953 research outputs found
c-axis Raman Scattering in MgB2: Observation of a Dirty-Limit Gap in the pi-bands
Raman scattering spectra from the ac-face of thick MgB2 single crystals were
measured in zz, xz and xx polarisations. In zz and xz polarisations a threshold
at around 29 cm^{-1} forms in the below Tc continuum but no pair-breaking peak
is seen, in contrast to the sharp pair-breaking peak at around 100 cm^{-1} seen
in xx polarisation. The zz and xz spectra are consistent with Raman scattering
from a dirty superconductor while the sharp peak in the xx spectra argues for a
clean system. Analysis of the spectra resolves this contradiction, placing the
larger and smaller gap magnitudes in the sigma and pi bands, and indicating
that relatively strong impurity scattering is restricted to the pi bands.Comment: Revised manuscript accepted for publication in Physical Review
Letter
Carbon-substitution effect on the electronic properties of MgB single crystals
The electronic properties of the carbon substituted MgB single crystals
are reported. The carbon substitution drops T below 2 K. In-plane
resistivity shows a remarkable increase in residual resistivity by
C-substitution, while the change of in-plane/out-of-plane Hall coefficients is
rather small. Raman scattering spectra indicate that the E-phonon
frequency radically hardens with increasing the carbon-content, suggesting the
weakening of electron-phonon coupling. Another striking C-effect is the
increases of the second critical fields in both in-plane and out-of-plane
directions, accompanied by a reduction in the anisotropy ratio. The possible
changes in the electronic state and the origin of T-suppression by
C-substitution are discussed.Comment: 6 pages, 8 figure
Signature of Carrier-Induced Ferromagnetism in Ti_{1-x}Co_{x}O_{2-delta}: Exchange Interaction Between High-Spin Co 2+ and the Ti 3d Conduction Band
X-ray photoemission spectroscopy measurements were performed on thin-film
samples of rutile Ti_{1-x}Co_{x}O_{2-delta} to reveal the electronic structure.
The Co 2p core level spectra indicate that the Co ions take the high-spin Co 2+
configuration, consistent with substitution on the Ti site. The high spin state
and the shift due to the exchange splitting of the conduction band suggest
strong hybridization between carriers in the Ti 3d t2g band and the t2g states
of the high-spin Co 2+. These observations support the argument that room
temperature ferromagnetism in Ti_{1-x}Co_{x}O_{2-delta} is intrinsic.Comment: 4 pages, 5 figures. Accepted for publication in Physical Review
Letter
Flux flow resistivity in the two-gap superconductivity
We investigate the flux flow state in a two-gap superconductor in which two
s-wave gaps with different amplitudes exist on two separate Fermi surfaces. The
flux flow resistivity is obtained on the basis of the Bardeen-Stephen relation
and the result agrees well with the anomalous field dependence of the flow
resistivity recently observed in the two-gap superconductor MgB2. Some typical
properties of the vortex in this system are also discussed.Comment: 5 pages, 1 figure. Some typos are corrected. Some comments are added.
To be published in J. Phys. Soc. Jp
Evidence for High-frequency Phonon Mediated S-wave Superconductivity : 11B-NMR Study of Al-doped MgB2
We report B-NMR study on Al-doped MgB that addresses a possible
mechanism for a high superconducting (SC) transition temperature () of
K in recently discovered MgB. The result of nuclear spin lattice
relaxation rate in the SC state revealed that the size in the SC gap is
not changed by substituting Al for Mg. The reduction on by Al-doping is
shown to be due to the decrease of . According to the McMillan
equation, the experimental relation between and the relative change in
allowed us to estimate a characteristic phonon frequency K and an electron-phonon coupling constant . These
results suggest that the high- superconductivity in MgB is mediated by
the strong electron-phonon coupling with high-frequency phonons.Comment: 6pages, 3figure
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Disorder induced collapse of the electron phonon coupling in MgB observed by Raman Spectroscopy
The Raman spectrum of the superconductor MgB has been measured as a
function of the Tc of the film. A striking correlation is observed between the
onset and the frequency of the mode. Analysis of the data with
the McMillan formula provides clear experimental evidence for the collapse of
the electron phonon coupling at the temperature predicted for the convergence
of two superconducting gaps into one observable gap. This gives indirect
evidence of the convergence of the two gaps and direct evidence of a transition
to an isotropic state at 19 K. The value of the electron phonon coupling
constant is found to be 1.22 for films with T 39K and 0.80 for films with
T19K.Comment: 5 pages, 4 figure
Mixed state properties of superconducting MgB2 single crystals
We report on measurements of the magnetic moment in superconducting MgB2
single crystals. We find \mu_0H_{c2}^c(0) = 3.2 T, \mu_0H_{c2}^{ab}(0) = 14.5
T, \gamma = 4.6, \mu_0H_c(0) = 0.28 T, and \kappa(T_c) = 4.7. The standard
Ginzburg-Landau and London model relations lead to a consistent data set and
indicate that MgB2 is a clean limit superconductor of intermediate coupling
strength with very pronounced anisotropy effects
Temperature-dependent Raman spectroscopy in BaRuO systems
We investigated the temperature-dependence of the Raman spectra of a
nine-layer BaRuO single crystal and a four-layer BaRuO epitaxial film,
which show pseudogap formations in their metallic states. From the polarized
and depolarized spectra, the observed phonon modes are assigned properly
according to the predictions of group theory analysis. In both compounds, with
decreasing temperature, while modes show a strong hardening, (or
) modes experience a softening or no significant shift. Their different
temperature-dependent behaviors could be related to a direct Ru metal-bonding
through the face-sharing of RuO. It is also observed that another
mode of the oxygen participating in the face-sharing becomes split at low
temperatures in the four layer BaRuO. And, the temperature-dependence of
the Raman continua between 250 600 cm is strongly correlated to
the square of the plasma frequency. Our observations imply that there should be
a structural instability in the face-shared structure, which could be closely
related to the pseudogap formation of BaRuO systems.Comment: 8 pages, 6 figures. to be published in Phys. Rev.
Extreme Electron-Phonon Coupling in Boron-based Layered Superconductors
The phonon-mode decomposition of the electron-phonon coupling in the
MgB2-like system Li_{1-x}BC is explored using first principles calculations. It
is found that the high temperature superconductivity of such systems results
from extremely strong coupling to only ~2% of the phonon modes. Novel
characteristics of E_2g branches include (1) ``mode lambda'' values of 25 and
greater compared to a mean of for other modes, (2) a precipitous
Kohn anomaly, and (3) E_2g phonon linewidths within a factor of ~2 of the
frequency itself, indicating impending breakdown of linear electron-phonon
theory. This behavior in borne out by recent inelastic x-ray scattering studies
of MgB2 by Shukla et al.Comment: 4 two-column pages, 4 figures. Equations simplified. Figure 4
changed. Comparison with new data include
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