30,701 research outputs found
Optical Studies of a Layered Manganite La_{1.2}Sr_{1.8}Mn_2O_7 : Polaron Correlation Effect
Optical conductivity spectra of a cleaved ab-plane of a
La_{1.2}Sr_{1.8}Mn_2O_7 single crystal exhibit a small polaron absorption band
in the mid-infrared region at overall temperatures. With decreasing temperature
(T) to Curie temperature (T_C), the center frequency of the small polaron band
moves to a higher frequency, resulting in a gap-like feature, and that it
collapses to a lower frequency below T_C. Interestingly, with decreasing T, the
stretching phonon mode hardens above T_C and softens below T_C. These
concurring changes of lattice and electronic structure indicate that short
range polaron correlation exist above T_C but disappear with a magnetic
ordering.Comment: 4 pages including 5 figures. submitted to Phys. Rev.
Spin/Orbital Pattern-Dependent Polaron Absorption in Nd(1-x)Sr(x)MnO3
We investigated optical properties of Nd(1-x)Sr(x)MnO3 (x= 0.40, 0.50, 0.55,
and 0.65) single crystals. In the spin/orbital disordered state, their
conductivity spectra look quite similar, and the strength of the mid-infrared
absorption peak is proportional to x(1-x) consistent with the polaron picture.
As temperature lowers, the Nd(1-x)Sr(x)MnO3 samples enter into various
spin/orbital ordered states, whose optical responses are quite different. These
optical responses can be explained by the spin/orbital ordering
pattern-dependent polaron hopping.Comment: 3 figures (gzipped
A Scaling Behavior of Spectral Weight Changes in Perovskite Manganites La_{0.7-y}Pr_{y}Ca_{0.3}MnO_3
Optical conductivity spectra of La_{0.7-y}Pr_{y}Ca_{0.3}MnO_3 were
systematically investigated. For metallic samples, the spectral weight below
0.5 eV, whose magnitude can be represented by the effective carrier number
N_{eff}(0.5 eV), increases as temperature becomes lower. Regardless of the Pr
doping, all the measured values of N_{eff}(0.5 eV)/T_C fall into one scaling
curve. This scaling behavior could be explained by the theoretical model by
Roeder et al. [Phys. Rev. Lett. 76, 1356 (1996)], which includes spin double
exchange and Jahn-Teller lattice coupling to holes. With the Pr doping,
far-infrared conductivities were found to be suppressed, probably due to the
Anderson localization.Comment: Latex 2e, 8 pages including 4 postscript figures, submitted at Apr 2
Dimensional Crossover driven by Magnetic Ordering in Optical Conductivity of Pr_{1/2}Sr_{1/2}MnO_3
We investigated optical properties of Pr_{0.5}Sr_{0.5}MnO_3, which has the
A-type antiferromagnetic ordering at a low temperature. We found that T-
dependence of spectral weight transfer shows a clear correlation with the
magnetic phase transition. In comparison with the optical conductivity results
of Nd_{0.5}Sr_{0.5}MnO_3, which has the CE-type antiferromagnetic charge
ordering, we showed that optical properties of Pr_{0.5}Sr_{0.5}MnO_3 near the
Neel temperature could be explained by a crossover from 3D to 2D metals.
Details of spectral weight changes are consistent with the polaron picture.Comment: 11 pages, 4 figures, submitted to PRL at June
Direct observation of the spin polarization in Au atomic wires on Si(553)
The spin-resolved electronic band structure of Au-induced metallic atomic wires on a vicinal silicon surface, Si(553), was investigated using spin-and angle-resolved photoelectron spectroscopy. We directly measured the spin polarization of three partially filled one-dimensional metallic bands, a one-third-filled band, and the doublet of nearly half-filled bands. For the half-filled doublet, the strong apparent spin polarization was observed near the Fermi energy with a minor out-of-plane spin component. This observation is consistent with the Rashba-type spin-orbit splitting and with a recent experiment on a similar doublet of Si(557)-Au. In contrast, the one-third-filled band does not show a substantial spin polarization within the experimental accuracy, indicating a much smaller spin splitting, if any. These results are discussed for the origin of the partially filled bands and for the intriguing broken-symmetry ground state observed at low temperature.X11116sciescopu
- …