High Order Coherent Control Sequences of Finite-Width Pulses

The performance of sequences of designed pulses of finite length $\tau$ is analyzed for a bath of spins and it is compared with that of sequences of ideal, instantaneous pulses. The degree of the design of the pulse strongly affects the performance of the sequences. Non-equidistant, adapted sequences of pulses, which equal instantaneous ones up to $\mathcal{O}(\tau^3)$, outperform equidistant or concatenated sequences. Moreover, they do so at low energy cost which grows only logarithmically with the number of pulses, in contrast to standard pulses with linear growth.Comment: 6 pages, 5 figures, new figures, published versio

Optimized Dynamical Decoupling for Time Dependent Hamiltonians

The validity of optimized dynamical decoupling (DD) is extended to analytically time dependent Hamiltonians. As long as an expansion in time is possible the time dependence of the initial Hamiltonian does not affect the efficiency of optimized dynamical decoupling (UDD, Uhrig DD). This extension provides the analytic basis for (i) applying UDD to effective Hamiltonians in time dependent reference frames, for instance in the interaction picture of fast modes and for (ii) its application in hierarchical DD schemes with $\pi$ pulses about two perpendicular axes in spin space. to suppress general decoherence, i.e., longitudinal relaxation and dephasing.Comment: 5 pages, no figure

Magnetic Properties of (VO)_2P_2O_7 from Frustrated Interchain Coupling

Neutron-scattering experiments on (VO)_2P_2O_7 reveal both a gapped magnon dispersion and an unexpected, low-lying second mode. The proximity and intensity of these modes suggest a frustrated coupling between the alternating spin chains. We deduce the minimal model containing such a frustration, and show that it gives an excellent account of the magnon dispersion, static susceptibility and electron spin resonance absorption. We consider two-magnon states which bind due to frustration, and demonstrate that these may provide a consistent explanation for the second mode.Comment: RevTeX, 5 pages, 6 figures, compressed from first versio

Excitations in one-dimensional S=1/2 quantum antiferromagnets

The transition from dimerized to uniform phases is studied in terms of spectral weights for spin chains using continuous unitary transformations (CUTs). The spectral weights in the S=1 channel are computed perturbatively around the limit of strong dimerization. We find that the spectral weight is concentrated mainly in the subspaces with a small number of elementary triplets (triplons), even for vanishing dimerization. So, besides spinons, triplons may be used as elementary excitations in spin chains. We conclude that there is no necessity to use fractional excitations in low-dimensional, undoped or doped quantum antiferromagnets.Comment: 4 pages, 1 figure include

Exchange-Only Dynamical Decoupling in the 3-Qubit Decoherence Free Subsystem

The Uhrig dynamical decoupling sequence achieves high-order decoupling of a single system qubit from its dephasing bath through the use of bang-bang Pauli pulses at appropriately timed intervals. High-order decoupling of single and multiple qubit systems from baths causing both dephasing and relaxation can also be achieved through the nested application of Uhrig sequences, again using single-qubit Pauli pulses. For the 3-qubit decoherence free subsystem (DFS) and related subsystem encodings, Pauli pulses are not naturally available operations; instead, exchange interactions provide all required encoded operations. Here we demonstrate that exchange interactions alone can achieve high-order decoupling against general noise in the 3-qubit DFS. We present decoupling sequences for a 3-qubit DFS coupled to classical and quantum baths and evaluate the performance of the sequences through numerical simulations

On the dynamics of coupled S=1/2 antiferromagnetic zig-zag chains

We investigate the elementary excitations of quasi one-dimensional S=1/2 systems built up from zig-zag chains with general isotropic exchange constants, using exact (Lanczos) diagonalization for 24 spins and series expansions starting from the decoupled dimer limit. For the ideal one-dimensional zig-zag chain we discuss the systematic variation of the basic (magnon) triplet excitation with general exchange parameters and in particular the presence of practically flat dispersions in certain regions of phase space. We extend the dimer expansion in order to include the effects of 3D interactions on the spectra of weakly interacting zig-zag chains. In an application to KCuCl_3 we show that this approach allows to determine the exchange interactions between individual pairs of spins from the spectra as determined in recent neutron scattering experiments.Comment: 8 pages, 9 figures; some changes, figure added; final versio

Doping dependence of spin excitations in the stripe phase of high-Tc superconductors

Based on the time-dependent Gutzwiller approximation for the extended Hubbard model we calculate the energy and momentum dependence of spin excitations for striped ground states. Our starting point correctly reproduces the observed doping dependence of the incommensurability in La-based cuprates and the dispersion of magnetic modes in the insulating parent compound. This allows us to make quantitative predictions for the doping evolution of the dispersion of magnetic modes in the stripe phase including the energy and intensity of the resonance peak as well as the velocity of the spin-wave like Goldstone mode. In the underdoped regime $n_h<1/8$ we find a weak linear dependence of $\omega_{res}$ on doping whereas the resonance energy significantly shifts to higher values when the charge concentration in the stripes starts to deviate from half-filling for $n_h>1/8$. The velocity $c$ is non-monotonous with a minimum at 1/8 in coincidence with a well known anomaly in $T_c$. Our calculations are in good agreement with available experimental data. We also compare our results with analogous computations based on linear spin-wave theory.Comment: 18 pages, 14 figures, revised and extended versio

Phenomenological theory of spin excitations in La- and Y-based cuprates

Motivated by recent inelastic neutron scattering (INS) experiments on La-based cuprates and based on the fermiology theories, we study the spin susceptibility for La-based (e.g., La$_{2-x}$Sr$_x$CuO$_4$) and Y-based (e.g., YBa$_2$Cu$_3$O$_y$) cuprates, respectively. The spin excitation in YBa$_2$Cu$_3$O$_y$ is dominated by a sharp resonance peak at the frequency 40 meV in the superconducting state. Below and above the resonance frequency, the incommensurate (IC) peaks develop and the intensity of the peaks decreases dramatically. In the normal state, the resonant excitation does not occur and the IC peaks are merged into commensurate ones. The spin excitation of La$_{2-x}$Sr$_x$CuO$_4$ is significantly different from that of Y-based ones, namely, the resonance peak does not exist due to the decreasing of the superconducting gap and the presence of the possible spin-stripe order. The spectra are only enhanced at the expected resonance frequency (about 18 meV) while it is still incommensurate. On the other hand, another frequency scale at the frequency 55 meV is also revealed, namely the spectra are commensurate and local maximum at this frequency. We elaborate all the results based on the Fermi surface topology and the d-wave superconductivity, and suggest that the spin-stripe order be also important in determining the spin excitation of La-based cuprates. A coherent picture for the spin excitations is presented for Y-based and La-based cuprates.Comment: 8 pages, 8 figure

Microscopic model for Bose-Einstein condensation and quasiparticle decay

Sufficiently dimerized quantum antiferromagnets display elementary S=1 excitations, triplon quasiparticles, protected by a gap at low energies. At higher energies, the triplons may decay into two or more triplons. A strong enough magnetic field induces Bose-Einstein condensation of triplons. For both phenomena the compound IPA-CuCl3 is an excellent model system. Nevertheless no quantitative model was determined so far despite numerous studies. Recent theoretical progress allows us to analyse data of inelastic neutron scattering (INS) and of magnetic susceptibility to determine the four magnetic couplings J1=-2.3meV, J2=1.2meV, J3=2.9meV and J4=-0.3meV. These couplings determine IPA-CuCl3 as system of coupled asymmetric S=1/2 Heisenberg ladders quantitatively. The magnetic field dependence of the lowest modes in the condensed phase as well as the temperature dependence of the gap without magnetic field corroborate this microscopic model.Comment: 6 pages, 5 figure

Efficient Coherent Control by Optimized Sequences of Pulses of Finite Duration

Reliable long-time storage of arbitrary quantum states is a key element for quantum information processing. In order to dynamically decouple a spin or quantum bit from a dephasing environment, we introduce an optimized sequence of $N$ control pulses of finite durations \tau\pp and finite amplitudes. The properties of this sequence of length $T$ stem from a mathematically rigorous derivation. Corrections occur only in order $T^{N+1}$ and \tau\pp^3 without mixed terms such as T^N\tau\pp or T^N\tau\pp^2. Based on existing experiments, a concrete setup for the verification of the properties of the advocated realistic sequence is proposed.Comment: 8 pages, 1 figur