Stripe charge ordering in SrO-terminated SrTiO3(001) surfaces

The local electronic structure of the SrO-terminated SrTiO3(001) surface was explored using scanning tunneling microscopy. At low bias voltages in the empty states, a unidirectional structure with a periodicity of 3 unit cells, superimposed on a c(2 x 2) reconstructed structure, was found to develop along the crystallographic a axis. This structure indicates a charge-ordered stripe induced by carrier doping from oxygen vacancies in the SrO and the subsurface TiO2 planes. In the filled states, localized deep in-gap states were observed in addition to large energy gaps in the tunneling spectra. This result represents inelastic tunneling due to significant electron-lattice interaction associated with unidirectional lattice distortion in the SrO-terminated surface.Comment: 6 pages, 5 figures, accepted for publication in PR

Ontogenetic changes of the water status and accumulated soluble compounds in developing and ripening mume (Prunus mume) fruit measured by 1H-NMR analysis

The physiological changes of intact mume (Prunus mume Sieb. et Zucc. cv. Rinshu) fruit tissues were examined by measuring the physical states of cell-associated water in the fruit tissues with developing and ripening using 1H-NMR spectroscopy. We found that the water molecules in mume fruit tissues existed in several different compartments with different mobilities. Additionally, spectral recovery in the water proton indicated reverse relationships between the pericarps and seeds at the immature and mature stages. In the pericarp tissues, the longest T1 and longer T2 markedly increased, while those in the seeds decreased. From these results, the change in the water status with growth stage had reverse trajectories in the pericarp and seed of the fruit. In the pericarp tissues, both water uptake and dry weight prominently increased with ripening. The epidermis and inner parenchymal cells of the pericarp tissues remarkably enlarged as a sigmoidal growth curve. Membrane permeability, indicating a loss of membrane integrity, increased in the pericarp tissues. The elongation in the fully vacuolated cells and changes in the membrane permeability in the pericarp tissues with ripening correlated to the longest T1. In contrast, the high mobility of water in the seeds began to decrease with maturation, while oil began to accumulate. Thus, the mobility of water, as analyzed in this study, is considered to reflect the results of physiological changes such as cellular heterogeneity and spatial arrangements both in the pericarp and in seed tissues for mume fruit with development and ripening

Single-Cell Multiomics Decodes Regulatory Programs for Mouse Secondary Palate Development

Perturbations in gene regulation during palatogenesis can lead to cleft palate, which is among the most common congenital birth defects. Here, we perform single-cell multiome sequencing and profile chromatin accessibility and gene expression simultaneously within the same cells (n = 36,154) isolated from mouse secondary palate across embryonic days (E) 12.5, E13.5, E14.0, and E14.5. We construct five trajectories representing continuous differentiation of cranial neural crest-derived multipotent cells into distinct lineages. By linking open chromatin signals to gene expression changes, we characterize the underlying lineage-determining transcription factors. In silico perturbation analysis identifies transcription factors SHOX2 and MEOX2 as important regulators of the development of the anterior and posterior palate, respectively. In conclusion, our study charts epigenetic and transcriptional dynamics in palatogenesis, serving as a valuable resource for further cleft palate research

Atomic-scale visualization of initial growth of homoepitaxial SrTiO3 thin film on an atomically ordered substrate

The initial homoepitaxial growth of SrTiO3 on a (\surd13\times\surd13) - R33.7{\deg}SrTiO3(001) substrate surface, which can be prepared under oxide growth conditions, is atomically resolved by scanning tunneling microscopy. The identical (\surd13\times\surd13) atomic structure is clearly visualized on the deposited SrTiO3 film surface as well as on the substrate. This result indicates the transfer of the topmost Ti-rich (\surd13\times\surd13) structure to the film surface and atomic-scale coherent epitaxy at the film/substrate interface. Such atomically ordered SrTiO3 substrates can be applied to the fabrication of atom-by-atom controlled oxide epitaxial films and heterostructures

Real space imaging of the metal - insulator phase separation in the band width controlled organic Mott system κ\kappa-(BEDT-TTF)2_{2}Cu[N(CN)2_{2}]Br

Systematic investigation of the electronic phase separation on macroscopic scale is reported in the organic Mott system $\kappa$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]Br. Real space imaging of the phase separation is obtained by means of scanning micro-region infrared spectroscopy using the synchrotron radiation. The phase separation appears near the Mott boundary and changes its metal-insulator fraction with the substitution ratio $x$ in $\kappa$-[($h$-BEDT-TTF)$_{1-x}$($d$-BEDT-TTF)$_{x}$]$_{2}$Cu[N(CN)$_{2}$]Br, of which band width is controlled by the substitution ratio $x$ between the hydrogenated BEDT-TTF molecule ($h$-BEDT-TTF) and the deuterated one ($d$-BEDT-TTF). The phase separation phenomenon observed in this class of organics is considered on the basis of the strongly correlated electronic phase diagram with the first order Mott transition.Comment: 10 pages, 8 figure

The electronic state of vortices in YBa2Cu3Oy investigated by complex surface impedance measurement

The electromagnetic response to microwaves in the mixed state of YBa2Cu3Oy(YBCO) was measured in order to investigate the electronic state inside and outside the vortex core. The magnetic-field dependence of the complex surface impedance at low temperatures was in good agreement with a general vortex dynamics description assuming that the field-independent viscous damping force and the linear restoring force were acting on the vortices. In other words, both real and imaginary parts of the complex resistivity, \rho_1, and \rho_2, were linear in B. This is explained by theories for d-wave superconductors. Using analysis based on the Coffey-Clem description of the complex penetration depth, we estimated that the vortex viscosity \eta at 10 K was (4 \sim 5) \times 10^{-7} Ns/m^2. This value corresponds to \omega_0 \tau \sim 0.3 - 0.5, where \omega_0 and \tau are the minimal gap frequency and the quasiparticle lifetime in the vortex core, respectively. These results suggest that the vortex core in YBCO is in the moderately clean regime. Investigation of the moderately clean vortex core in high-temperature superconductors is significant because physically new effects may be expected due to d-wave characteristics and to the quantum nature of cuprate superconductors. The behavior of Z_s as a function of B across the first order transition (FOT) of the vortex lattice was also investigated. Unlike Bi2Sr2CaCu2Oy (BSCCO), no distinct anomaly was observed around the FOT in YBCO. Our results suggest that the rapid increase of X_s due to the change of superfluid density at the FOT would be observed only in highly anisotropic two-dimensional vortex systems like BSCCO. We discuss these results in terms of the difference of the interlayer coupling and the energy scale between the two materials.Comment: 10 pages, 6 figures, to be published in Phys. Rev. B, one reference adde

Direct observation of the washboard noise of a driven vortex lattice in a high-temperature superconductor, Bi2Sr2CaCu2Oy

We studied the conduction noise spectrum in the vortex state of a high-temperature superconductor, Bi2Sr2CaCu2Oy, subject to a uniform driving force. Two characteristic features, a broadband noise (BBN) and a narrow-band noise (NBN), were observed in the vortex-solid phase. The origin of the large BBN was determined to be plastic motion of the vortices, whereas the NBN was found to originate from the washboard modulation of the translational velocity of the driven vortices. We believe this to be the first observation ofComment: 4 pages, 4 figures, to appear in Phys. Rev. Let