Closed formula for the relative entropy of entanglement in all dimensions

The relative entropy of entanglement is defined in terms of the relative entropy between an entangled state and its closest separable state (CSS). Given a multipartite-state on the boundary of the set of separable states, we find a closed formula for all the entangled state for which this state is a CSS. Quite amazing, our formula holds for multipartite states in all dimensions. In addition we show that if an entangled state is full rank, then its CSS is unique. For the bipartite case of two qubits our formula reduce to the one given in Phys. Rev. A 78, 032310 (2008).Comment: 8 pages, 1 figure, significantly revised; theorem 1 is now providing necessary and sufficient conditions to determine if a state is CS

Atemporal diagrams for quantum circuits

A system of diagrams is introduced that allows the representation of various elements of a quantum circuit, including measurements, in a form which makes no reference to time (hence ``atemporal''). It can be used to relate quantum dynamical properties to those of entangled states (map-state duality), and suggests useful analogies, such as the inverse of an entangled ket. Diagrams clarify the role of channel kets, transition operators, dynamical operators (matrices), and Kraus rank for noisy quantum channels. Positive (semidefinite) operators are represented by diagrams with a symmetry that aids in understanding their connection with completely positive maps. The diagrams are used to analyze standard teleportation and dense coding, and for a careful study of unambiguous (conclusive) teleportation. A simple diagrammatic argument shows that a Kraus rank of 3 is impossible for a one-qubit channel modeled using a one-qubit environment in a mixed state.Comment: Minor changes in references. Latex 32 pages, 13 figures in text using PSTrick

Rate-dependent morphology of Li2O2 growth in Li-O2 batteries

Compact solid discharge products enable energy storage devices with high gravimetric and volumetric energy densities, but solid deposits on active surfaces can disturb charge transport and induce mechanical stress. In this Letter we develop a nanoscale continuum model for the growth of Li2O2 crystals in lithium-oxygen batteries with organic electrolytes, based on a theory of electrochemical non-equilibrium thermodynamics originally applied to Li-ion batteries. As in the case of lithium insertion in phase-separating LiFePO4 nanoparticles, the theory predicts a transition from complex to uniform morphologies of Li2O2 with increasing current. Discrete particle growth at low discharge rates becomes suppressed at high rates, resulting in a film of electronically insulating Li2O2 that limits cell performance. We predict that the transition between these surface growth modes occurs at current densities close to the exchange current density of the cathode reaction, consistent with experimental observations.Comment: 8 pages, 6 fig

Interplay between computable measures of entanglement and other quantum correlations

Composite quantum systems can be in generic states characterized not only by entanglement, but also by more general quantum correlations. The interplay between these two signatures of nonclassicality is still not completely understood. In this work we investigate this issue focusing on computable and observable measures of such correlations: entanglement is quantified by the negativity N, while general quantum correlations are measured by the (normalized) geometric quantum discord D_G. For two-qubit systems, we find that the geometric discord reduces to the squared negativity on pure states, while the relationship $D_G \geq N^2$ holds for arbitrary mixed states. The latter result is rigorously extended to pure, Werner and isotropic states of two-qudit systems for arbitrary d, and numerical evidence of its validity for arbitrary states of a qubit and a qutrit is provided as well. Our results establish an interesting hierarchy, that we conjecture to be universal, between two relevant and experimentally friendly nonclassicality indicators. This ties in with the intuition that general quantum correlations should at least contain and in general exceed entanglement on mixed states of composite quantum systems.Comment: 10 pages, 4 figure

Dynamic quantum clustering: a method for visual exploration of structures in data

A given set of data-points in some feature space may be associated with a Schrodinger equation whose potential is determined by the data. This is known to lead to good clustering solutions. Here we extend this approach into a full-fledged dynamical scheme using a time-dependent Schrodinger equation. Moreover, we approximate this Hamiltonian formalism by a truncated calculation within a set of Gaussian wave functions (coherent states) centered around the original points. This allows for analytic evaluation of the time evolution of all such states, opening up the possibility of exploration of relationships among data-points through observation of varying dynamical-distances among points and convergence of points into clusters. This formalism may be further supplemented by preprocessing, such as dimensional reduction through singular value decomposition or feature filtering.Comment: 15 pages, 9 figure

Quantum Nonlocal Boxes Exhibit Stronger Distillability

The hypothetical nonlocal box (\textsf{NLB}) proposed by Popescu and Rohrlich allows two spatially separated parties, Alice and Bob, to exhibit stronger than quantum correlations. If the generated correlations are weak, they can sometimes be distilled into a stronger correlation by repeated applications of the \textsf{NLB}. Motivated by the limited distillability of \textsf{NLB}s, we initiate here a study of the distillation of correlations for nonlocal boxes that output quantum states rather than classical bits (\textsf{qNLB}s). We propose a new protocol for distillation and show that it asymptotically distills a class of correlated quantum nonlocal boxes to the value $1/2 (3\sqrt{3}+1) \approx 3.098076$, whereas in contrast, the optimal non-adaptive parity protocol for classical nonlocal boxes asymptotically distills only to the value 3.0. We show that our protocol is an optimal non-adaptive protocol for 1, 2 and 3 \textsf{qNLB} copies by constructing a matching dual solution for the associated primal semidefinite program (SDP). We conclude that \textsf{qNLB}s are a stronger resource for nonlocality than \textsf{NLB}s. The main premise that develops from this conclusion is that the \textsf{NLB} model is not the strongest resource to investigate the fundamental principles that limit quantum nonlocality. As such, our work provides strong motivation to reconsider the status quo of the principles that are known to limit nonlocal correlations under the framework of \textsf{qNLB}s rather than \textsf{NLB}s.Comment: 25 pages, 7 figure

Properties of contact matrices induced by pairwise interactions in proteins

The total conformational energy is assumed to consist of pairwise interaction energies between atoms or residues, each of which is expressed as a product of a conformation-dependent function (an element of a contact matrix, C-matrix) and a sequence-dependent energy parameter (an element of a contact energy matrix, E-matrix). Such pairwise interactions in proteins force native C-matrices to be in a relationship as if the interactions are a Go-like potential [N. Go, Annu. Rev. Biophys. Bioeng. 12. 183 (1983)] for the native C-matrix, because the lowest bound of the total energy function is equal to the total energy of the native conformation interacting in a Go-like pairwise potential. This relationship between C- and E-matrices corresponds to (a) a parallel relationship between the eigenvectors of the C- and E-matrices and a linear relationship between their eigenvalues, and (b) a parallel relationship between a contact number vector and the principal eigenvectors of the C- and E-matrices; the E-matrix is expanded in a series of eigenspaces with an additional constant term, which corresponds to a threshold of contact energy that approximately separates native contacts from non-native ones. These relationships are confirmed in 182 representatives from each family of the SCOP database by examining inner products between the principal eigenvector of the C-matrix, that of the E-matrix evaluated with a statistical contact potential, and a contact number vector. In addition, the spectral representation of C- and E-matrices reveals that pairwise residue-residue interactions, which depends only on the types of interacting amino acids but not on other residues in a protein, are insufficient and other interactions including residue connectivities and steric hindrance are needed to make native structures the unique lowest energy conformations.Comment: Errata in DOI:10.1103/PhysRevE.77.051910 has been corrected in the present versio