of
(EuY)TbMnO () and
(Eu,Y)GdMnO (), whose average ionic radii of
-site (: rare earth) cations are equal to that of Tb, in order to
reveal the effect of rare earth 4 magnetic moments on the magnetoelectric
properties. In spite of the same -site ionic radii, the magnetoelectric
properties of the two systems are remarkably different from each other. A small
amount of Tb substitution on sites () totally destroys
ferroelectric polarization along the a axis (), and an increase in Tb
concentration stabilizes the phase. On the other hand, Gd substitution
() extinguishes the phase, and slightly suppresses the
phase. These results demonstrate that the magnetoelectric properties of
MnO strongly depend on the characteristics of the rare earth 4
moments.Comment: 10 pages, 5 figures Submitted to Journal of the Physical Society of
Japa
Chemical potential shift and spectral weight transfer in PrCaMnO revealed by photoemission spectroscopy
We have studied the chemical potential shift and changes in the electronic
density of states near the Fermi level () as a function of carrier
concentration in PrCaMnO (PCMO, ) through
the measurements of photoemission spectra. The results showed that the chemical
potential shift was suppressed for x \agt 0.3, where the charge exchange
(CE)-type antiferromagnetic charge-ordered state appears at low temperatures.
We consider this observation to be related to charge self-organization such as
stripe formation on a microscopic scale in this composition range. Together
with the previous observation of monotonous chemical potential shift in
LaSrMnO, we conclude that the tendency toward the charge
self-organization increases with decreasing bandwidth. In the valence band,
spectral weight of the Mn 3 electrons in PCMO was transferred from
1 eV below to the region near with hole doping, leading to a
finite intensity at even in the paramagnetic insulating phase for x \agt
0.3, probably related with the tendency toward charge self-organization. The
finite intensity at in spite of the insulating transport behavior is
consistent with fluctuations involving ferromagnetic metallic states.Comment: 6 pages, 5 figure
Magnetic Field resulting from non-linear electrical transport in single crystals of charge-ordered Pr Ca MnO}
In this letter we report that the current induced destabilization of the
charge ordered (CO) state in a rare-earth manganite gives rise to regions with
ferromagnetic correlation. We did this experiment by measurement of the I-V
curves in single crystal of the CO system
PrCaMnO and simultanously measuring the magnetization
of the current carrying conductor using a high T SQUID working at T = 77K.
We have found that the current induced destabilization of the CO state leads to
a regime of negative differential resistance which leads to a small enhancement
of the magnetization of the sample, indicating ferromagnetically aligned
moments.Comment: 4 pages LateX, 4 eps figure
Influence of Mg, Ag and Al substitutions on the magnetic excitations in the triangular-lattice antiferromagnet CuCrO2
Magnetic excitations in CuCrO, CuCrMgO,
CuAgCrO, and CuCrAlO have been
studied by powder inelastic neutron scattering to elucidate the element
substitution effects on the spin dynamics in the Heisenberg triangular-lattice
antiferromagnet CuCrO. The magnetic excitations in
CuCrMgO consist of a dispersive component and a flat
component. Though this feature is apparently similar to CuCrO, the energy
structure of the excitation spectrum shows some difference from that in
CuCrO. On the other hand, in CuAgCrO and
CuCrAlO the flat components are much reduced, the
low-energy parts of the excitation spectra become intense, and additional
low-energy diffusive spin fluctuations are induced. We argued the origins of
these changes in the magnetic excitations are ascribed to effects of the doped
holes or change of the dimensionality in the magnetic correlations.Comment: 7 pages, 5 figure
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