Giant enhanced optical nonlinearity of colloidal nanocrystals with a graded-index host

The effective linear and third-order nonlinear optical properties of metallic colloidal crystal immersed in a graded-index host fluid are investigated theoretically. The local electric fields are extracted self-consistently based on the layer-to-layer interactions, which are readily given by the Lekner summation method. The resultant optical absorption and nonlinearity enhancement show a series of sharp peaks, which merge in a broadened resonant band. The sharp peaks become a continuous band for increasing packing density and number of layers. We believe that the sharp peaks arise from the in-plane dipolar interactions and the surface plasmon resonance, whereas the continuous band is due to the presence of the gradient in the host refractive index. These results have not been observed in homogeneous and randomly-dispersed colloids, and thus would be of great interest in optical nanomaterial engineering.Comment: Submitted to Applied Physics Letter

Protein folding in hydrophobic-polar lattice model: a flexible ant colony optimization approach

This paper proposes a flexible ant colony (FAC) algorithm for solving protein folding problems based on the hydrophobic-polar square lattice model. Collaborations of novel pheromone and heuristic strategies in the proposed algorithm make it more effective in predicting structures of proteins compared with other state-of-the-art algorithms

Dispersion and transitions of dipolar plasmon modes in graded plasmonic waveguides

Coupled plasmon modes are studied in graded plasmonic waveguides, which are periodic chains of metallic nanoparticles embedded in a host with gradually varying refractive indices. We identify three types of localized modes called "light", "heavy", and "light-heavy" plasmonic gradons outside the passband, according to various degrees of localization. We also demonstrate new transitions among extended and localized modes when the interparticle separation $d$ is smaller than a critical $d_c$, whereas the three types of localized modes occur for $d>d_c$, with no extended modes. The transitions can be explained with phase diagrams constructed for the lossless metallic systems.Comment: Preliminary results have been presented at ETOPIM 7. Submitted to Appl. Phys. Let