2,143 research outputs found
Incidence of the Tomonaga-Luttinger liquid state on the NMR spin lattice relaxation in Carbon Nanotubes
We report 13C nuclear magnetic resonance measurements on single wall carbon
nanotube (SWCNT) bundles. The temperature dependence of the nuclear
spin-lattice relaxation rate, 1/T1, exhibits a power-law variation, as expected
for a Tomonage-Luttinger liquid (TLL). The observed exponent is smaller than
that expected for the two band TLL model. A departure from the power law is
observed only at low T, where thermal and electronic Zeeman energy merge.
Extrapolation to zero magnetic field indicates gapless spin excitations. The
wide T range on which power-law behavior is observed suggests that SWCNT is so
far the best realization of a one-dimensional quantum metal.Comment: 5 pages, 4 figure
Spin Dynamics at the Mott Transition and in the Metallic State of the Cs_{3}C_{60} Superconducting Phases
We present here ^{13}C and ^{133}Cs NMR spin lattice relaxation T_{1} data in
the A15 and fcc-Cs_{3}C_{60} phases for increasing hydrostatic pressure through
the transition at p_{c} from a Mott insulator to a superconductor. We evidence
that for p>> p_{c} the (T_{1}T)^{-1} data above T_{c} display metallic like
Korringa constant values which match quantitatively previous data taken on
other A_{3}C_{60} compounds. However below the pressure for which T_{c} goes
through a maximum, (T_{1}T)^{-1} is markedly increased with respect to the
Korringa values expected in a simple BCS scenario. This points out the
importance of electronic correlations near the Mott transition. For p > p_{c}
singular T dependences of (T_{1}T)^{-1} are detected for T >> T_{c}. It will be
shown that they can be ascribed to a large variation with temperature of the
Mott transition pressure p_{c} towards a liquid-gas like critical point, as
found at high T for usual Mott transitions.Comment: 6 pages, 6 figures, submitted to EP
59Co Nuclear Quadrupole Resonance Studies of Superconducting and Non-superconducting Bilayer Water Intercalated Sodium Cobalt Oxides NaxCoO2.yH2O
We report 59Co nuclear quadrupole resonance (NQR) studies of bilayer water
intercalated sodium cobalt oxides NaxCoO2.yH2O (BLH) with the superconducting
transition temperatures, 2 K < T_c <= 4.6 K, as well as a magnetic BLH sample
without superconductivity. We obtained a magnetic phase diagram of T_c and the
magnetic ordering temperature T_M against the peak frequency nu_3 59Co NQR
transition I_z = +- 5/2 +-7/2 and found a dome shape superconducting phase.
The 59Co NQR spectrum of the non-superconducting BLH shows a broadening below
T_M without the critical divergence of 1/T_1 and 1/T_2, suggesting an
unconventional magnetic ordering. The degree of the enhancement of 1/T_1T at
low temperatures increases with the increase of nu_3 though the optimal
nu_3~12.30 MHz. In the NaxCoO2.yH2O system, the optimal-T_c superconductivity
emerges close to the magnetic instability. T_c is suppressed near the phase
boundary at nu_3~12.50 MHz, which is not a conventional magnetic quantum
critical point.Comment: 4 pages, 5 figure
Superconducting Properties of MgB2 Bulk Materials Prepared by High Pressure Sintering
High-density bulk materials of a newly discovered 40K intermetallic MgB2
superconductor were prepared by high pressure sintering. Superconducting
transition with the onset temperature of 39K was confirmed by both magnetic and
resistive measurements. Magnetization versus field (M-H) curve shows the
behavior of a typical Type II superconductor and the lower critical field
Hc1(0) estimated from M-H curve is 0.032T. The bulk sample shows good
connection between grains and critical current density Jc estimated from the
magnetization hysteresis using sample size was 2x104A/cm2 at 20K and 1T. Upper
critical field Hc2(0) determined by extrapolating the onset of resistive
transition and assuming a dirty limit is 18T.Comment: 3Pages PD
Electron-Phonon mechanism for Superconductivity in NaCoO: Valence-Band Suhl-Kondo effect Driven by Shear Phonons
To study the possible mechanism of superconductivity in NaCoO,
we examine the interaction between all the relevant optical phonons (breathing
and shear phonons) and -electrons of Co-ions, and study
the transition temperature for a s-wave superconductivity. The obtained is very low when the -valence-bands are far below the Fermi level.
However, is strongly enhanced when the top of the
-valence-bands is close to the Fermi level (say -50meV), thanks to
interband hopping of Cooper pairs caused by shear phonons. This ``valence-band
Suhl-Kondo mechanism'' due to shear phonons is significant to understand the
superconductivity in NaCoO. By the same mechanism, the kink
structure of the band-dispersion observed by ARPES, which indicates the strong
mass-enhancement () due to optical phonons, is also explained.Comment: 5 pages, 4 figures; v2:Added references, published in J. Phys. Soc.
Jp
23Na NMR study of non-superconducting double-layer hydrate NaxCoO2.yH2O
We report 23Na NMR studies of the polycrystalline samples of double-layer
hydrated cobalt oxides NaxCoO2.yH2O (x ~ 0.35 and y ~ 1.3) with the
superconducting transition temperatures Tc < 1.8K and ~4.5K, and the dehydrated
NaxCoO2 (x ~ 0.35). The hyperfine field and the electric field gradient at the
Na sites in the non-hydrated Na0.7CoO2 and the dehydrated Na0.35CoO2 are found
to be significantly reduced by the hydration, which indicates a strong
shielding effect of the intercalated water molecules on the Na sites. The
temperature dependence of 23 Na nuclear spin-lattice relaxation rate 1/23T1 of
the non-superconducting double-layer hydrate NaxCoO2.yH2O is found to be
similar to that of the non-hydrated Na0.7CoO2, whose spin dynamics is
understood by A-type (intra-layer ferromagnetic and inter-layer
antiferromagnetic) spin fluctuations. The superconducting phase is located
close to the quantum critical point with the A-type magnetic instability.Comment: 4 pages, 4 figure
Anisotropic Behavior of Knight Shift in Superconducting State of Na_xCoO_2yH_2O
The Co Knight shift was measured in an aligned powder sample of
Na_xCoO_2yH_2O, which shows superconductivity at T_c \sim 4.6 K. The
Knight-shift components parallel (K_c) and perpendicular to the c-axis (along
the ab plane K_{ab}) were measured in both the normal and superconducting (SC)
states. The temperature dependences of K_{ab} and K_c are scaled with the bulk
susceptibility, which shows that the microscopic susceptibility deduced from
the Knight shift is related to Co-3d spins. In the SC state, the Knight shift
shows an anisotropic temperature dependence: K_{ab} decreases below 5 K,
whereas K_c does not decrease within experimental accuracy. This result raises
the possibility that spin-triplet superconductivity with the spin component of
the pairs directed along the c-axis is realized in Na_xCoO_2yH_2O.Comment: 5 pages, 5 figures, to be published in Journal of Physical Society of
Japan vol. 75, No.
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