16 research outputs found
Spectroscopy of vibrational modes in metal nanoshells
We study the spectrum of vibrational modes in metal nanoparticles with a
dielectric core. Vibrational modes are excited by the rapid heating of the
particle lattice that takes place after laser excitation, and can be monitored
by means of pump-probe spectroscopy as coherent oscillations of transient
optical spectra. In nanoshells, the presence of two metal surfaces results in a
substantially different energy spectrum of acoustic vibrations than for solid
particles. We calculated the energy spectrum as well as the damping of
nanoshell vibrational modes. The oscillator strength of fundamental breathing
mode is larger than that in solid nanoparticles. At the same time, in very thin
nanoshells, the fundamental mode is overdamped due to instantaneous energy
transfer to the surrounding medium
Continuum limit of amorphous elastic bodies: A finite-size study of low frequency harmonic vibrations
The approach of the elastic continuum limit in small amorphous bodies formed
by weakly polydisperse Lennard-Jones beads is investigated in a systematic
finite-size study. We show that classical continuum elasticity breaks down when
the wavelength of the sollicitation is smaller than a characteristic length of
approximately 30 molecular sizes. Due to this surprisingly large effect
ensembles containing up to N=40,000 particles have been required in two
dimensions to yield a convincing match with the classical continuum predictions
for the eigenfrequency spectrum of disk-shaped aggregates and periodic bulk
systems. The existence of an effective length scale \xi is confirmed by the
analysis of the (non-gaussian) noisy part of the low frequency vibrational
eigenmodes. Moreover, we relate it to the {\em non-affine} part of the
displacement fields under imposed elongation and shear. Similar correlations
(vortices) are indeed observed on distances up to \xi~30 particle sizes.Comment: 28 pages, 13 figures, 3 table
Photophysics of nanometer sized metal particles electron phonon coupling and coherent excitation of breathing vibrational modes
Measurement of Blood flow through Av-Fistulae by Means of Doppler Sonography in Regularly Haemodialysed Patients
Femtosecond optical investigation of electron-lattice interactions in an ensemble and a single metal nanoparticle
no abstrac
Study of the ElectronâPhonon Relaxation in Thin Metal Films Using Transient Thermoreflectance Technique
Stability, size and optical properties of silver nanoparticles prepared by laser ablation in different carrier media
Fungal biomolecules assisted biosynthesis of AuâAg alloy nanoparticles and evaluation of their catalytic property
The coalescence of supported gold nanoparticles induced by nanosecond laser irradiation
Gold nanoparticles supported on a quartz substrate are fabricated by e-beam lithography and subjected to nanosecond laser irradiation to induce coalescence. In combination with ex-situ scanning electron microscopy and optical extinction spectra, transmission is monitored in-situ to determine the characteristic coalescence time, the threshold fluence for the onset of coalescence and the produced particle morphology. Parallel molecular dynamics simulation is employed and shown to reasonably predict the coalescence time, thus explaining the experimental results