1 research outputs found
Planar 17O NMR study of Pr_yY_{1-y}Ba_2Cu_3O_{6+x}
We report the planar ^{17}O NMR shift in Pr substituted YBa_{2}Cu_{3}O_{6+x},
which at x=1 exhibits a characteristic pseudogap temperature dependence,
confirming that Pr reduces the concentration of mobile holes in the CuO_{2}
planes. Our estimate of the rate of this counterdoping effect, obtained by
comparison with the shift in pure samples with reduced oxygen content, is found
insufficient to explain the observed reduction of T_c. From the temperature
dependent magnetic broadening of the ^{17}O NMR we conclude that the Pr moment
and the local magnetic defect induced in the CuO_2 planes produce a long range
spin polarization in the planes, which is likely associated with the extra
reduction of T_c. We find a qualitatively different behaviour in the oxygen
depleted Pr_yY_{1-y}Ba_2Cu_3O_{6.6}, i.e. the suppression of T is nearly
the same, but the magnetic broadening of the ^{17}O NMR appears weaker. This
difference may signal a weaker coupling of the Pr to the planes in the
underdoped compound, which might be linked with the larger Pr to CuO_2 plane
distance, and correspondingly weaker hybridization.Comment: 8 pages, 9 figures, accepted in Phys Rev