Experimental characterization of H ₂ /water multiphase flow in heterogeneous sandstone rock at the core scale relevant for underground hydrogen storage (UHS)

Geological porous reservoirs provide the volume capacity needed for large scale underground hydrogen storage (UHS). To effectively exploit these reservoirs for UHS, it is crucial to characterize the hydrogen transport properties inside porous rocks. In this work, for the first time in the community, we have performed H 2/water multiphase flow experiments at core scale under medical X-ray CT scanner. This has allowed us to directly image the complex transport properties of H 2 when it is injected or retracted from the porous rock. The important effective functions of capillary pressure and relative permeability are also measured, for both drainage and imbibition. The capillary pressure measurements are combined with MICP data to derive a receding contact angle for the H 2/water/sandstone rock system. The rock core sample is a heterogeneous Berea sandstone (17 cm long and 3.8 cm diameter). Our investigation reveals the interplay between gravitational, capillary, and viscous forces. More specifically, it illustrates complex displacement patterns in the rock, including gravity segregation, enhancement of spreading of H 2 due to capillary barriers, and the formation of fingers/channel during imbibition which lead to significant trapping of hydrogen. These findings shed new light on our fundamental understanding of the transport characteristics of H 2/water relevant for UHS.Petroleum Engineerin

Multiscale Finite Volume Formulation for Compositional Flows (abstract)

Geoscience & EngineeringCivil Engineering and Geoscience

Multiscale formulation for coupled flow-heat equations arising from single-phase flow in fractured geothermal reservoirs

Efficient heat exploitation strategies from geothermal systems demand for accurate and efficient simulation of coupled flow-heat equations on large-scale heterogeneous fractured formations. While the accuracy depends on honouring high-resolution discrete fractures and rock heterogeneities, specially avoiding excessive upscaled quantities, the efficiency can be maintained if scalable model-reduction computational frameworks are developed. Addressing both aspects, this work presents a multiscale formulation for geothermal reservoirs. To this end, the nonlinear time-dependent (transient) multiscale coarse-scale system is obtained, for both pressure and temperature unknowns, based on elliptic locally solved basis functions. These basis functions account for fine-scale heterogeneity and discrete fractures, leading to accurate and efficient simulation strategies. The flow-heat coupling is treated in a sequential implicit loop, where in each stage, the multiscale stage is complemented by an ILU(0) smoother stage to guarantee convergence to any desired accuracy. Numerical results are presented in 2D to systematically analyze the multiscale approximate solutions compared with the fine scale ones for many challenging cases, including the outcrop-based geological fractured field. These results show that the developed multiscale formulation casts a promising framework for the real-field enhanced geothermal formations.Petroleum Engineerin

Multiscale finite-element method for linear elastic geomechanics

The demand for accurate and efficient simulation of geomechanical effects is widely increasing in the geoscience community. High resolution characterizations of the mechanical properties of subsurface formations are essential for improving modeling predictions. Such detailed descriptions impose severe computational challenges and motivate the development of multiscale solution strategies. We propose a multiscale solution framework for the geomechanical equilibrium problem of heterogeneous porous media based on the finite-element method. After imposing a coarsescale grid on the given fine-scale problem, the coarse-scale basis functions are obtained by solving local equilibrium problems within coarse elements. These basis functions form the restriction and prolongation operators used to obtain the coarse-scale system for the displacement-vector. Then, a two-stage preconditioner that couples the multiscale system with a smoother is derived for the iterative solution of the fine-scale linear system. Various numerical experiments are presented to demonstrate accuracy and robustness of the method.Petroleum Engineerin

Multiscale simulation of inelastic creep deformation for geological rocks

Subsurface geological formations provide giant capacities for large-scale (TWh) storage of renewable energy, once this energy (e.g. from solar and wind power plants) is converted to green gases, e.g. hydrogen. The critical aspects of developing this technology to full-scale will involve estimation of storage capacity, safety, and efficiency of a subsurface formation. Geological formations are often highly heterogeneous and, when utilized for cyclic energy storage, entail complex nonlinear rock deformation physics. In this work, we present a novel computational framework to study rock deformation under cyclic loading, in presence of nonlinear time-dependent creep physics. Both classical and relaxation creep methodologies are employed to analyze the variation of the total strain in the specimen over time. Implicit time-integration scheme is employed to preserve numerical stability, due to the nonlinear process. Once the computational framework is consistently defined using finite element method on the fine scale, a multiscale strategy is developed to represent the nonlinear deformation not only at fine but also coarser scales. This is achieved by developing locally computed finite element basis functions at coarse scale. The developed multiscale method also allows for iterative error reduction to any desired level, after being paired with a fine-scale smoother. Numerical test cases are studied to investigate various aspects of the developed computational workflow, from benchmarking with experiments to analysing the impact of nonlinear deformation for a field-scale relevant environment. Results indicate the applicability of the developed multiscale method in order to employ nonlinear physics in their laboratory-based scale of relevance (i.e., fine scale), yet perform field-relevant simulations. The developed simulator is made publicly available at https://gitlab.tudelft.nl/ADMIRE_Public/mechanics.Petroleum Engineerin

Monotone multiscale finite volume method

The MultiScale Finite Volume (MSFV) method is known to produce non-monotone solutions. The causes of the non-monotone solutions are identified and connected to the local flux across the boundaries of primal coarse cells induced by the basis functions. We propose a monotone MSFV (m-MSFV) method based on a local stencil-fix that guarantees monotonicity of the coarse-scale operator, and thus, the resulting approximate fine-scale solution. Detection of non-physical transmissibility coefficients that lead to non-monotone solutions is achieved using local information only and is performed algebraically. For these ‘critical’ primal coarse-grid interfaces, a monotone local flux approximation, specifically, a Two-Point Flux Approximation (TPFA), is employed. Alternatively, a local linear boundary condition can be used for the dual basis functions to reduce the degree of non-monotonicity. The local nature of the two strategies allows for ensuring monotonicity in local sub-regions, where the non-physical transmissibility occurs. For practical applications, an adaptive approach based on normalized positive off-diagonal coarse-scale transmissibility coefficients is developed. Based on the histogram of these normalized coefficients, one can remove the large peaks by applying the proposed modifications only for a small fraction of the primal coarse grids. Though the m-MSFV approach can guarantee monotonicity of the solutions to any desired level, numerical results illustrate that employing the m-MSFV modifications only for a small fraction of the domain can significantly reduce the non-monotonicity of the conservative MSFV solutions.Geoscience & EngineeringCivil Engineering and Geoscience

Adaptive Dynamic Multilevel Simulation of Fractured Geothermal Reservoirs

An algebraic dynamic multilevel (ADM) method for fully-coupled simulation of flow and heat transport in heterogeneous fractured geothermal reservoirs is presented. Fractures are modeled explicitly using the projection-based embedded discrete method (pEDFM), which accurately represents fractures with generic conductivity values, from barriers to highly-conductive manifolds. A fully implicit scheme is used to obtain the coupled discrete system including mass and energy balance equations with two main unknowns (i.e., pressure and temperature) at fine-scale level. The ADM method is then developed to map the fine-scale discrete system to a dynamic multilevel coarse grid, independently for matrix and fractures. To obtain the ADM map, multilevel multiscale coarse grids are constructed for matrix as well as for each fracture at all coarsening levels. On this hierarchical nested grids, multilevel multiscale basis functions (for flow and heat) are solved locally at the beginning of the simulation. They are used during the ADM simulation to allow for accurate multilevel systems in presence of parameter heterogeneity. The resolution of ADM simulations is defined dynamically based on the solution gradient (i.e. front tracking technique) using a user-defined threshold. The ADM mapping occurs algebraically using the so-called ADM prolongation and restriction operators, for all unknowns. A variety of 2D and 3D fractured test cases with homogeneous and heterogeneous permeability maps are studied. It is shown that ADM is able to model the coupled mass-heat transport accurately by employing only a fraction of fine-scale grid cells. Therefore, it promises an efficient approach for simulation of large and real-field scale fractured geothermal reservoirs. All software developments of this paper is publicly available at https://gitlab.com/DARSim2simulator.Numerical AnalysisPetroleum Engineerin

A stabilized mixed-FE scheme for frictional contact and shear failure analyses in deformable fractured media

Simulation of fracture contact mechanics in deformable fractured media is of paramount important in computational mechanics. Previous studies have revealed that compressive loading may produce mode II fractures, which is quite different from mode I fractures induced by tensile loading. Furthermore, fractures can cross each other. This will increase the complexity of their network deformation under different loading types significantly. In this work, a stabilized mixed-finite element (FE) scheme with Lagrange multipliers is proposed in the framework of variational formulation, which is able to simulate frictional contact, shear failure (mode II) and opening (mode I) of multiple crossing fractures. A novel treatment is devised to guarantee physical solutions at the intersection of crossing fractures. A preconditioner is introduced to re-scale the saddle-point algebraic system and to preserve the numerical robustness. Then, a solution strategy is designed to calculate the unknowns, displacement and Lagrange multipliers, in one algebraic system. Later, numerical tests are conducted to study mechanical behaviors of fractured media. Benchmark study is performed to verify the presented mixed-FE scheme. A deformable medium with crossing fractures is simulated under mixed-mode loading types. The characteristics of fracture contact, surface sliding, opening and variation of stress intensity factor are analyzed. Simulation results show that the curve of slippage induced by compression, as well as the opening induced by internal fluid pressure, along the fracture length holds a parabolic shape. The diagonal contact point, at the intersecting position of the crossing fractures, is studied in detail, specially under different stress states. Finally, the impact of intersecting fractures on frictional contact mechanics is investigated for different loading conditions.Numerical AnalysisDelft Institute of Applied MathematicsPetroleum Engineerin

Monotone Multiscale Finite Volume Method for Flow in Heterogeneous Porous Media

The MultiScale Finite-Volume (MSFV) method is known to produce non-monotone solutions. The causes of the non-monotone solutions are identified and connected to the local flux across the boundaries of primal coarse cells induced by the basis functions. We propose a monotone MSFV (m-MSFV) method based on a local stencil-fix that guarantees monotonicity of the coarse-scale operator, and thus the resulting approximate fine-scale solution. Detection of non-physical transmissibility coefficients that lead to non-monotone solutions is achieved using local information only and is performed algebraically. For these 'critical' primal coarse-grid interfaces, a monotone local flux approximation, specifically, a Two- Point Flux Approximation (TPFA), is employed. Alternatively, a local linear boundary condition is used for the basis functions to reduce the degree of non-monotonicity. The local nature of the two strategies allows for ensuring monotonicity in local sub-regions, where the non-physical transmissibility occurs. For practical applications, an adaptive approach based on normalized positive off-diagonal coarse-scale transmissibility coefficients is developed. Based on the histogram of these normalized coefficients, one can remove the large peaks by applying the proposed modifications only for a small fraction of the primal coarse grids. Though the m-MSFV approach can guarantee monotonicity of the solutions to any desired level, numerical results illustrate that employing the m-MSFV modifications only for a small fraction of the domain can significantly reduce the non-monotonicity of the conservative MSFV solutions.Geoscience & EngineeringCivil Engineering and Geoscience

CO_2 Storage in deep saline aquifers: impacts of fractures on hydrodynamic trapping

Natural or induced fractures are typically present in subsurface geological formations. Therefore, they need to be carefully studied for reliable estimation of the long-term carbon dioxide storage. Instinctively, flow-conductive fractures may undermine storage security as they increase the risk of CO2 leakage if they intersect the CO2 plume. In addition, fractures may act as flow barriers, causing significant pressure gradients over relatively small regions near fractures. Nevertheless, despite their high sensitivities, the impact of fractures on the full-cycle storage process has not been fully quantified and understood. In this study, a numerical model is developed and applied to analyze the role of discrete fractures on the flow and transport mechanism of CO2 plumes in simple and complex fracture geometries. A unified framework is developed to model the essential hydrogeological trapping mechanisms. Importantly, the projection-based embedded discrete fracture model is incorporated into the framework to describe fractures with varying conductivities. Impacts of fracture location, inclination angle, and fracture-matrix permeability ratio are systemically studied for a single fracture system. Moreover, the interplay between viscous and gravity forces in such fractured systems is analyzed. Results indicate that the fracture exhibits differing effects regarding different trapping mechanisms. Generally speaking, highly-conductive fractures facilitate dissolution trapping while weakening residual trapping, and flow barriers can assist dissolution trapping for systems with a relatively low gravity number. The findings from the test cases for single fracture geometries are found applicable to a larger-scale domain with complex fracture networks. This indicates the scalability of the study for field-relevant applications.Numerical AnalysisPetroleum Engineerin