時空間反転対称な磁性体における非線形電流生成の理論的研究

京都大学新制・課程博士博士(理学)甲第22991号理博第4668号新制||理||1670(附属図書館)京都大学大学院理学研究科物理学・宇宙物理学専攻(主査)教授 柳瀬 陽一, 教授 川上 則雄, 教授 石田 憲二学位規則第4条第1項該当Doctor of ScienceKyoto UniversityDFA

Chiral photocurrent in parity-violating magnet and enhanced response in topological antiferromagnet

Rectified electric current induced by irradiating light, so-called photocurrent, is an established phenomenon in optoelectronic physics. In this paper, we present a comprehensive classification of the photocurrent response arising from the parity violation in bulk systems. We clarify the contrasting role of $\mathcal{T}$- and $\mathcal{PT}$-symmetries and consequently find a new type of photocurrent phenomena characteristic of parity-violating magnets, intrinsic Fermi surface effect and gyration current. Especially, the gyration current is induced by the circularly-polarized light and it is the counterpart of the shift current caused by the linearly-polarized light. This photocurrent adds a new functionality of materials studied in various fields of condensed matter physics such as multiferroics and spintronics. A list of materials is provided. Furthermore, we show that the gyration current is strongly enhanced by topologically nontrivial band dispersion. On the basis of the microscopic analysis of Dirac models, we demonstrate the divergent photocurrent response and elucidate the importance of tilting of Dirac cones.Comment: 28 pages, 8 figures, 4 table

Nonlinear optical responses in noncentrosymmetric superconductors

The unique nonreciprocal responses of superconductors, which stem from the Cooper pairs' quantum condensation, have been attracting attention. Recently, theories of the second-order nonlinear response in noncentrosymmetric superconductors were formulated based on the Bogoliubov-de Gennes theory. In this paper, we study the mechanism and condition for second-order optical responses of time-reversal symmetric superconductors. The numerical results show the characteristic photocurrent and second harmonic generation in the superconducting state. However, the superconductivity-induced nonlinear optical responses disappear under some conditions on pair potential. We show that the coexistence of intraband and interband pairing is necessary for the second-order superconducting optical responses. In addition, the superconducting Berry curvature factor, which is related to a component of Berry curvature in the superconducting state, is essential for the nonlinear responses. Thus, we derived the microscopic conditions where the superconducting nonlinear response appears.Comment: 21 pages and 9 figure