212 research outputs found
Evidence for mass renormalization in LaNiO$"" sub 3_: an in situ soft x-ray photoemission study of epitaxial films
We investigate the electronic structure of high-quality single-crystal
LaNiO (LNO) thin films using in situ photoemission spectroscopy (PES). The
in situ high-resolution soft x-ray PES measurements on epitaxial thin films
reveal the intrinsic electronic structure of LNO. We find a new sharp feature
in the PES spectra crossing the Fermi level, which is derived from the
correlated Ni 3 electrons. This feature shows significant enhancement
of spectral weight with decreasing temperature. From a detailed analysis of
resistivity data, the enhancement of spectral weight is attributed to
increasing electron correlations due to antiferromagnetic fluctuations.Comment: 4 pages, 4 figures. submitted to Phys. Rev.
Photoemission evidence for a Mott-Hubbard metal-insulator transition in VO
The temperature () dependent metal-insulator transition (MIT) in VO is
investigated using bulk sensitive hard x-ray ( 8 keV) valence band, core
level, and V 2 resonant photoemission spectroscopy (PES). The valence
band and core level spectra are compared with full-multiplet cluster model
calculations including a coherent screening channel. Across the MIT, V 3
spectral weight transfer from the coherent ( final)
states at Fermi level to the incoherent ( final)
states, corresponding to the lower Hubbard band, lead to gap-formation. The
spectral shape changes in V 1 and V 2 core levels as well as the valence
band are nicely reproduced from a cluster model calculations, providing
electronic structure parameters. Resonant-PES finds that the
states resonate across the V 2 threshold in
addition to the and states. The results support
a Mott-Hubbard transition picture for the first order MIT in VO.Comment: 6 pages, 3 figures. to be published in Phys. Rev.
Coexistence of Bloch electrons and glassy electrons in Ca10(Ir4As8)(Fe2_xIrxAs2)5 revealed by angle-resolved photoemission spectroscopy
Angle-resolved photoemission spectroscopy of Ca10(Ir4As8)(Fe2_xIrxAs2)5 shows
that the Fe 3d electrons in the FeAs layer form the hole-like Fermi pocket at
the zone center and the electron-like Fermi pockets at the zone corners as
commonly seen in various Fe-based superconductors. The FeAs layer is heavily
electron doped and has relatively good two dimensionality. On the other hand,
the Ir 5d electrons are metallic and glassy probably due to atomic disorder
related to the Ir 5d orbital instability. Ca10(Ir4As8)(Fe2_xIrxAs2)5 exhibits a
unique electronic state where the Bloch electrons in the FeAs layer coexist
with the glassy electrons in the Ir4As8 layer.Comment: 4 pages, 3 figure
Self-Energy Effects on the Low- to High-Energy Electronic Structure of SrVO3
The correlated electronic structure of SrVO3 has been investigated by
angle-resolved photoemission spectroscopy using in-situ prepared thin films.
Pronounced features of band renormalization have been observed: a sharp kink
~60 meV below the Fermi level (EF) and a broad so-called "high-energy kink"
~0.3 eV below EF as in the high-Tc cuprates although SrVO3 does not show
magnetic fluctuations. We have deduced the self-energy in a wide energy range
by applying the Kramers-Kronig relation to the observed spectra. The obtained
self-energy clearly shows a large energy scale of ~0.7 eV which is attributed
to electron-electron interaction and gives rise to the ~0.3 eV "kink" in the
band dispersion as well as the incoherent peak ~1.5eV below EF. The present
analysis enables us to obtain consistent picture both for the incoherent
spectra and the band renormalization.Comment: 5 pages, 3 figure
Giant Rashba splitting of quasi-1D surface states on Bi/InAs(110)-(21)
Electronic states on the Bi/InAs(110)-(21) surface and its
spin-polarized structure are revealed by angle-resolved photoelectron
spectroscopy (ARPES), spin-resolved ARPES, and density-functional-theory
calculation. The surface state showed quasi-one-dimensional (Q1D) dispersion
and a nearly metallic character; the top of the hole-like surface band is just
below the Fermi level. The size of the Rashba parameter ()
reached quite a large value (5.5 eV\AA). The present result would provide
a fertile playground for further studies of the exotic electronic phenomena in
1D or Q1D systems with the spin-split electronic states as well as for advanced
spintronic devices.Comment: 8 pages (double column), 7 figures and 1 tabl
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