1,131 research outputs found
Formation of an Icosahedral Structure during the Freezing of Gold Nanoclusters: Surface-Induced Mechanism
The freezing behavior of gold nanoclusters was studied by employing molecular
dynamics simulations based on a semi-empirical embedded-atom method.
Investigations of the gold nanoclusters revealed that, just after freezing,
ordered nano-surfaces with a fivefold symmetry were formed with interior atoms
remaining in the disordered state. Further lowering of temperatures induced
nano-crystallization of the interior atoms that proceeded from the surface
towards the core region, finally leading to an icosahedral structure. These
dynamic processes explain why the icosahedral cluster structure is dominantly
formed in spite of its energetic metastability.Comment: 9 pages, 4 figures(including 14 eps-files
The Haldane-Rezayi Quantum Hall State and Magnetic Flux
We consider the general abelian background configurations for the
Haldane-Rezayi quantum Hall state. We determine the stable configurations to be
the ones with the spontaneous flux of with .
This gives the physical mechanism by which the edge theory of the state becomes
identical to the one for the 331 state. It also provides a new experimental
consequence which can be tested in the enigmatic plateau in a single
layer system.Comment: RevTex, 5 pages, 2 figures. v2:minor corrections. v4: published
version. Discussion on the thermodynamic limit adde
Direct observation of the mass renormalization in SrVO by angle resolved photoemission spectroscopy
We have performed an angle-resolved photoemission study of the
three-dimensional perovskite-type SrVO. Observed spectral weight
distribution of the coherent part in the momentum space shows cylindrical Fermi
surfaces consisting of the V 3 orbitals as predicted by
local-density-approximation (LDA) band-structure calculation. The observed
energy dispersion shows a moderately enhanced effective mass compared to the
LDA results, corresponding to the effective mass enhancement seen in the
thermodynamic properties. Contributions from the bulk and surface electronic
structures to the observed spectra are discussed based on model calculations.Comment: 5 pages, 5 figure
Theoretical study of the thermal behavior of free and alumina-supported Fe-C nanoparticles
The thermal behavior of free and alumina-supported iron-carbon nanoparticles
is investigated via molecular dynamics simulations, in which the effect of the
substrate is treated with a simple Morse potential fitted to ab initio data. We
observe that the presence of the substrate raises the melting temperature of
medium and large nanoparticles ( = 0-0.16, = 80-1000, non-
magic numbers) by 40-60 K; it also plays an important role in defining the
ground state of smaller Fe nanoparticles ( = 50-80). The main focus of our
study is the investigation of Fe-C phase diagrams as a function of the
nanoparticle size. We find that as the cluster size decreases in the
1.1-1.6-nm-diameter range the eutectic point shifts significantly not only
toward lower temperatures, as expected from the Gibbs-Thomson law, but also
toward lower concentrations of C. The strong dependence of the maximum C
solubility on the Fe-C cluster size may have important implications for the
catalytic growth of carbon nanotubes by chemical vapor deposition.Comment: 13 pages, 11 figures, higher quality figures can be seen in article 9
at http://alpha.mems.duke.edu/wahyu
Charge ordering and chemical potential shift in LaSrNiO studied by photoemission spectroscopy
We have studied the chemical potential shift in LaSrNiO and
the charge ordering transition in LaSrNiO by
photoemission spectroscopy. The result shows a large ( 1 eV/hole)
downward shift of the chemical potential with hole doping in the high-doping
regime ( 0.33) while the shift is suppressed in the low-doping
regime ( 0.33). This suppression is attributed to a
segregation of doped holes on a microscopic scale when the hole concentration
is lower than . In the sample, the
photoemission intensity at the chemical potential vanishes below the charge
ordering transition temperature 240 K.Comment: 5 pages, 4 figure
Chemical Potential Shift in NdCeCuO: Contrasting Behaviors of the Electron- and Hole-Doped Cuprates
We have studied the chemical potential shift in the electron-doped
superconductor NdCeCuO by precise measurements of
core-level photoemission spectra. The result shows that the chemical potential
monotonously increases with electron doping, quite differently from
LaSrCuO, where the shift is suppressed in the underdoped
region.
If the suppression of the shift in LaSrCuO is attributed
to strong stripe fluctuations, the monotonous increase of the chemical
potential is consistent with the absence of stripe fluctuations in
NdCeCuO. The chemical potential jump between
NdCuO and LaCuO is found to be much smaller than the
optical band gaps.Comment: 4 pages, 5 figure
Persistent edge currents for paired quantum hall states
We study the behavior of the persistent edge current for paired quantum Hall
states on the cylinder. We show that the currents are periodic with the unit
flux . At low temperatures, they exhibit anomalous oscillations in
their flux dependence.The shape of the functions converges to the sawtooth
function periodic with .Comment: RevTex 8 pages. one figure. to appear in Phys.Rev.
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