Magnetic Penetration Depth Measurements of Pr2−x_{2-x}Cex_xCuO4−δ_{4-\delta} Films on Buffered Substrates: Evidence for a Nodeless Gap

We report measurements of the inverse squared magnetic penetration depth, $\lambda^{-2}(T)$, in Pr$_{2-x}$Ce$_{x}$CuO$_{4-\delta}$ ($0.115 \leq x \leq 0.152$) superconducting films grown on SrTiO$_3$ (001) substrates coated with a buffer layer of insulating Pr$_{2}$CuO$_{4}$. $\lambda^{-2}(0)$, $T_c$ and normal-state resistivities of these films indicate that they are clean and homogeneous. Over a wide range of Ce doping, $0.124\leq x \leq 0.144$, $\lambda^{-2}(T)$ at low $T$ is flat: it changes by less than 0.15% over a factor of 3 change in $T$, indicating a gap in the superconducting density of states. Fits to the first 5% decrease in $\lambda^{-2}(T)$ produce values of the minimum superconducting gap in the range of $0.29\leq\Delta_{\rm min}/k_BT_c\leq1.01$.Comment: 4 pages 5 figure

Evidence for a Nodeless Gap from the Superfluid Density of Optimally Doped Pr_{1.855}Ce_{0.145}CuO_{4-y} Films

We present measurements of the ab-plane magnetic penetration depth, \lambda(T), in five optimally doped Pr_{1.855}Ce_{0.145}CuO_{4-y} films for 1.6 K \leq T \leq T_c \sim 24 K. Low resistivities, high superfluid densities n_s(T)\propto \lambda^{-2}(T), high T_c's, and small transition widths are reproducible and indicative of excellent film quality. For all five films, \lambda^{-2}(T)/\lambda^{-2}(0) at low T is well fitted by an exponential temperature dependence with a gap, \Delta_{min}, of 0.85 k_B T_c. This behavior is consistent with a nodeless gap and is incompatible with d-wave superconductivity.Comment: 5 pages, 4 figures, reorganized for clarit

Anisotropic Optical Conductivity of Nd2-xCexCuO4 Thin Films

Opticcal conductivity spectra $\sigma_1(\omega)$ of Nd2-xCexCuO4 thin films, measured by the reflectance-transmittance method (R-T method) which has been proposed to investigate far-infrared spectroscopy, are investigated based on the anisotropic pairing model. Precise measurements of the frequency-dependent conductivity enable us to examine quantitatively the nature of the superconducting gap through infrared properties in the electron-doped high-Tc superconductors. We show that the behavior of optical conductivity $\sigma_1$ is consistent with the anisotropic superconducting gap and is well explained by the formula for d-wave pairing in the low-energy regime of the far-infrared region. Our results suggest that the electron-doped cuprate superconductors Nd2-xCexCuO4 have nodes in the superconducting gap.Comment: 4 pages, 3 figure

Electronic States in the Antiferromagnetic Phase of Electron-Doped High-Tc Cuprates

We investigate the electronic states in the antiferromagnetic (AF) phase of electron-doped cuprates by using numerically exact diagonalization technique for a t-t'-t''-J model. When AF correlation develops with decreasing temperature, a gaplike behavior emerges in the optical conductivity. Simultaneously, the coherent motion of carriers due to the same sublattice hoppings is enhanced. We propose that the phase is characterized as an AF state with small Fermi surface around the momentum k=(\pi,0) and (0,\pi). This is a remarkable contrast to the behavior of hole-doped cuprates.Comment: RevTeX, 5 pages, 4 figures, to appear in Phys. Rev. B Brief Report

Magnetic Field Dependence of Electronic Specific Heat in Pr_{1.85} Ce_{0.15} CuO_4

The specific heat of electron-doped Pr_{1.85} Ce_{0.15} CuO_4 single crystals is reported for the temperature range 2 - 10 K and magnetic field range 0 - 10 T. A non-linear magnetic field dependence is observed for the field range 0 - 2 T. Our data supports a model with lines of nodes in the gap function of these superconductors. Theoretical calculations of the electronic specific heat for dirty d-wave, clean d-wave, and s-wave symmetries are compared to our data.Comment: 10 pages Latex and 4 eps figures, submitted to Phys. Rev.

Theory for Electron-Doped Cuprate Superconductors: d-wave symmetry order parameter

Using as a model the Hubbard Hamiltonian we determine various basic properties of electron-doped cuprate superconductors like ${Nd}_{2-x}{Ce}_{x}{CuO}_{4}$ and ${Pr}_{2-x}{Ce}_{x}{CuO}_{4}$ for a spin-fluctuation-induced pairing mechanism. Most importantly we find a narrow range of superconductivity and like for hole-doped cuprates $d_{x^{2}-y^{2}}$ - symmetry for the superconducting order parameter. The superconducting transition temperatures $T_{c}(x)$ for various electron doping concentrations $x$ are calculated to be much smaller than for hole-doped cuprates due to the different Fermi surface and a flat band well below the Fermi level. Lattice disorder may sensitively distort the symmetry $d_{x^{2}-y^{2}}$ via electron-phonon interaction

Microwave Electrodynamics of Electron-Doped Cuprate Superconductors

We report microwave cavity perturbation measurements of the temperature dependence of the penetration depth, lambda(T), and conductivity, sigma(T) of Pr_{2-x}Ce_{x}CuO_{4-delta} (PCCO) crystals, as well as parallel-plate resonator measurements of lambda(T) in PCCO thin films. Penetration depth measurements are also presented for a Nd_{2-x}Ce_{x}CuO_{4-delta} (NCCO) crystal. We find that delta-lambda(T) has a power-law behavior for T<T_c/3, and conclude that the electron-doped cuprate superconductors have nodes in the superconducting gap. Furthermore, using the surface impedance, we have derived the real part of the conductivity, sigma_1(T), below T_c and found a behavior similar to that observed in hole-doped cuprates.Comment: 4 pages, 4 figures, 1 table. Submitted to Physical Review Letters revised version: new figures, sample characteristics added to table, general clarification give

Evidence of a d to s-wave pairing symmetry transition in the electron-doped cuprate superconductor Pr2−x_{2-x}Cex_xCuO4_4

We present point contact spectroscopy (PCS) data for junctions between a normal metal and the electron doped cuprate superconductor Pr$_{2-x}$Ce$_x$CuO$_4$ (PCCO). For the underdoped compositions of this cuprate ($x \sim 0.13$) we observe a peak in the conductance-voltage characteristics of the point contact junctions. The shape and magnitude of this peak suggests the presence of Andreev bound states at the surface of underdoped PCCO which is evidence for a d-wave pairing symmetry. For overdoped PCCO ($x \sim 0.17$) the PCS data does not show any evidence of Andreev bound states at the surface suggesting an s-wave pairing symmetry.Comment: 4 pages Latex, 4 eps figures included. Submitted to Phys. Rev. Let

Nonmonotonic d_{x^2-y^2} Superconducting Order Parameter in Nd_{2-x}Ce_xCuO_4

Low energy polarized electronic Raman scattering of the electron doped superconductor Nd_1.85Ce_0.15CuO_4 (T_c=22 K) has revealed a nonmonotonic d_{x^2-y^2} superconducting order parameter. It has a maximum gap of 4.4 k_BT_c at Fermi surface intersections with antiferromagnetic Brillouin zone (the ``hot spots'') and a smaller gap of 3.3 k_BT_c at fermionic Brillouin zone boundaries. The gap enhancement in the vicinity of the ``hot spots'' emphasizes role of antiferromagnetic fluctuations and similarity in the origin of superconductivity for electron- and hole-doped cuprates.Comment: 4 pages, 4 figure

Angular dependence of the penetration depth in unconventional superconductors

We examine the Meissner state nonlinear electrodynamic effects on the field and angular dependence of the low temperature penetration depth, $\lambda$, of superconductors in several kinds of unconventional pairing states, with nodes or deep minima (``quasinodes'') in the energy gap. Our calculations are prompted by the fact that, for typical unconventional superconducting material parameters, the predicted size of these effects for $\lambda$ exceeds the available experimental precision for this quantity by a much larger factor than for others. We obtain expressions for the nonlinear component of the penetration depth, $\Delta\lambda$, for different two- and three- dimensional nodal or quasinodal structures. Each case has a characteristic signature as to its dependence on the size and orientation of the applied magnetic field. This shows that $\Delta\lambda$ measurements can be used to elucidate the nodal or quasinodal structure of the energy gap. For nodal lines we find that $\Delta\lambda$ is linear in the applied field, while the dependence is quadratic for point nodes. For layered materials with $\rm{YBa_2Cu_3O_{7-\delta}}$ (YBCO) type anisotropy, our results for the angular dependence of $\Delta\lambda$ differ greatly from those for tetragonal materials and are in agreement with experiment. For the two- and three- dimensional quasinodal cases, $\Delta\lambda$ is no longer proportional to a power of the field and the field and angular dependences are not separable, with a suppression of the overall signal as the node is filled in.Comment: 16 pages plus nine figure