19 research outputs found
Photoinduced time-resolved electrodynamics of superconducting metals and alloys
The photoexcited state in superconducting metals and alloys was studied via
pump-probe spectroscopy. A pulsed Ti:sapphire laser was used to create the
non-equilibrium state and the far-infrared pulses of a synchrotron storage
ring, to which the laser is synchronized, measured the changes in the material
optical properties. Both the time- and frequency- dependent photoinduced
spectra of Pb, Nb, NbN, Nb{0.5}Ti{0.5}N, and Pb{0.75}Bi{0.25} superconducting
thin films were measured in the low-fluence regime. The time dependent data
establish the regions where the relaxation rate is dominated either by the
phonon escape time (phonon bottleneck effect) or by the intrinsic quasiparticle
recombination time. The photoinduced spectra measure directly the reduction of
the superconducting gap due to an excess number of quasiparticles created by
the short laser pulses. This gap shift allows us to establish the temperature
range over which the low fluence approximation is valid.Comment: 12 pages with 10 figure
Time-resolved spectroscopy using synchrotron infrared pulses
Electron synchrotron storage rings, such as the VUV ring at the National Synchrotron Light Source (NSLS), produce short pulses of infrared (IR) radiation suitable for investigating the time-dependent phenomena in a variety of interesting experimental systems. In contrast to other pulses sources of IR, the synchrotron produces a continuum spectral output over the entire IR (and beyond), though at power levels typically below those obtained from laser systems. The infrared synchrotron radiation (IRSR) source is therefore well-suited as a probe using standard FTIR spectroscopic techniques. Here the authors describe the pump-probe spectroscopy facility being established at the NSLS and demonstrate the technique by measuring the photocarrier decay in a semiconductor
Sub-nanosecond, time-resolved, broadband infrared spectroscopy using synchrotron radiation
A facility for sub-nanosecond time-resolved (pump-probe) infrared
spectroscopy has been developed at the National Synchrotron Light Source of
Brookhaven National Laboratory. A mode-locked Ti:sapphire laser produces 2 ps
duration, tunable near-IR pump pulses synchronized to probe pulses from a
synchrotron storage ring. The facility is unique on account of the broadband
infrared from the synchrotron, which allows the entire spectral range from 2
cm-1 (0.25 meV) to 20,000 cm-1 (2.5 eV) to be probed. A temporal resolution of
200 ps, limited by the infrared synchrotron-pulse duration, is achieved. A
maximum time delay of 170 ns is available without gating the infrared detector.
To illustrate the performance of the facility, a measurement of electron-hole
recombination dynamics for an HgCdTe semiconductor film in the far- and mid
infrared range is presented.Comment: 11 pages with 9 figures include
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Time resolved spectroscopy using synchrotron infrared pulses
Electron synchrotron storage rings, such as the VUV ring at the National Synchrotron Light Source (NSLS), produce short pulses of infrared (IR) radiation suitable for investigating the time-dependent phenomena in a variety of interesting experimental systems. In contrast to other pulses sources of IR, the synchrotron produces a continuum spectral output over the entire IR (and beyond), though at power levels typically below those obtained from laser systems. The infrared synchrotron radiation (IRSR) source is therefore well-suited as a probe using standard FTIR spectroscopic techniques. Here the authors describe the pump-probe spectroscopy facility being established at the NSLS and demonstrate the technique by measuring the photocarrier decay in a semiconductor
An extended area blackbody for radiometric calibration
SBIR is developing an enhanced blackbody for improved radiometric testing. The main feature of the blackbody is an improved coating with higher emissivity than the standard coating used. Comparative measurements of the standard and improved coatings are reported, including reflectance. The coatings were also tested with infrared imagers and a broadband emissivity estimate derived from the imagery data. In addition, a control algorithm for constant slew rate has been implemented, primarily for use in minimum resolvable temperature measurements. The system was tested over a range of slew rates from 0.05 K/min to 10 K/min and its performance reported
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TIME-RESOLVED INFRARED SPECTROSCOPY IN THE U121R BEAMLINE AT THE NSLS
A facility for performing time-resolved infrared spectroscopy has been developed at the NSLS, primarily at beamline U12IR. The pulsed IR light from the synchrotron is used to perform pump-probe spectroscopy. The authors present here a description of the facility and results for the relaxation of photoexcitations in both a semiconductor and superconductor
Coexisting one-dimensional and three-dimensional spectral signatures in TaTe4
Using angle-resolved photoemission spectroscopy, we probe the electronic band structure of TaTe4 single crystal samples. Resistivity and optical measurements were also performed on the same samples. The experimental data indicate a combination of quasi-one-dimensional and three-dimensional electronic properties. We observe a finite spectral intensity, but no dispersing quasiparticle states near the chemical potential. [S0163-1829(99)06611-4]
Development of a high-definition IR LED scene projector
Next-generation Infrared Focal Plane Arrays (IRFPAs) are demonstrating ever increasing frame rates, dynamic range, and format size, while moving to smaller pitch arrays.1 These improvements in IRFPA performance and array format have challenged the IRFPA test community to accurately and reliably test them in a Hardware-In-the-Loop environment utilizing Infrared Scene Projector (IRSP) systems. The rapidly-evolving IR seeker and sensor technology has, in some cases, surpassed the capabilities of existing IRSP technology. To meet the demands of future IRFPA testing, Santa Barbara Infrared Inc. is developing an Infrared Light Emitting Diode IRSP system. Design goals of the system include a peak radiance >2.0W/cm2/sr within the 3.0-5.0μm waveband, maximum frame rates >240Hz, and >4million pixels within a form factor supported by pixel pitches ≤32μm. This paper provides an overview of our current phase of development, system design considerations, and future development work