446 research outputs found
Experimental band structure of the nearly half-metallic CuCrSe: An optical and magneto-optical study
Diagonal and off-diagonal optical conductivity spectra have been determined
form the measured reflectivity and magneto-optical Kerr effect (MOKE) over a
broad range of photon energy in the itinerant ferromagnetic phase of
CuCrSe at various temperatures down to T=10 K. Besides the low-energy
metallic contribution and the lower-lying charge transfer transition at
2 eV, a sharp and distinct optical transition was observed in the
mid-infrared region around 0.5 eV with huge magneto-optical activity.
This excitation is attributed to a parity allowed transition through the Se-Cr
hybridization-induced gap in the majority spin channel. The large off-diagonal
conductivity is explained by the high spin polarization in the vicinity of the
Fermi level and the strong spin-orbit interaction for the related charge
carriers. The results are discussed in connection with band structure
calculations
Coexistence of localized and itinerant electrons in BaFe2X3 (X = S and Se) revealed by photoemission spectroscopy
We report a photoemission study at room temperature on BaFe2X3 (X = S and Se)
and CsFe2Se3 in which two-leg ladders are formed by the Fe sites. The Fe 2p
core-level peaks of BaFe2X3 are broad and exhibit two components, indicating
that itinerant and localized Fe 3d sites coexist similar to KxFe2-ySe2. The Fe
2p core-level peak of CsFe2Se3 is rather sharp and is accompanied by a
charge-transfer satellite. The insulating ground state of CsFe2Se3 can be
viewed as a Fe2+ Mott insulator in spite of the formal valence of +2.5. The
itinerant versus localized behaviors can be associated with the stability of
chalcogen p holes in the two-leg ladder structure.Comment: 5 pages, 5 figures, Accepted in publication for Physical Review
Pressure-induced changes in the magnetic and valence state of EuFe2As2
We present the results of electrical resistivity, ac specific heat, magnetic
susceptibility, X-ray absorption spectroscopy (XAS) and X-ray magnetic circular
dichroism (XMCD) of the ternary iron arsenide EuFe2As2 single crystal under
pressure. Applying pressure leads to a continuous suppression of the
antiferromagnetism associated with Fe moments and the antiferromagnetic
transition temperature becomes zero in the vicinity of a critical pressure Pc
~2.5-2.7 GPa. Pressure-induced re-entrant superconductivity, which is highly
sensitive to the homogeneity of the pressure, only appears in the narrow
pressure region in the vicinity of Pc due to the competition between
superconductivity and the antiferromagnetic ordering of Eu2+ moments. The
antiferromagnetic state of Eu2+ moments changes to the ferromagnetic state
above 6 GPa. We also found that the ferromagnetic order is suppressed with
further increasing pressure, which is connected with a valence change of Eu
ions.Comment: 7 pages, 7 figures, accepted for publication in Phys. Rev.
Anomalous Hall effect as a probe of the chiral order in spin glasses
Anomalous Hall effect arising from the noncoplanar spin configuration
(chirality) is discussed as a probe of the chiral order in spin glasses. It is
shown that the Hall coefficient yields direct information about the linear and
nonlinear chiral susceptibilities of the spin sector, which has been hard to
obtain experimentally from the standard magnetic measurements. Based on the
chirality scenario of spin-glass transition, predictions are given on the
behavior of the Hall resistivity of canonical spin glasses.Comment: Order estimate of the effect given, one reference added. To appear in
Phys. Rev. Letter
Spin Chirality Fluctuation and Anomalous Hall Effect in Itinerant Ferromagnets
The anomalous Hall effect due to the spin chirality order and fluctuation is
studied theoretically in a Kondo lattice model without the relativistic
spin-orbit interaction. Even without the correlations of the localized spins,
can emerge depending on the lattice structure and the spin
anisotropy. We reveal the condition for this chirality-fluctuation driven
mechanism for . Our semiquantitative estimates for a pyrochlore
oxide NdMoO give a finite \sigma_{xy} \sim 10 \Ohm^{-1} \cm^{-1}
together with a high resistivity \rho_{xx} \sim 10^{-4}-10^{-3} \Ohm \cm, in
agreement with experiments.Comment: 5 pages, including 4 figure
Parity-broken ground state for the spin-1 pyrochlore antiferromagnet
The ground-state properties of the spin-1 pyrochlore antiferromagnet are
studied by applying the VBS-like tetrahedron-unit decomposition to the original
spin system. The symmetrization required on every vertex is taken into account
by introducing a ferromagnetic coupling. The pairwise effective Hamiltonian
between the adjacent tetrahedrons is obtained by considering the next nearest
neighbor and the third neighbor exchange interactions. We find that the
transverse component of the spin chirality exhibits a long-range order,
breaking the parity symmetry of the tetrahedral group, while the chirality
itself is not broken.Comment: 4 pages, 3 figures, REVTeX(ver.3.1
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