Event-by-event study of prompt neutrons from 239Pu(n,f)

Employing a recently developed Monte Carlo model, we study the fission of 240Pu induced by neutrons with energies from thermal to just below the threshold for second chance fission. Current measurements of the mean number of prompt neutrons emitted in fission, together with less accurate measurements of the neutron energy spectra, place remarkably fine constraints on predictions of microscopic calculations. In particular, the total excitation energy of the nascent fragments must be specified to within 1 MeV to avoid disagreement with measurements of the mean neutron multiplicity. The combination of the Monte Carlo fission model with a statistical likelihood analysis also presents a powerful tool for the evaluation of fission neutron data. Of particular importance is the fission spectrum, which plays a key role in determining reactor criticality. We show that our approach can be used to develop an estimate of the fission spectrum with uncertainties several times smaller than current experimental uncertainties for outgoing neutron energies up to 2 MeV.Comment: 17 pages, 20 figure

Proton-Rich Nuclear Statistical Equilibrium

Proton-rich material in a state of nuclear statistical equilibrium (NSE) is one of the least studied regimes of nucleosynthesis. One reason for this is that after hydrogen burning, stellar evolution proceeds at conditions of equal number of neutrons and protons or at a slight degree of neutron-richness. Proton-rich nucleosynthesis in stars tends to occur only when hydrogen-rich material that accretes onto a white dwarf or neutron star explodes, or when neutrino interactions in the winds from a nascent proto-neutron star or collapsar-disk drive the matter proton-rich prior to or during the nucleosynthesis. In this paper we solve the NSE equations for a range of proton-rich thermodynamic conditions. We show that cold proton-rich NSE is qualitatively different from neutron-rich NSE. Instead of being dominated by the Fe-peak nuclei with the largest binding energy per nucleon that have a proton to nucleon ratio close to the prescribed electron fraction, NSE for proton-rich material near freeze-out temperature is mainly composed of Ni56 and free protons. Previous results of nuclear reaction network calculations rely on this non-intuitive high proton abundance, which this paper will explain. We show how the differences and especially the large fraction of free protons arises from the minimization of the free energy as a result of a delicate competition between the entropy and the nuclear binding energy.Comment: 4 pages, 7 figure

The Ultraviolet flash accompanying GRBs from neutron-rich internal shocks

In the neutron-rich internal shocks model for Gamma-ray Burts (GRBs), the Lorentz factors (LFs) of ions shells are variable, so are the LFs of accompanying neutron shells. For slow neutron shells with a typical LF tens, the typical beta-decay radius reads R_{\beta,s} several 10^{14} cm, which is much larger than the typical internal shocks radius 10^{13} cm, so their impact on the internal shocks may be unimportant. However, as GRBs last long enough (T_{90}>20(1+z) s), one earlier but slower ejected neutron shell will be swept successively by later ejected ion shells in the range 10^{13}-10^{15} cm, where slow neutrons have decayed significantly. We show in this work that ion shells interacting with the beta-decay products of slow neutron shells can power a ultraviolet (UV) flash bright to 12th magnitude during the prompt gamma-ray emission phase or slightly delayed, which can be detected by the upcoming Satellite SWIFT in the near future.Comment: 6 pages (2 eps figures), accepted for publication in ApJ

Initial Design Calculations for a Detection System that will Observe Resonant Excitation of the 680 keV state in 238U

We present calculations and design considerations for a detection system that could be used to observe nuclear resonance fluorescence in {sup 238}U. This is intended as part of an experiment in which a nearly monochromatic beam of light incident on a thin foil of natural uranium resonantly populates the state at 680 keV in {sup 238}U. The beam of light is generated via Compton upscattering of laser light incident on a beam of relativistic electrons. This light source has excellent energy and angular resolution. In the current design study we suppose photons emitted following de-excitation of excited nuclei to be observed by a segmented array of BGO crystals. Monte Carlo calculations are used to inform estimates for the design and performance of this detector system. We find that each detector in this array should be shielded by about 2 cm of lead. The signal to background ratio for each of the BGO crystals is larger than ten. The probability that a single detector observes a resonant photon during a single pulse of the light source is near unity

Estimate of the 9Be(n,el) Cross-section Uncertainties for the ENDL99 and ENDF/B-VII Evaluations

Uncertainties for the ENDL99 and ENDF/B-VII evaluations of the {sup 9}Be (n, el) cross section have been estimated for incident neutron energies up to 20 MeV. The uncertainties were obtained by extracting the spread of the experimental data about the evaluations, using a sophisticated procedure to ensure smoothness of the uncertainty as a function of energy. The technique used to obtain the uncertainties is described briefly in this report, and the resulting error bands are given for the two evaluations

On the Use of Rossi Alpha Critical Assembly Measurements for Validating and Constraining Nuclear Data

Critical assemblies are exquisitely sensitive to details of the microscopic nuclear reactions that govern neutron multiplication. For this reason experimental studies of critical assemblies represent a cornerstone in the process of validating nuclear data. Several different characteristics of a critical system can be measured. The most commonly considered is the so-called effective k eigenvalue, k{sub eff}. Another well-measured property of these systems is {alpha}{sub 0}, the inverse e-folding time of the neutron population in the absence of {beta}-delayed neutrons. Through Monte Carlo calculations and appear to perturbation theory they show that for fast critical systems {alpha}{sub 0} and k{sub eff} can be viewed as lying on a single straight line for any reasonable assumptions about the underlying nuclear data. This means that the two quantities provide the same constraint on nuclear data. In principle, {alpha}{sub 0} could be associated with a very small uncertainty, and this would make the measurements for neutron multiplication rates more useful than k{sub eff} for constraining nuclear data. In practice, though, uncertainties in k{sub eff} and {alpha}{sub 0} are dominated by uncertainties in the representation of the critical system, and not by pure measurement errors for these quantities. This, together with the linear relation between {alpha}{sub 0} and k{sub eff}, implies that the two measured quantities provide exactly the same constraint on nuclear data. They do not consider other measured or inferred characteristics of critical assemblies, such as neutron generation times or spectral indices, that may be valuable in the validation process

Photon Production through Multi-step Processes Important in Nuclear Fluorescence Experiments

The authors present calculations describing the production of photons through multi-step processes occurring when a beam of gamma rays interacts with a macroscopic material. These processes involve the creation of energetic electrons through Compton scattering, photo-absorption and pair production, the subsequent scattering of these electrons, and the creation of energetic photons occurring as these electrons are slowed through Bremsstrahlung emission. Unlike single Compton collisions, during which an energetic photon that is scattered through a large angle loses most of its energy, these multi-step processes result in a sizable flux of energetic photons traveling at large angles relative to an incident photon beam. These multi-step processes are also a key background in experiments that measure nuclear resonance fluorescence by shining photons on a thin foil and observing the spectrum of back-scattered photons. Effective cross sections describing the production of backscattered photons are presented in a tabular form that allows simple estimates of backgrounds expected in a variety of experiments. Incident photons with energies between 0.5 MeV and 8 MeV are considered. These calculations of effective cross sections may be useful for those designing NRF experiments or systems that detect specific isotopes in well-shielded environments through observation of resonance fluorescence

Contraband Detection with Nuclear Resonance Fluorescence: Feasibility and Impact

In this report they show that cargo interrogation systems developed to thwart trafficking of illicit nuclear materials could also be powerful tools in the larger fight against contraband smuggling. In particular, in addition to detecting special nuclear materials, cargo scanning systems that exploit nuclear resonance fluorescence to detect specific isotopes can be used to help find: chemical weapons; some drugs as well as some chemicals regulated under the controlled substances act; precious metals; materials regulated under export control laws; and commonly trafficked fluorocarbons

The difficulty in using orphan afterglows to measure gamma-ray burst beaming

If gamma-ray burst (GRB) emission is strongly collimated then GRBs occur throughout the Universe at a rate much higher than is detected. Since the emission from the optical afterglow is thought to be more isotropic than the gamma-ray emission, it has been hypothesized that a search for orphan afterglows (those without the triggering GRB) would allow strong constraints to be placed on the degree of GRB collimation. We show here that, within the context of leading models of GRB jet evolution, measurement of the GRB beaming angle using optical orphan searches is extremely difficult, perhaps impossible in practice. This is because in the leading model of GRB jets, the effective afterglow beaming angle scales with the jet angle for small angles, and so the ratio of detected orphan afterglows to GRBs is independent of the jet opening angle. Thus, the number of expected afterglow detections is the same for moderate jet angles (e.g. 20 deg) as for arbitrarily small jet angles (<< 0.1 deg). For nearly isotropic GRB geometry, or for radio afterglow searches in which the jet has become non-relativistic, the ratio of afterglows to GRBs may give information on collimation. However, using a simple model we estimate the expected number of orphan detections in current supernova surveys, and find this number to be less than one, for all jet opening angles. Even for future supernova surveys, the small detection rate and lack of dependence on collimation angle appear to ruin the prospects of determining GRB beaming by this method. Radio searches may provide the best hope to find the missing orphans.Comment: 12 pages, 3 figures, submitted to Ap

Nuclear Composition of Gamma-Ray Burst Fireballs

We study three processes that shape the nuclear composition of GRB fireballs: (1) neutronization in the central engine, (2) nucleosynthesis in the fireball as it expands and cools, and (3) spallation of nuclei in subsequent internal shocks. The fireballs are found to have a neutron excess and a marginally successful nucleosynthesis. They are composed of free nucleons, alpha-particles, and deuterium. A robust result is the survival of a significant neutron component, which has important implications. First, as shown in previous works, neutrons can lead to observable multi-GeV neutrino emission. Second, as we show in an accompanying paper, neutrons impact the explosion dynamics at radii up to 10^{17} cm and change the mechanism of the GRB afterglow emission.Comment: 33 pages, accepted to Ap