3 research outputs found
Electrical transport properties of nanostructured ferromagnetic perovskite oxides La_0.67Ca_0.33MnO_3 and La_0.5Sr_0.5CoO_3 at low temperatures (5 K > T >0.3 K) and high magnetic field
We report a comprehensive study of the electrical and magneto-transport
properties of nanocrystals of La_0.67Ca_0.33MnO_3 (LCMO) (with size down to 15
nm) and La_0.5Sr_0.5CoO_3 (LSCO) (with size down to 35 nm) in the temperature
range 0.3 K to 5 K and magnetic fields upto 14 T. The transport,
magnetotransport and non-linear conduction (I-V curves) were analysed using the
concept of Spin Polarized Tunnelling in the presence of Coulomb blockade. The
activation energy of transport, \Delta, was used to estimate the tunnelling
distances and the inverse decay length of the tunnelling wave function (\chi)
and the height of the tunnelling barrier (\Phi_B). The magnetotransport data
were used to find out the magnetic field dependences of these tunnelling
parameters. The data taken over a large magnetic field range allowed us to
separate out the MR contributions at low temperatures arising from tunnelling
into two distinct contributions. In LCMO, at low magnetic field, the transport
and the MR are dominated by the spin polarization, while at higher magnetic
field the MR arises from the lowering of the tunnel barrier by the magnetic
field leading to an MR that does not saturate even at 14 T. In contrast, in
LSCO, which does not have substantial spin polarization, the first contribution
at low field is absent, while the second contribution related to the barrier
height persists. The idea of inter-grain tunnelling has been validated by
direct measurements of the non-linear I-V data in this temperature range and
the I-V data was found to be strongly dependent on magnetic field. We made the
important observation that a gap like feature (with magnitude ~ E_C, the
Coulomb charging energy) shows up in the conductance g(V) at low bias for the
systems with smallest nanocrystal size at lowest temperatures (T < 0.7 K). The
gap closes as the magnetic field and the temperature are increased.Comment: 13 figure