403 research outputs found
Magnetic field dependence of charge stripe order in La2-xBaxCuO4 (x~1/8)
We have carried out a detailed investigation of the magnetic field dependence
of charge ordering in La2-xBaxCuO4 (x~1/8) utilizing high-resolution x-ray
scattering. We find that the charge order correlation length increases as the
magnetic field greater than ~5T is applied in the superconducting phase (T=2K).
The observed unusual field dependence of the charge order correlation length
suggests that the static charge stripe order competes with the superconducting
ground state in this sample.Comment: 4 pages, 4 figure
Doping dependence of charge-transfer excitations in La_{2-x}Sr_xCuO_4
We report a resonant inelastic x-ray scattering (RIXS) study of the doping
dependence of charge-transfer excitations in . The mome
ntum dependence of these charge excitations are studied over the whole
Brillouin zone in underdoped (x=0.05) and optimally doped (x=0.17) samples, and
compared with that of the undoped (x=0) sample. We observe a large change in
the RIXS spectra between the x=0 and x=0.17 sample, while the RIXS spectra of
the x=0.05 sample are similar to that of the x=0 sample. The most prominent
effect of doped-holes on the charge excitation spectra is the appearance of a
continuum of intensity, which exhibits a strong momentum-dependence below 2 eV.
For the x=0.17 sample, some of the spectral weight from the lowest-lying
charge-transfer excitation of the undoped compound is transferred to the
continuum intensity below the gap, in agreement with earlier optical studies.
However, the higher energy charge-transfer excitation carries significant
spectral weight even for the x=0.17 sample. The doping dependence of the
dispersion of this charge-transfer excitation is also discussed and compared
with recent theoretical calculations.Comment: 7 pages, 6 figures, to appear in Phys. Rev.
Resonant inelastic X-ray scattering study of overdoped LaSrCuO
Resonant inelastic x-ray scattering (RIXS) at the copper K absorption edge
has been performed for heavily overdoped samples of LaSrCuO
with and 0.30. We have observed the charge transfer and
molecular-orbital excitations which exhibit resonances at incident energies of
and 8.998 keV, respectively. From a comparison with previous
results on undoped and optimally-doped samples, we determine that the
charge-transfer excitation energy increases monotonically as doping increases.
In addition, the -dependences of the RIXS spectral weight and absorption
spectrum exhibit no clear peak at keV in contrast to results in
the underdoped samples. The low-energy ( eV) continuum excitation
intensity has been studied utilizing the high energy resolution of 0.13 eV
(FWHM). A comparison of the RIXS profiles at and
indicates that the continuum intensity exists even at in the
overdoped samples, whereas it has been reported only at and
for the sample. Furthermore, we also found an additional excitation on
top of the continuum intensity at the and positions.Comment: 7 pages, 7 figure
Resonant inelastic x-ray scattering study of charge excitations in La2CuO4
We report a resonant inelastic x-ray scattering study of the dispersion
relations of charge transfer excitations in insulating LaCuO. These
data reveal two peaks, both of which show two-dimensional characteristics. The
lowest energy excitation has a gap energy of eV at the zone center,
and a dispersion of eV. The spectral weight of this mode becomes
dramatically smaller around (, ). The second peak shows a smaller
dispersion ( eV) with a zone-center energy of eV. We argue
that these are both highly dispersive exciton modes damped by the presence of
the electron-hole continuum.Comment: 5 pages, 3 figure
Correlated Polarons in Dissimilar Perovskite Manganites
We report x-ray scattering studies of broad peaks located at a (0.5 0 0)/(0
0.5 0)-type wavevector in the paramagnetic insulating phases of
La_{0.7}Ca_{0.3}MnO_{3} and Pr_{0.7}Ca_{0.3}MnO_{3}. We interpret the
scattering in terms of correlated polarons and measure isotropic correlation
lengths of 1-2 lattice constants in both samples. Based on the wavevector and
correlation lengths, the correlated polarons are found to be consistent with
CE-type bipolarons. Differences in behavior between the samples arise as they
are cooled through their respective transition temperatures and become
ferromagnetic metallic (La_{0.7}Ca_{0.3}MnO_{3}) or charge and orbitally
ordered insulating (Pr_{0.7}Ca_{0.3}MnO_{3}). Since the primary difference
between the two samples is the trivalent cation size, these results illustrate
the robust nature of the correlated polarons to variations in the relative
strength of the electron-phonon coupling, and the sensitivity of the
low-temperature ground state to such variations.Comment: 13 pages, 6 figure
Development of an instrument for measuring different types of cognitive load
According to cognitive load theory, instructions can impose three types of cognitive load on the learner: intrinsic load, extraneous load, and germane load. Proper measurement of the different types of cognitive load can help us understand why the effectiveness and efficiency of learning environments may differ as a function of instructional formats and learner characteristics. In this article, we present a ten-item instrument for the measurement of the three types of cognitive load. Principal component analysis on data from a lecture in statistics for PhD students (n = 56) in psychology and health sciences revealed a three-component solution, consistent with the types of load that the different items were intended to measure. This solution was confirmed by a confirmatory factor analysis of data from three lectures in statistics for different cohorts of bachelor students in the social and health sciences (ns = 171, 136, and 148), and received further support from a randomized experiment with university freshmen in the health sciences (n = 58)
Holographic analysis of diffraction structure factors
We combine the theory of inside-source/inside-detector x-ray fluorescence
holography and Kossel lines/x ray standing waves in kinematic approximation to
directly obtain the phases of the diffraction structure factors. The influence
of Kossel lines and standing waves on holography is also discussed. We obtain
partial phase determination from experimental data obtaining the sign of the
real part of the structure factor for several reciprocal lattice vectors of a
vanadium crystal.Comment: 4 pages, 3 figures, submitte
Orbital Correlations in Doped Manganites
We review our recent x-ray scattering studies of charge and orbital order in
doped manganites, with specific emphasis on the role of orbital correlations in
Pr_1-xCa_xMnO_3. For x=0.25, we find an orbital structure indistinguishable
from the undoped structure with long range orbital order at low temperatures.
For dopings 0.3<x<0.5, we find scattering consistent with a charge and
orbitally ordered CE-type structure. While in each case the charge order peaks
are resolution limited, the orbital order exhibits only short range
correlations. We report the doping dependence of the correlation length and
discuss the connection between the orbital correlations and the finite magnetic
correlation length observed on the Mn^3+ sublattice with neutron scattering
techniques. The physical origin of these domains, which appear to be isotropic,
remains unclear. We find that weak orbital correlations persist well above the
phase transitions, with a correlation length of 1-2 lattice constants at high
temperatures. Significantly, we observe similar correlations at high
temperatures in La_0.7Ca_0.3MnO_3, which does not have an orbitally ordered
ground state, and we conclude that such correlations are robust to variations
in the relative strength of the electron-phonon coupling.Comment: 22 pagegs, 7 figure
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