1,310 research outputs found
Spin Defects in Spin-Peierls Systems
We examine spin-Peierls systems in the presence of spin defects which are
introduced by replacing magnetic ions with non-magnetic ones
in . By using the action for the bosonized Hamiltonian, it
is shown directly that the antiferromagnetic state induced by the spin defects
coexists with the spin-Peierls states. Further the doping dependences of both
transition temperature of spin-Peierls state and the spin gap have been
calculated. The transition temperature of the present estimation shows good
agreement quantitatively with that observed in Cu_{1-\de} Zn_\de O_3 for the
region of the doping rate, \de<0.02.Comment: jpsj style, 11 pages, 2 figure
Critical neutron scattering study of the compositional phase transition in Mg-doped CuGeO3
Cu1-xMgxGeO3 undergoes a first-order phase transition at a critical
concentration xc between an antiferromagnetic (AF) state on dimerized lattice
(D-AF) and an AF Neel state on undistorted uniform lattice (U-AF). Previous
magnetic susceptibility measurements showed xc = 0.023 while a recent neutron
scattering study reported xc = 0.027 +- 0.001. The present critical scattering
due to antiferromagnetic fluctuations near the superlattice reflection
(0,1,1/2) unambiguously determines xc = 0.028 +- 0.001 at TN = 3.4 ~ 4 K. Also
at T = 1.3 K, the phase boundary was determined as xc = 0.028 +- 0.001 by
observation of a jump of an effective magnetic moment across xc.Comment: 8 pages,3 figures, Post Scripts, PACS numbers: 75.30.Kz, 75.40.-s,
61.12, 75.30.K. submitted to Journal of Physical Society of Japa
High-field Electron Spin Resonance of Cu_{1-x}Zn_{x}GeO_{3}
High-Field Electron Spin Resonance measurements were made on powder samples
of Cu_{1-x}Zn_{x}GeO_{3} (x=0.00, 0.01, 0.02, 0.03 and 0.05) at different
frequencies (95, 110, 190, 220, 330 and 440 GHz) at low temperatures. The
spectra of the doped samples show resonances whose positions are dependent on
Zn concentration, frequency and temperature. The analysis of intensity
variation of these lines with temperature allows us to identify them as
originating in transitions within states situated inside the Spin Peierls gap.
A qualitative explanation of the details of the spectra is possible if we
assume that these states in the gap are associated with "loose" spins created
near the Zn impurities, as recently theoreticaly predicted. A new phenomenon of
quenching of the ESR signal across the Dimerized to Incommensurate
phase-boundary is observed.Comment: 4 pages, 5 ps figures in the text, submitted to Phys. Rev. Let
Separation of the magnetic phases at the N\'{e}el point in the diluted spin-Peierls magnet CuGeO3
The impurity induced antiferromagnetic ordering of the doped spin-Peierls
magnet Cu(1-x)Mg(x)GeO(3) was studied by ESR technique. Crystals with the Mg
concentration x<4% demonstrate a coexistence of paramagnetic and
antiferromagnetic ESR modes. This coexistence indicates the separation of a
macroscopically uniform sample in the paramagnetic and antiferromagnetic
phases. In the presence of the long-range spin-Peierls order (in a sample with
x=1.71%) the volume of the antiferromagnetic phase immediately below the
N\'{e}el point T_N is much smaller than the volume of the paramagnetic phase.
In the presence of the short-range spin-Peierls order (in samples with x=2.88%,
x= 3.2%) there are comparable volumes of paramagnetic and antiferromagnetic
phases at T=T_N. The fraction of the antiferromagnetic phase increases with
lowering temperature. In the absence of the spin-Peierls dimerization (at
x=4.57%)the whole sample exhibits the transition into the antiferromagnetic
state and there is no phase separation. The phase separation is explained by
the consideration of clusters of staggered magnetization located near impurity
atoms. In this model the areas occupied by coherently correlated spins expand
with decreasing temperature and the percolation of the ordered area through a
macroscopic distance occurs.Comment: 7pages, 10 figure
Elementary excitations, exchange interaction and spin-Peierls transition in CuGeO
The microscopic description of the spin-Peierls transition in pure and doped
CuGeO_3 is developed taking into account realistic details of crystal
structure. It it shown that the presence of side-groups (here Ge) strongly
influences superexchange along Cu-O-Cu path, making it antiferromagnetic.
Nearest-neighbour and next-nearest neighbour exchange constants and
are calculated. Si doping effectively segments the CuO_2-chains
leading to or even slightly ferromagnetic. Strong
sensitivity of the exchange constants to Cu-O-Cu and (Cu-O-Cu)-Ge angles may be
responsible for the spin-Peierls transition itself (``bond-bending mechanism''
of the transition). The nature of excitations in the isolated and coupled
spin-Peierls chains is studied and it is shown that topological excitations
(solitons) play crucial role. Such solitons appear in particular in doped
systems (Cu_{1-x}Zn_xGeO_3, CuGe_{1-x}Si_xO_3) which can explain the
phase diagram.Comment: 7 pages, revtex, 7 Postscript figure
Temperature Dependence of Spin and Bond Ordering in a Spin-Peierls System
We investigate thermodynamic properties of a one-dimensional S=1/2
antiferromagnetic Heisenberg model coupled to a lattice distortion by a quantum
Monte Carlo method. In particular we study how spin and lattice dimerize as a
function of the temperature, which gives a fundamental process of the
spin-Peierls transition in higher dimensions. The degree of freedom of the
lattice is taken into account adiabatically and the thermal distribution of the
lattice distortion is obtained by the thermal bath algorithm. We find that the
dimerization develops as the temperature decreases and it converges to the
value of the dimerization of the ground state at T=0. Furthermore we find that
the coupling constants of spins fluctuate quite largly at high temperature and
there thermodynamic properties deviate from those of the uniform chain. Doping
of non-magnetic impurities causes cut of the chain into short chains with open
boundary. We investigate thermodynamic properties of open chains taking
relaxation of the lattice into consideration. We find that strong bonds locate
at the edges and a defect of the bond alternation appears in the chain with odd
number of sites, which causes enhancement of the staggered magnetic order. We
find a spreaded staggered structure which indicates that the defect moves
diffusively in the chain even at very low temperature.Comment: 7 pages, 17 figures; added comments on section 2 and 3, corrected
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Phase diagram of disordered spin-Peierls systems
We study the competition between the spin-Peierls and the antiferromagnetic
ordering in disordered quasi-one-dimensional spin systems. We obtain the
temperature vs disorder-strength phase diagram, which qualitatively agrees with
recent experiments on doped CuGeO_3.Comment: 4 pages, revtex, epsf, 2 Postscript figure
Temperature-dependent spin gap and singlet ground state in BaCuSi2O6
Bulk magnetic measurements and inelastic neutron scattering were used to
investigate the spin-singlet ground state and magnetic gap excitations in
BaCuSi2O6, a quasi-2-dimensional antiferromagnet with a bilayer structure. The
results are well described by a model based on weakly interacting
antiferromagnetic dimers. A strongly temperature-dependent dispersion in the
gap modes was found. We suggest that the observed excitations are analogous to
magneto-excitons in light rare-earth compounds, but are an intrinsic property
of a simple Heisenberg Hamiltonian for the S=1/2 magnetic bilayer.Comment: 10 pages, 4 figures, REVTeX and PS for text, PS for figures direct
download: http://papillon.phy.bnl.gov/preprints/bacusio.htm
Pressure dependence of the spin gap in BaVS_3
We carried out magnetotransport experiments under hydrostatic pressure in
order to study the nature of the metal-insulator transition in BaVS.
Scaling relations for are established and the pressure dependence
of the spin gap is determined. Our new results, in conjunction with a
re-analysis of earlier specific heat and susceptibility data, demonstrate that
the transition is weakly second order. The nature of the phase diagram in the
---- space is discussed.Comment: 5 pages, 5 figures, submitted to PRB Rap. Co
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