5,061 research outputs found
Charge collective modes in an incommensurately modulated cuprate
We report the first measurement of collective charge modes of insulating
Sr14Cu24O41 using inelastic resonant x-ray scattering over the complete
Brillouin zone. Our results show that the intense excitation modes at the
charge gap edge predominantly originate from the ladder-containing planar
substructures. The observed ladder modes (E vs. Q) are found to be dispersive
for momentum transfers along the "legs" but nearly localized along the "rungs".
Dispersion and peakwidth characteristics are similar to the charge spectrum of
1D Mott insulators, and we show that our results can be understood in the
strong coupling limit (U >> t_{ladder}> t_{chain}). The observed behavior is in
marked contrast to the charge spectrum seen in most two dimensional cuprates.
Quite generally, our results also show that momentum-tunability of inelastic
scattering can be used to resolve mode contributions in multi-component
incommensurate systems.Comment: 4+ pages, 5 figure
Semimetal to semimetal charge density wave transition in 1T-TiSe
We report an infrared study on 1-TiSe, the parent compound of the
newly discovered superconductor CuTiSe. Previous studies of this
compound have not conclusively resolved whether it is a semimetal or a
semiconductor: information that is important in determining the origin of its
unconventional CDW transition. Here we present optical spectroscopy results
that clearly reveal that the compound is metallic in both the high-temperature
normal phase and the low-temperature CDW phase. The carrier scattering rate is
dramatically different in the normal and CDW phases and the carrier density is
found to change with temperature. We conclude that the observed properties can
be explained within the scenario of an Overhauser-type CDW mechanism.Comment: 4 pages, 4 page
Fermi surface topology and low-lying quasiparticle structure of magnetically ordered Fe1+xTe
We report the first photoemission study of Fe1+xTe - the host compound of the
newly discovered iron-chalcogenide superconductors. Our results reveal a pair
of nearly electron- hole compensated Fermi pockets, strong Fermi velocity
renormalization and an absence of a spin-density-wave gap. A shadow hole pocket
is observed at the "X"-point of the Brillouin zone which is consistent with a
long-range ordered magneto-structural groundstate. No signature of Fermi
surface nesting instability associated with Q= pi(1/2, 1/2) is observed. Our
results collectively reveal that the Fe1+xTe series is dramatically different
from the undoped phases of the high Tc pnictides and likely harbor unusual
mechanism for superconductivity and quantum magnetic order.Comment: 5 pages, 4 Figures; Submitted to Phys. Rev. Lett. (2009
Emergence of Fermi pockets in an excitonic CDW melted novel superconductor
A superconducting (SC) state (Tc ~ 4.2K) has very recently been observed upon
successful doping of the CDW ordered triangular lattice TiSe, with copper.
Using high resolution photoemission spectroscopy we identify, for the first
time, the momentum space locations of the doped electrons that form the Fermi
sea of the parent superconductor. With doping, we find that the kinematic
nesting volume increases whereas the coherence of the CDW order sharply drops.
In the superconducting doping, we observe the emergence of a large density of
states in the form of a narrow electron pocket near the \textit{L}-point of the
Brillouin Zone with \textit{d}-like character. The \textit{k}-space electron
distributions highlight the unconventional interplay of CDW to SC cross-over
achieved through non-magnetic copper doping.Comment: 4+ pages, 5 figures; Accepted for publication in Phys. Rev. Lett.
(2007
Anomalous metallic state of CuTiSe: an optical spectroscopy study
We report an optical spectroscopy study on the newly discovered
superconductor CuTiSe. Consistent with the development from a
semimetal or semiconductor with a very small indirect energy gap upon doping
TiSe, it is found that the compound has a low carrier density. Most
remarkably, the study reveals a substantial shift of the "screened" plasma edge
in reflectance towards high energy with decreasing temperature. This
phenomenon, rarely seen in metals, indicates either a sizeable increase of the
conducting carrier concentration or/and a decrease of the effective mass of
carriers with reducing temperature. We attribute the shift primarily to the
later effect.Comment: 4 figures, 4+ page
Complete d-Band Dispersion and the Mobile Fermion Scale in NaxCoO2
We utilize fine-tuned polarization selection coupled with excitation-energy
variation of photoelectron signal to image the \textit{complete d}-band
dispersion relation in sodium cobaltates. A hybridization gap anticrossing is
observed along the Brillouin zone corner and the full quasiparticle band is
found to emerge as a many-body entity lacking a pure orbital polarization. At
low dopings, the quasiparticle bandwidth (Fermion scale, many-body
\textit{E} 0.25 eV) is found to be smaller than most known oxide
metals. The low-lying density of states is found to be in agreement with
bulk-sensitive thermodynamic measurements for nonmagnetic dopings where the 2D
Luttinger theorem is also observed to be satisfied.Comment: 4+ pages, 5 Fig
Low-lying quasiparticle states and hidden collective charge instabilities in parent cobaltate superconductors (NaxCoO2)
We report a state-of-the-art photoemission (ARPES) study of high quality
single crystals of the NaxCoO2 series focusing on the fine details of the
low-energy states. The Fermi velocity is found to be small (< 0.5 eV.A) and
only weakly anisotropic over the Fermi surface at all dopings setting the size
of the pair wavefunction to be on the order of 10-20 nanometers. In the low
doping regime the exchange inter-layer splitting vanishes and two dimensional
collective instabilities such as 120-type fluctuations become kinematically
allowed. Our results suggest that the unusually small Fermi velocity and the
unique symmetry of kinematic instabilities distinguish cobaltates from other
unconventional oxide superconductors such as the cuprates or the ruthenates.Comment: Accepted for publication in Phys. Rev. Lett. (2006
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