212 research outputs found
Revealing the role of electrons and phonons in the ultrafast recovery of charge density wave correlations in 1-TiSe
Using time- and angle-resolved photoemission spectroscopy with selective
near- and mid-infrared photon excitations, we investigate the femtosecond
dynamics of the charge density wave (CDW) phase in 1-TiSe, as well as
the dynamics of CDW fluctuations at 240 K. In the CDW phase, we observe the
coherent oscillation of the CDW amplitude mode. At 240 K, we single out an
ultrafast component in the recovery of the CDW correlations, which we explain
as the manifestation of electron-hole correlations. Our momentum-resolved study
of femtosecond electron dynamics supports a mechanism for the CDW phase
resulting from the cooperation between the interband Coulomb interaction, the
mechanism of excitonic insulator phase formation, and electron-phonon coupling.Comment: 9 pages, 6 figure
Understanding the complex phase diagram of uranium: the role of electron-phonon coupling
We report an experimental determination of the dispersion of the soft phonon
mode along [1,0,0] in uranium as a function of pressure. The energies of these
phonons increase rapidly, with conventional behavior found by 20 GPa, as
predicted by recent theory. New calculations demonstrate the strong pressure
(and momentum) dependence of the electron-phonon coupling, whereas the
Fermi-surface nesting is surprisingly independent of pressure. This allows a
full understanding of the complex phase diagram of uranium, and the interplay
between the charge-density wave and superconductivity
Purification and characterization of hepatic glutathione S-transferases of rhesus monkeys. A family of enzymes similar to the human hepatic glutathione S-transferases
Emergence of the nematic electronic state in FeSe
We present a comprehensive study of the evolution of the nematic electronic
structure of FeSe using high resolution angle-resolved photoemission
spectroscopy (ARPES), quantum oscillations in the normal state and
elastoresistance measurements. Our high resolution ARPES allows us to track the
Fermi surface deformation from four-fold to two-fold symmetry across the
structural transition at ~87 K which is stabilized as a result of the dramatic
splitting of bands associated with dxz and dyz character. The low temperature
Fermi surface is that a compensated metal consisting of one hole and two
electron bands and is fully determined by combining the knowledge from ARPES
and quantum oscillations. A manifestation of the nematic state is the
significant increase in the nematic susceptibility as approaching the
structural transition that we detect from our elastoresistance measurements on
FeSe. The dramatic changes in electronic structure cannot be explained by the
small lattice effects and, in the absence of magnetic fluctuations above the
structural transition, points clearly towards an electronically driven
transition in FeSe stabilized by orbital-charge ordering.Comment: Latex, 8 pages, 4 figure
Electronic anisotropies revealed by detwinned angle-resolved photo-emission spectroscopy measurements of FeSe
We report high resolution ARPES measurements of detwinned FeSe single
crystals. The application of a mechanical strain is used to promote the volume
fraction of one of the orthorhombic domains in the sample, which we estimate to
be 80 detwinned. While the full structure of the electron pockets
consisting of two crossed ellipses may be observed in the tetragonal phase at
temperatures above 90~K, we find that remarkably, only one peanut-shaped
electron pocket oriented along the longer axis contributes to the ARPES
measurement at low temperatures in the nematic phase, with the expected pocket
along being not observed. Thus the low temperature Fermi surface of FeSe as
experimentally determined by ARPES consists of one elliptical hole pocket and
one orthogonally-oriented peanut-shaped electron pocket. Our measurements
clarify the long-standing controversies over the interpretation of ARPES
measurements of FeSe
Collapse of the Mott gap and emergence of a nodal liquid in lightly doped SrIrO
Superconductivity in underdoped cuprates emerges from an unusual electronic
state characterised by nodal quasiparticles and an antinodal pseudogap. The
relation between this state and superconductivity is intensely studied but
remains controversial. The discrimination between competing theoretical models
is hindered by a lack of electronic structure data from related doped Mott
insulators. Here we report the doping evolution of the Heisenberg
antiferromagnet SrIrO, a close analogue to underdoped cuprates. We
demonstrate that metallicity emerges from a rapid collapse of the Mott gap with
doping, resulting in lens-like Fermi contours rather than disconnected Fermi
arcs as observed in cuprates. Intriguingly though, the emerging electron liquid
shows nodal quasiparticles with an antinodal pseudogap and thus bares strong
similarities with underdoped cuprates. We conclude that anisotropic pseudogaps
are a generic property of two-dimensional doped Mott insulators rather than a
unique hallmark of cuprate high-temperature superconductivity
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