Photoassociation Of Ultracold Atoms

Physic

Reply to "Comment on 'Stimulated Raman adiabatic passage from an atomic to a molecular Bose-Einstein condensate'"

In the Comment by M. Mackie \textit{et al.} [arXiv: physics/0212111 v.4], the authors suggest that the molecular conversion efficiency in atom-molecule STIRAP can be improved by lowering the initial atomic density, which in turn requires longer pulse durations to maintain adiabaticity. Apart from the fact that the mean-field approximation becomes questionable at low densities, we point out that a low-density strategy with longer pulses has several problems. It generally requires higher pulse energies, and increases radiative losses. We also show that even within the approximations used in the Comment, their example leads to no efficiency improvement compared to our high-density case. In a more careful analysis including radiative losses neglected in the Comment, the proposed strategy gives almost no conversion owing to the longer pulse durations required.Comment: Accepted for publication in Phys. Rev.

Multi-channel scattering and Feshbach resonances: Effective theory, phenomenology, and many-body effects

A low energy effective theory based on a microscopic multi-channel description of the atom-atom interaction is derived for the scattering of alkali atoms in different hyperfine states. This theory describes all scattering properties, including medium effects, in terms of the singlet and triplet scattering lengths and the range of the atom-atom potential and provides a link between a microscopic description of Feshbach scattering and more phenomenological approaches. It permits the calculation of medium effects on the resonance coming from the occupation of closed channel states. The examination of such effects are demonstrated to be of particular relevance to an experimentally important Feshbach resonance for $^{40}$K atoms. We analyze a recent rethermalization rate experiment on $^{40}$K and demonstrate that a measurement of the temperature dependence of this rate can determine the magnetic moment of the Feshbach molecule. Finally, the energy dependence of the Feshbach interaction is shown to introduce a negative effective range inversely proportional to the width of the resonance. Since our theory is based on a microscopic multi-channel picture, it allows the explicit calculation of corrections to commonly used approximations such as the neglect of the effective range and the treatment of the Feshbach molecule as a point boson.Comment: 10 pages, 5 figures. Typos corrected. Accepted for PR

Bragg spectroscopy of a superfluid Bose-Hubbard gas

Bragg spectroscopy is used to measure excitations of a trapped, quantum-degenerate gas of 87Rb atoms in a 3-dimensional optical lattice. The measurements are carried out over a range of optical lattice depths in the superfluid phase of the Bose-Hubbard model. For fixed wavevector, the resonant frequency of the excitation is found to decrease with increasing lattice depth. A numerical calculation of the resonant frequencies based on Bogoliubov theory shows a less steep rate of decrease than the measurements.Comment: 11 pages, 4 figure

Linking Ultracold Polar Molecules

We predict that pairs of polar molecules can be weakly bound together in an ultracold environment, provided that a dc electric field is present. The field that links the molecules together also strongly influences the basic properties of the resulting dimer, such as its binding energy and predissociation lifetime. Because of their long-range character these dimers will be useful in disentangling cold collision dynamics of polar molecules. As an example, we estimate the microwave photoassociation yield for OH-OH cold collisions.Comment: 4 pages 2 figure

Determination of the s-wave Scattering Length of Chromium

We have measured the deca-triplet s-wave scattering length of the bosonic chromium isotopes $^{52}$Cr and $^{50}$Cr. From the time constants for cross-dimensional thermalization in atomic samples we have determined the magnitudes $|a(^{52}Cr)|=(170 \pm 39)a_0$ and $|a(^{50}Cr)|=(40 \pm 15)a_0$, where $a_0=0.053nm$. By measuring the rethermalization rate of $^{52}$Cr over a wide temperature range and comparing the temperature dependence with the effective-range theory and single-channel calculations, we have obtained strong evidence that the sign of $a(^{52}Cr)$ is positive. Rescaling our $^{52}$Cr model potential to $^{50}$Cr strongly suggests that $a(^{50}Cr)$ is positive, too.Comment: v3: corrected typo in y-axis scaling of Figs. 3 and

Manipulation of Cold Atomic Collisions by Cavity QED Effects

We show how the dynamics of collisions between cold atoms can be manipulated by a modification of spontaneous emission times. This is achieved by placing the atomic sample in a resonant optical cavity. Spontaneous emission is enhanced by a combination of multiparticle entanglement together with a higher density of modes of the modified vacuum field, in a situation akin to superradiance. A specific situation is considered and we show that this effect can be experimentally observed as a large suppression in trap-loss rates.Comment: RevTex, 2 EPS figures; scheduled for Phys. Rev. Lett. 19 Feb 01, with minor change

Coherent Atom Interactions Mediated by Dark-State Polaritons

We suggest a technique to induce effective, controllable interactions between atoms that is based on Raman scattering into an optical mode propagating with a slow group velocity. The resulting excitation corresponds to the creation of spin-flipped atomic pairs in a way that is analogous to correlated photon emission in optical parametric amplification. The technique can be used for fast generation of entangled atomic ensembles, spin squeezing and applications in quantum information processing.Comment: 4 pages, 3 figures, minor typos correcte

Rate limit for photoassociation of a Bose-Einstein condensate

We simulate numerically the photodissociation of molecules into noncondensate atom pairs that accompanies photoassociation of an atomic Bose-Einstein condensate into a molecular condensate. Such rogue photodissociation sets a limit on the achievable rate of photoassociation. Given the atom density \rho and mass m, the limit is approximately 6\hbar\rho^{2/3}/m. At low temperatures this is a more stringent restriction than the unitary limit of scattering theory.Comment: 5 pgs, 18 refs., 3 figs., submitted to Phys. Rev. Let